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"edge_dark_ratios": { "top": 0.022, "bottom": 0.115, "left": 0.153, "right": 0.083 }, "excluded_risk_level": "high", "region_id": "p1:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/12", "page": 1, "label": "text", "order": 12000, "source_page_order": 13, "layout_order": 13, "layout_page_order": 14, "bbox": [ 202.17, 310.46, 355.49, 93.18 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Li and Mn rich (LMR) layered oxides, written as x Li2MnO3 \u0001 (1 \u0000 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure and superior performance of LMR oxides make them one of the most promising candidates for the next-generation cathode materials. However, the commercialization of these materials is hindered by several drawbacks, such as low initial Coulombic efficiency, the degradation of voltage and capacity during cycling, and poor rate performance. This review summarizes research progress in solving these concerns of LMR cathodes over the past decade by following three classes of strategies: morphology design, bulk design, and surface modification. We elaborate on the processing procedures, electrochemical performance, mechanisms, and limitations of each approach, and finally put forward the concerns left and the possible solutions for the commercialization of LMR cathodes.", "text_preview": "Li and Mn rich (LMR) layered oxides, written as x Li2MnO3 \u0001 (1 \u0000 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure an…", "word_count": 150, "cleaned_text": "Li and Mn rich (LMR) layered oxides, written as x Li2MnO3 \u0001 (1 \u0000 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure and superior performance of LMR oxides make them one of the most promising candidates for the next-generation cathode materials. However, the commercialization of these materials is hindered by several drawbacks, such as low initial Coulombic efficiency, the degradation of voltage and capacity during cycling, and poor rate performance. This review summarizes research progress in solving these concerns of LMR cathodes over the past decade by following three classes of strategies: morphology design, bulk design, and surface modification. We elaborate on the processing procedures, electrochemical performance, mechanisms, and limitations of each approach, and finally put forward the concerns left and the possible solutions for the commercialization of LMR cathodes.", "cleaned_text_preview": "Li and Mn rich (LMR) layered oxides, written as x Li2MnO3 \u0001 (1 \u0000 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure an…", "included_in_body": false, "body_decision_reason": "inside_abstract", "parser_body_decision_reason": "inside_abstract", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p1:body_region:0", "role_guess": "abstract_candidate", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", 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"layout_order": 15, "layout_page_order": 16, "bbox": [ 37.59, 364.44, 116.82, 40.52 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective", "text_preview": "Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective", "word_count": 15, "cleaned_text": "Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective", "cleaned_text_preview": "Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective", "included_in_body": false, "body_decision_reason": "front_matter_heading", "parser_body_decision_reason": "front_matter_heading", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "front_matter_heading", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": true, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": "front_matter", "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.009, "bottom": 0.116, "left": 0.179, "right": 0.013 }, "excluded_risk_level": "low", "region_id": "p1:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/13", "page": 1, "label": "text", "order": 13000, "source_page_order": 14, "layout_order": 16, "layout_page_order": 17, "bbox": [ 202.17, 404.52, 355.42, 18.23 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.", "text_preview": "Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.", "word_count": 24, "cleaned_text": "Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press.", "cleaned_text_preview": "Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press.", "included_in_body": false, "body_decision_reason": "first_page_metadata", "parser_body_decision_reason": "first_page_metadata", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p1:body_region:0", "role_guess": "metadata", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": true, "affiliation_block": true, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.004, "bottom": 0.056, "left": 0.048, "right": 0.107 }, "excluded_risk_level": "low", "region_id": "p1:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/14", "page": 1, "label": "text", "order": 14000, "source_page_order": 15, "layout_order": 17, "layout_page_order": 18, "bbox": [ 120.08, 460.31, 168.57, 57.35 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking University. His main research work is Li-Rich cathode materials with high voltage and high energy density for Li ion batteries.", "text_preview": "Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking Uni…", "word_count": 54, "cleaned_text": "Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking University. His main research work is Li-Rich cathode materials with high voltage and high energy density for Li ion batteries.", "cleaned_text_preview": "Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking Uni…", "included_in_body": false, "body_decision_reason": "inside_front_matter", "parser_body_decision_reason": "inside_front_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "reference", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": true, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.135, "bottom": 0.053, "left": 0.154, "right": 0.051 }, "excluded_risk_level": "low", "region_id": "p1:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/15", "page": 1, "label": "footnote", "order": 15000, "source_page_order": 16, "layout_order": 18, "layout_page_order": 19, "bbox": [ 42.07, 692.51, 264.1, 18.63 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan).", "text_preview": "⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan).", "word_count": 11, "cleaned_text": "⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan).", "cleaned_text_preview": "⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan).", "included_in_body": false, "body_decision_reason": "first_page_metadata", "parser_body_decision_reason": "first_page_metadata", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "footnote", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": true, "affiliation_block": true, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.02, "bottom": 0.109, "left": 0.048, "right": 0.024 }, "excluded_risk_level": "low", "region_id": "p1:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/16", "page": 1, "label": "footnote", "order": 16000, "source_page_order": 17, "layout_order": 19, "layout_page_order": 20, "bbox": [ 43.09, 712.68, 148.31, 7.21 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "1 These authors contributed equally to this work.", "text_preview": "1 These authors contributed equally to this work.", "word_count": 8, "cleaned_text": "1 These authors contributed equally to this work.", "cleaned_text_preview": "1 These authors contributed equally to this work.", "included_in_body": false, "body_decision_reason": "outside_body_flow_footnote", "parser_body_decision_reason": "outside_body_flow_footnote", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "footnote", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.033, "bottom": 0.1, "left": 0.076, "right": 0.045 }, "excluded_risk_level": "low", "region_id": "p1:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/21", "page": 1, "label": "page_footer", "order": 21000, "source_page_order": 22, "layout_order": 20, "layout_page_order": 21, "bbox": [ 37.59, 731.92, 136.91, 5.93 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "https://doi.org/10.1016/j.jechem.2021.01.034", "text_preview": "https://doi.org/10.1016/j.jechem.2021.01.034", "word_count": 1, "cleaned_text": "", "cleaned_text_preview": "", "included_in_body": false, "body_decision_reason": "first_page_metadata", "parser_body_decision_reason": "first_page_metadata", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "page_footer", "zone": "bottom_margin", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": true, "metadata_line": true, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": true, "edge_dark_ratios": { "top": 0.125, "bottom": 0.11, "left": 0.259, "right": 0.278 }, "excluded_risk_level": "low", "region_id": "p1:bottom_margin:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/17", "page": 1, "label": "text", "order": 17000, "source_page_order": 18, "layout_order": 21, "layout_page_order": 22, "bbox": [ 389.08, 458.95, 168.57, 48.74 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion batteries.", "text_preview": "Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research intere…", "word_count": 46, "cleaned_text": "Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion batteries.", "cleaned_text_preview": "Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research intere…", "included_in_body": false, "body_decision_reason": "inside_front_matter", "parser_body_decision_reason": "inside_front_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p1:body_region:0", "role_guess": "body_candidate_excluded", "zone": "page_body", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.147, "bottom": 0.043, "left": 0.128, "right": 0.128 }, "excluded_risk_level": "high", "region_id": "p1:page_body:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/22", "page": 1, "label": "page_footer", "order": 22000, "source_page_order": 23, "layout_order": 22, "layout_page_order": 23, "bbox": [ 37.59, 738.73, 520.05, 8.3 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.", "text_preview": "2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.", "word_count": 25, "cleaned_text": "2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press.", "cleaned_text_preview": "2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. 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Li, Z. Li, C. Chen et al.", "text_preview": "Y. Li, Z. Li, C. Chen et al.", "word_count": 8, "cleaned_text": "Y. Li, Z. Li, C. Chen et al.", "cleaned_text_preview": "Y. Li, Z. Li, C. 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He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion and sodium ion batteries.", "text_preview": "Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His researc…", "word_count": 50, "cleaned_text": "Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion and sodium ion batteries.", "cleaned_text_preview": "Cong Chen received his B.S. degree from South China University of Technology in 2018. 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He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. His main research interests include advanced silicon carbon materials for lithium ion batteries (LIBs) and advanced technology for interface research in LIBs, such as in-situ AFM and EQCM.", "text_preview": "Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. Hi…", "word_count": 62, "cleaned_text": "Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. 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Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on development of functional materials for energy storage.", "text_preview": "Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests ma…", "word_count": 44, "cleaned_text": "Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on development of functional materials for energy storage.", "cleaned_text_preview": "Shenyang Xu received his B.S. degree from Tiangong University in 2015. 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She has over 10 years' experience in material characterization using wide range of analytical tools including FIB, SEM and TEM. Her research interests mainly focus on the FIB and TEM characterization of battery materials.", "text_preview": "Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FI…", "word_count": 50, "cleaned_text": "Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FIB, SEM and TEM. Her research interests mainly focus on the FIB and TEM characterization of battery materials.", "cleaned_text_preview": "Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. 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He has over 10 years' experience in material characterization using wide range of analytical tools including XRD, XPS, SEM and TEM. His research interests mainly focus on the ex/in-situ TEM and ex/in-situ XRD characterization of battery materials.", "text_preview": "Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools includi…", "word_count": 53, "cleaned_text": "Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools including XRD, XPS, SEM and TEM. 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He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institute of Technology in 2006. He worked at Velocys during 2006-2011 and UES during 2011-2014.", "text_preview": "Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institut…", "word_count": 46, "cleaned_text": "Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institute of Technology in 2006. He worked at Velocys during 2006-2011 and UES during 2011-2014.", "cleaned_text_preview": "Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. 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From 2014 to 2018, he was a postdoc at School of Advanced Materials, Peking University, and became an assistant research professor since 2018. Meanwhile, he was a research scholar in Brookhaven National Lab from 2016 to 2019, then in the University of Chicago since 2019. He has been engaged in the fields of electrode materials for Liion batteries, crystal growth and structure analysis of nonlinear optical crystals.", "text_preview": "Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, h…", "word_count": 100, "cleaned_text": "Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, he was a postdoc at School of Advanced Materials, Peking University, and became an assistant research professor since 2018. Meanwhile, he was a research scholar in Brookhaven National Lab from 2016 to 2019, then in the University of Chicago since 2019. He has been engaged in the fields of electrode materials for Liion batteries, crystal growth and structure analysis of nonlinear optical crystals.", "cleaned_text_preview": "Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. 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Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathclyde, Glasgow, UK, with ''Patrick D. Ritchie Prize' for the best Ph.D. in 1994. With more than a decade experience in large international incorporations, Prof. Pan has been engaged in fundamental research and product development of novel optoelectronic and energy storage materials and devices. As Chief Scientist, Prof. Pan led eight entities in Shenzhen to win 150 million RMB grant for the national new energy vehicles", "text_preview": "Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathc…", "word_count": 99, "cleaned_text": "Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathclyde, Glasgow, UK, with ''Patrick D. Ritchie Prize' for the best Ph.D. in 1994. With more than a decade experience in large international incorporations, Prof. Pan has been engaged in fundamental research and product development of novel optoelectronic and energy storage materials and devices. As Chief Scientist, Prof. Pan led eight entities in Shenzhen to win 150 million RMB grant for the national new energy vehicles", "cleaned_text_preview": "Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. 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(a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d synthesized from two different precursors (C for conventional precursor and H for hierarchically structured precursor). Reproduced from Ref. [27] with permission from American Chemical Society. (d) Structural scheme showing the honeycomb pattern consisting of Li@Mn6 superstructure units in LMR layered oxide. Reproduced from Ref. [29]) with permission from Royal Society of Chemistry.", "text_preview": "Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d …", "word_count": 88, "cleaned_text": "Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d synthesized from two different precursors (C for conventional precursor and H for hierarchically structured precursor). Reproduced from Ref. [27] with permission from American Chemical Society. (d) Structural scheme showing the honeycomb pattern consisting of Li@Mn6 superstructure units in LMR layered oxide. Reproduced from Ref. [29]) with permission from Royal Society of Chemistry.", "cleaned_text_preview": "Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d …", "included_in_body": false, "body_decision_reason": "outside_body_flow_caption", "parser_body_decision_reason": "outside_body_flow_caption", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "caption", "zone": "body_zone", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.054, "bottom": 0.075, "left": 0.167, "right": 0.167 }, "excluded_risk_level": "low", "region_id": "p3:body_zone:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/42", "page": 3, "label": "caption", "order": 42000, "source_page_order": 7, "layout_order": 42, "layout_page_order": 7, "bbox": [ 37.59, 613.15, 182.82, 14.49 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Table 1 Researches about understanding the structure of LMR oxides.", "text_preview": "Table 1 Researches about understanding the structure of LMR oxides.", "word_count": 10, "cleaned_text": "Table 1 Researches about understanding the structure of LMR oxides.", "cleaned_text_preview": "Table 1 Researches about understanding the structure of LMR oxides.", "included_in_body": false, "body_decision_reason": "outside_body_flow_caption", "parser_body_decision_reason": "outside_body_flow_caption", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:0", "role_guess": "caption", "zone": "body_zone", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.034, "bottom": 0.183, "left": 0.183, "right": 0.04 }, "excluded_risk_level": "low", "region_id": "p3:body_zone:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/43", "page": 3, "label": "page_footer", "order": 43000, "source_page_order": 8, "layout_order": 43, "layout_page_order": 8, "bbox": [ 291.91, 764.24, 11.38, 5.93 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "370", "text_preview": "370", "word_count": 1, "cleaned_text": "370", "cleaned_text_preview": "370", "included_in_body": false, "body_decision_reason": "docling_page_footer", "parser_body_decision_reason": "docling_page_footer", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "page_footer", "zone": "bottom_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": true, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.216, "bottom": 0.088, "left": 0.093, "right": 0.259 }, "excluded_risk_level": "low", "region_id": "p3:bottom_margin:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/44", "page": 4, "label": "page_header", "order": 44000, "source_page_order": 2, "layout_order": 44, "layout_page_order": 1, "bbox": [ 37.59, 47.86, 69.84, 6.37 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Y. 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(a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chemical Society. (c) p DOS of O 2 p orbitals and Mn 3 d orbitals in Li2MnO3 and the corresponding oxygen environment model. Reproduced from Ref. [47] with permission from Springer Nature. (d) Cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 synthesized by two different synthesis methods at 0.1 C in the voltage range of 2.0-4.8 V. (e) The corresponding capacity-voltage profiles of the re-synthesized Li1.2Ni0.13Co0.13Mn0.54O2 in (d). Reproduced from Ref. [53] with permission from Elsevier. (f) Schematic representation for the structural transformation of trigonal LiMO2 component ( R -3m) and monoclinic Li2MnO3 component ( C 2/ m ) in Li1.2Ni0.1Mn0.525Co0.175O2 during cycling. Reproduced from Ref. [54] with permission from American Chemical Society. (g) Selected area electron diffraction (SAED) pattern obtained along [0001] zone axis of Li1.2Co0.1Mn0.55Ni0.15O2 cathode at the charging voltage of 4.5 V. (h) Schematic diagram of TM migration in Li1.2Co0.1Mn0.55Ni0.15O2 cathode when holding at 4.5 V. Reproduced from Ref. [55] with permission from Royal Society of Chemistry.", "text_preview": "Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chem…", "word_count": 186, "cleaned_text": "Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chemical Society. (c) p DOS of O 2 p orbitals and Mn 3 d orbitals in Li2MnO3 and the corresponding oxygen environment model. Reproduced from Ref. [47] with permission from Springer Nature. (d) Cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 synthesized by two different synthesis methods at 0.1 C in the voltage range of 2.0-4.8 V. (e) The corresponding capacity-voltage profiles of the re-synthesized Li1.2Ni0.13Co0.13Mn0.54O2 in (d). Reproduced from Ref. [53] with permission from Elsevier. (f) Schematic representation for the structural transformation of trigonal LiMO2 component ( R -3m) and monoclinic Li2MnO3 component ( C 2/ m ) in Li1.2Ni0.1Mn0.525Co0.175O2 during cycling. Reproduced from Ref. [54] with permission from American Chemical Society. (g) Selected area electron diffraction (SAED) pattern obtained along [0001] zone axis of Li1.2Co0.1Mn0.55Ni0.15O2 cathode at the charging voltage of 4.5 V. (h) Schematic diagram of TM migration in Li1.2Co0.1Mn0.55Ni0.15O2 cathode when holding at 4.5 V. Reproduced from Ref. [55] with permission from Royal Society of Chemistry.", "cleaned_text_preview": "Fig. 2. 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[a] ICE denotes initial Coulombic efficiency.", "text_preview": "Notes. [a] ICE denotes initial Coulombic efficiency.", "word_count": 7, "cleaned_text": "Notes. [a] ICE denotes initial Coulombic efficiency.", "cleaned_text_preview": "Notes. 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(a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3 \u0001 (1x )LiMnO2 nanorods. Reproduced from Ref. [63] with permission from Elsevier. (c) Schematic illustration of the synthetic process of orthogonally arranged nanoplates. Reproduced from Ref. [64] with permission from American Chemical Society. (d) Scheme of the fabrication process of 3D hollow porous bowl-shaped Li1.2Ni0.13Co0.13Mn0.54O2 particles. Reproduced from Ref. [66] with permission from Elsevier. (e) Schematic diagram of the suppression of voltage fading through a preferred orientation (110) plane. Reproduced from Ref. [67] with permission from Royal Society of Chemistry.", "text_preview": "Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. 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(a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100 mA g \u0000 1 . Reproduced from Ref. [84] with permission from Royal Society of Chemistry. (c) Schematic diagram of pristine LMR, LMR with surface-doped with Na (Na-LMR) and LMR with homogenously Na doping (Na/SDS-LMR) before cycling and after 200 cycles. Reproduced from Ref. [85] with permission from Wiley-VCH. (d) Schematic illustration for the structure of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . (e) The rate performance of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . Reproduced from Ref. [88] with permission from Royal Society of Chemistry. (f) Schematic diagram of Na and F co-doping in Li1.2Ni0.2Mn0.6O2 cathode. (g) The cycling performance of Li1.2Ni0.2Mn0.6O2 cathode (LNMO), Na doped LNMO cathode (Na-LNMO), F doped LNMO cathode (F-LNMO) and Na and F co-doped LNMO cathode (Na&FLNMO) at 0.1 C in the voltage range of 2.0-4.8 V. Reproduced from Ref. [95] with permission from Elsevier.", "text_preview": "Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100…", "word_count": 158, "cleaned_text": "Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100 mA g \u0000 1 . Reproduced from Ref. [84] with permission from Royal Society of Chemistry. (c) Schematic diagram of pristine LMR, LMR with surface-doped with Na (Na-LMR) and LMR with homogenously Na doping (Na/SDS-LMR) before cycling and after 200 cycles. Reproduced from Ref. [85] with permission from Wiley-VCH. (d) Schematic illustration for the structure of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . (e) The rate performance of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . Reproduced from Ref. [88] with permission from Royal Society of Chemistry. (f) Schematic diagram of Na and F co-doping in Li1.2Ni0.2Mn0.6O2 cathode. (g) The cycling performance of Li1.2Ni0.2Mn0.6O2 cathode (LNMO), Na doped LNMO cathode (Na-LNMO), F doped LNMO cathode (F-LNMO) and Na and F co-doped LNMO cathode (Na&FLNMO) at 0.1 C in the voltage range of 2.0-4.8 V. Reproduced from Ref. [95] with permission from Elsevier.", "cleaned_text_preview": "Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100…", "included_in_body": false, "body_decision_reason": "outside_body_flow_caption", "parser_body_decision_reason": "outside_body_flow_caption", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "caption", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], 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(a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from Elsevier. (c) Schematic illustration of different oxygen migration model in bare and SnO2 coated Li1.2Ni0.13Co0.13Mn0.54O2 (filled with oxygen vacancies at the surface). Reproduced from Ref. [103] with permission from Elsevier. (d) Schematic diagram for the surficial structure of AlPO4 coated LMR oxide. (e) The Coulombic efficiency of the LMR oxides coated with different ALD cycles of AlPO4 during long-term cycling. Reproduced from Ref. [104] with permission from Elsevier.", "text_preview": "Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from E…", "word_count": 95, "cleaned_text": "Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from Elsevier. (c) Schematic illustration of different oxygen migration model in bare and SnO2 coated Li1.2Ni0.13Co0.13Mn0.54O2 (filled with oxygen vacancies at the surface). Reproduced from Ref. [103] with permission from Elsevier. (d) Schematic diagram for the surficial structure of AlPO4 coated LMR oxide. (e) The Coulombic efficiency of the LMR oxides coated with different ALD cycles of AlPO4 during long-term cycling. Reproduced from Ref. [104] with permission from Elsevier.", "cleaned_text_preview": "Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. 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[116] with permission from Elsevier. (e) Cycle performance of uncoated Li1.2Ni0.13Co0.13Mn0.54O2 (LR) and Mg2TiO4 coated Li1.2Ni0.13Co0.13Mn0.54O2 (LR@MTO) at 2 C. Reproduced from Ref. [117] with permission from John Wiley and Sons.", "cleaned_text_preview": "Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. 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(a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li1.2Mn0.54Ni0.13Co0.13O2 oxide in the bulk and the spinel structure at the surface after GO modification. Reproduced from Ref. [118] with permission from Royal Society of Chemistry. (c) The synthetic scheme of chemical adsorption to modified MoO2S2 at the surface of LMR cathode and the corresponding structure at each step. (d) HRTEM and the corresponding FFT and refined lattice images of the MoO2S2 modified LMR cathode. Reproduced from Ref. [119] with permission from American Chemical Society.", "text_preview": "Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li…", "word_count": 108, "cleaned_text": "Fig. 9. 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(a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode and un-modified cathode at C/3. (c) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode after 100 cycles along [100] zone axis and the corresponding atomic models. Reproduced from Ref. [122] with permission from American Chemical Society. (d) XRD patterns of Li1.2Ni0.16Mn0.56Co0.08O2 samples doped by different Al contents. (e) The average voltage of the Li1.2Ni0.16Mn0.56Co0.08O2 cathode doped by different Al contents during cycling at 0.1 C. Reproduced from Ref. [124] with permission from John Wiley and Sons.", "text_preview": "Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. 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