page source_page_order layout_page_order layout_order ref label role_guess included_in_body excluded_risk_level body_decision_reason parser_body_decision_reason production_usage visual_asset_type visual_asset_label visual_asset_caption_preview truncation_marker inside_body_region body_region_id zone column column_index column_count region_id background_rgb background_class is_gray_background has_frame_evidence bbox text_preview cleaned_text_preview text cleaned_text 1 1 1 0 #/texts/0 page_header page_header False low docling_page_header docling_page_header False None top_margin column_2_of_2 2 2 p1:top_margin:column_2_of_2:white [255, 255, 255] white False False [228.36, 47.78, 129.01, 6.37] Journal of Power Sources 306 (2016) 70 e 77 Journal of Power Sources 306 (2016) 70 e 77 Journal of Power Sources 306 (2016) 70 e 77 Journal of Power Sources 306 (2016) 70 e 77 1 2 2 1 #/texts/1 text front_matter_heading False low first_page_metadata first_page_metadata False None page_body column_2_of_2 2 2 p1:page_body:column_2_of_2:gray [229, 229, 229] gray True False [216.51, 79.77, 156.17, 1.59] Contents lists available at ScienceDirect Contents lists available at ScienceDirect Contents lists available at ScienceDirect Contents lists available at ScienceDirect 1 3 3 2 #/texts/2 section_header title_candidate False low non_body_heading non_body_heading False None page_body column_2_of_2 2 2 p1:page_body:column_2_of_2:gray [229, 229, 229] gray True False [210.56, 98.49, 167.92, 12.99] Journal of Power Sources Journal of Power Sources Journal of Power Sources Journal of Power Sources 1 4 4 3 #/texts/3 text metadata False low first_page_metadata first_page_metadata False None page_body column_2_of_2 2 2 p1:page_body:column_2_of_2:gray [229, 229, 229] gray True False [165.09, 135.72, 258.93, 1.59] j o urnal homepage: www.elsevier.com/locate/jpowsour j o urnal homepage: j o urnal homepage: www.elsevier.com/locate/jpowsour j o urnal homepage: 1 5 5 4 #/texts/4 section_header title_candidate False low non_body_heading non_body_heading False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.83, 178.39, 420.44, 29.76] An investigation of functionalized electrolyte using succinonitrile additive for high voltage lithium-ion batteries An investigation of functionalized electrolyte using succinonitrile additive for high voltage lithium-ion batteries An investigation of functionalized electrolyte using succinonitrile additive for high voltage lithium-ion batteries An investigation of functionalized electrolyte using succinonitrile additive for high voltage lithium-ion batteries 1 6 6 5 #/texts/5 text affiliation False medium front_matter_author_line front_matter_author_line False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.83, 217.13, 438.2, 26.17] Renjie Chen a, b, * , Fan Liu a , Yan Chen a , Yusheng Ye a , Yongxin Huang a , Feng Wu a, b, ** , Li Li a, b Renjie Chen a, b, * , Fan Liu a , Yan Chen a , Yusheng Ye a , Yongxin Huang a , Feng Wu a, b, ** , Li Li a, b Renjie Chen a, b, * , Fan Liu a , Yan Chen a , Yusheng Ye a , Yongxin Huang a , Feng Wu a, b, ** , Li Li a, b Renjie Chen a, b, * , Fan Liu a , Yan Chen a , Yusheng Ye a , Yongxin Huang a , Feng Wu a, b, ** , Li Li a, b 1 7 7 6 #/texts/6 footnote footnote False low docling_footnote docling_footnote False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.82, 250.08, 437.89, 15.93] a School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China a School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China a School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China a School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China 1 8 8 7 #/texts/7 footnote footnote False low docling_footnote docling_footnote False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.83, 267.2, 250.38, 7.37] b Collaborative Innovation Center of Electric Vehicles in Beijing, Beijing 100081, China b Collaborative Innovation Center of Electric Vehicles in Beijing, Beijing 100081, China b Collaborative Innovation Center of Electric Vehicles in Beijing, Beijing 100081, China b Collaborative Innovation Center of Electric Vehicles in Beijing, Beijing 100081, China 1 9 9 8 #/texts/8 section_header front_matter_heading False low front_matter_heading front_matter_heading False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:unknown None unknown False False [32.83, 305.29, 86.34, 0.06] h i g h l i g h t s h i g h l i g h t s h i g h l i g h t s h i g h l i g h t s 1 13 13 12 #/texts/12 section_header front_matter_heading False low front_matter_heading front_matter_heading False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:unknown None unknown False False [32.83, 537.0, 95.61, 0.06] a r t i c l e i n f o a r t i c l e i n f o a r t i c l e i n f o a r t i c l e i n f o 1 14 14 13 #/texts/13 text unknown_text False high outside_body_flow outside_body_flow False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.83, 558.33, 107.65, 48.74] Article history: Received 16 July 2015 Received in revised form 27 October 2015 Accepted 28 October 2015 Available online 13 December 2015 Article history: Received 16 July 2015 Received in revised form 27 October 2015 Accepted 28 October 2015 Available online 13 December 2015 Article history: Received 16 July 2015 Received in revised form 27 October 2015 Accepted 28 October 2015 Available online 13 December 2015 Article history: Received 16 July 2015 Received in revised form 27 October 2015 Accepted 28 October 2015 Available online 13 December 2015 1 18 15 14 #/texts/17 footnote footnote False low first_page_metadata first_page_metadata False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.83, 648.88, 251.1, 24.01] * Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. * Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. * Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. * Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. 1 19 16 15 #/texts/18 footnote footnote False low first_page_metadata first_page_metadata False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.83, 675.13, 251.1, 23.95] ** Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. ** Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. ** Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. ** Corresponding author. School of Materials Science & Engineering, Beijing Key Laboratory of Environmental Science and Engineering, Beijing Institute of Technology, Beijing 100081, China. 1 20 17 16 #/texts/19 footnote footnote False low first_page_metadata first_page_metadata False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [32.83, 701.71, 250.98, 14.5] E-mail addresses: chenrj@bit.edu.cn (R. Chen), wufeng863@vip.sina.com (F. Wu). E-mail addresses: chenrj@bit.edu.cn (R. Chen), wufeng863@vip.sina.com (F. Wu). E-mail addresses: chenrj@bit.edu.cn (R. Chen), wufeng863@vip.sina.com (F. Wu). E-mail addresses: chenrj@bit.edu.cn (R. Chen), wufeng863@vip.sina.com (F. Wu). 1 21 18 17 #/texts/20 page_footer page_footer False low first_page_metadata first_page_metadata False None bottom_margin column_1_of_2 1 2 p1:bottom_margin:column_1_of_2:white [248, 251, 252] white False False [32.83, 728.64, 144.66, 5.94] http://dx.doi.org/10.1016/j.jpowsour.2015.10.105 http://dx.doi.org/10.1016/j.jpowsour.2015.10.105 1 22 19 18 #/texts/21 page_footer page_footer False low first_page_metadata first_page_metadata False None bottom_margin column_1_of_2 1 2 p1:bottom_margin:column_1_of_2:white [255, 255, 255] white False False [32.83, 735.78, 156.13, 7.43] 0378-7753/ © 2015 Elsevier B.V. All rights reserved. 0378-7753/ © 2015 Elsevier B.V. All rights reserved. 0378-7753/ © 2015 Elsevier B.V. All rights reserved. 0378-7753/ © 2015 Elsevier B.V. All rights reserved. 1 15 20 19 #/texts/14 section_header body_heading False low body_heading body_heading False None page_body column_2_of_2 2 2 p1:page_body:column_2_of_2:unknown None unknown False False [197.22, 305.29, 152.63, 0.06] g r a p h i c a l a b s t r a c t g r a p h i c a l a b s t r a c t g r a p h i c a l a b s t r a c t g r a p h i c a l a b s t r a c t 1 16 21 20 #/texts/15 section_header abstract_heading False low abstract_heading abstract_heading False None page_body column_2_of_2 2 2 p1:page_body:column_2_of_2:unknown None unknown False False [197.23, 537.0, 67.73, 0.06] a b s t r a c t a b s t r a c t a b s t r a c t a b s t r a c t 1 17 22 21 #/texts/16 text abstract_candidate False medium inside_abstract inside_abstract False None page_body column_2_of_2 2 2 p1:page_body:column_2_of_2:white [255, 255, 255] white False False [197.23, 551.28, 355.66, 73.58] Succinonitrile (SN) has been used as functional additive to improve the thermal stability and broaden the oxidation electrochemical window of commercial electrolyte 1 M LiPF6/EC/DEC (1:1, by volume) for highvoltage LIBs… Succinonitrile (SN) has been used as functional additive to improve the thermal stability and broaden the oxidation electrochemical window of commercial electrolyte 1 M LiPF6/EC/DEC (1:1, by volume) for highvoltage LIBs… Succinonitrile (SN) has been used as functional additive to improve the thermal stability and broaden the oxidation electrochemical window of commercial electrolyte 1 M LiPF6/EC/DEC (1:1, by volume) for highvoltage LIBs (cathode: Li1.2Ni0.2Mn0.6O2, anode: Li). 1 wt % SN-based electrolyte showed a wide electrochemical oxidation window of 5.4 V vs Li þ /Li and excellent thermal stability demonstrated by thermogravimetry (TG) and X-ray photoelectron spectroscopy (XPS), as well as theoretical analysis according to molecular orbital theory. The LNMO (Li1.2Ni0.2Mn0.6O2) battery with 1 wt % SN-based electrolyte showed better cyclability and capacity retention when charged to higher cut-off voltage. The improved battery performance is mainly attributed to the formation of uniform cathode electrolyte interface (CEI) Succinonitrile (SN) has been used as functional additive to improve the thermal stability and broaden the oxidation electrochemical window of commercial electrolyte 1 M LiPF6/EC/DEC (1:1, by volume) for highvoltage LIBs (cathode: Li1.2Ni0.2Mn0.6O2, anode: Li). 1 wt % SN-based electrolyte showed a wide electrochemical oxidation window of 5.4 V vs Li þ /Li and excellent thermal stability demonstrated by thermogravimetry (TG) and X-ray photoelectron spectroscopy (XPS), as well as theoretical analysis according to molecular orbital theory. The LNMO (Li1.2Ni0.2Mn0.6O2) battery with 1 wt % SN-based electrolyte showed better cyclability and capacity retention when charged to higher cut-off voltage. The improved battery performance is mainly attributed to the formation of uniform cathode electrolyte interface (CEI) 2 3 1 22 #/texts/24 text front_matter_heading False low front_matter_heading front_matter_heading True p2:body_region:0 front_matter column_1_of_2 1 2 p2:front_matter:column_1_of_2:white [255, 255, 255] white False False [42.52, 72.47, 51.66, 31.68] Keywords: Succinonitrile High voltage Thermal stability Keywords: Succinonitrile High voltage Thermal stability Keywords: Succinonitrile High voltage Thermal stability Keywords: Succinonitrile High voltage Thermal stability 2 4 2 23 #/texts/25 text abstract_candidate False medium inside_abstract inside_abstract True p2:body_region:0 front_matter column_1_of_2 1 2 p2:front_matter:column_1_of_2:white [255, 255, 255] white False False [42.52, 106.77, 87.78, 5.94] Cathode electrolyte interface Cathode electrolyte interface Cathode electrolyte interface Cathode electrolyte interface 2 5 3 24 #/texts/26 section_header body_heading False low body_heading body_heading True p2:body_region:0 body_zone column_1_of_2 1 2 p2:body_zone:column_1_of_2:white [255, 255, 255] white False False [42.52, 155.29, 62.12, 7.97] 1. Introduction 1. Introduction 1. Introduction 1. Introduction 2 1 8 29 #/texts/22 page_header page_header False low docling_page_header docling_page_header True p2:body_region:1 top_margin column_2_of_2 2 2 p2:top_margin:column_2_of_2:white [255, 255, 255] white False False [218.72, 47.78, 167.65, 6.37] R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 2 2 9 30 #/texts/23 page_header page_header False low docling_page_header docling_page_header True p2:body_region:1 top_margin column_2_of_2 2 2 p2:top_margin:column_2_of_2:white [255, 255, 255] white False False [555.48, 48.2, 7.11, 5.94] 71 71 71 71 2 11 11 32 #/texts/32 text metadata False low outside_body_flow_metadata_line outside_body_flow_metadata_line True p2:body_region:1 front_matter column_2_of_2 2 2 p2:front_matter:column_2_of_2:white [255, 255, 255] white False False [425.93, 95.74, 136.69, 8.36] © 2015 Elsevier B.V. All rights reserved. © 2015 Elsevier B.V. All rights reserved. © 2015 Elsevier B.V. All rights reserved. © 2015 Elsevier B.V. All rights reserved. 2 15 15 36 #/texts/36 section_header body_heading False low body_heading body_heading True p2:body_region:1 body_zone column_2_of_2 2 2 p2:body_zone:column_2_of_2:white [255, 255, 255] white False False [311.53, 511.09, 65.35, 7.97] 2. Experimental 2. Experimental 2. Experimental 2. Experimental 2 16 16 37 #/texts/37 section_header body_heading False low body_heading body_heading True p2:body_region:1 body_zone column_2_of_2 2 2 p2:body_zone:column_2_of_2:white [255, 255, 255] white False False [311.53, 532.44, 139.92, 7.42] 2.1. Preparation of electrolyte systems 2.1. Preparation of electrolyte systems 2.1. Preparation of electrolyte systems 2.1. Preparation of electrolyte systems 2 18 18 39 #/texts/39 caption caption False low outside_body_flow_caption outside_body_flow_caption True p2:body_region:1 bottom_margin column_2_of_2 2 2 p2:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [199.33, 737.02, 206.37, 6.38] Fig. 1. The reaction mechanism of eliminating H2O and HF by nitriles. Fig. 1. The reaction mechanism of eliminating H2O and HF by nitriles. Fig. 1. The reaction mechanism of eliminating H2O and HF by nitriles. Fig. 1. The reaction mechanism of eliminating H2O and HF by nitriles. 3 1 1 40 #/texts/40 page_header page_header False low docling_page_header docling_page_header True p3:body_region:0 top_margin column_1_of_2 1 2 p3:top_margin:column_1_of_2:white [255, 255, 255] white False False [32.82, 48.21, 7.16, 5.94] 72 72 72 72 3 3 2 41 #/texts/42 section_header body_heading False low body_heading body_heading True p3:body_region:0 body_zone column_1_of_2 1 2 p3:body_zone:column_1_of_2:white [255, 255, 255] white False False [32.83, 66.77, 229.41, 7.42] 2.2. Preparation of the electrodes and the construction of cells 2.2. Preparation of the electrodes and the construction of cells 2.2. Preparation of the electrodes and the construction of cells 2.2. Preparation of the electrodes and the construction of cells 3 5 4 43 #/texts/44 section_header body_heading False low body_heading body_heading True p3:body_region:0 body_zone column_1_of_2 1 2 p3:body_zone:column_1_of_2:white [255, 255, 255] white False False [32.83, 171.36, 129.89, 7.42] 2.3. Electrochemical measurements 2.3. Electrochemical measurements 2.3. Electrochemical measurements 2.3. Electrochemical measurements 3 10 9 48 #/texts/49 section_header body_heading False low body_heading body_heading True p3:body_region:0 body_zone column_1_of_2 1 2 p3:body_zone:column_1_of_2:white [255, 255, 255] white False False [32.83, 453.81, 116.72, 7.42] 2.4. Materials characterizations 2.4. Materials characterizations 2.4. Materials characterizations 2.4. Materials characterizations 3 13 12 51 #/texts/52 section_header body_heading False low body_heading body_heading True p3:body_region:0 body_zone column_1_of_2 1 2 p3:body_zone:column_1_of_2:white [255, 255, 255] white False False [32.83, 568.41, 105.41, 7.97] 3. Results and discussions 3. Results and discussions 3. Results and discussions 3. Results and discussions 3 2 15 54 #/texts/41 page_header page_header False low docling_page_header docling_page_header False None top_margin column_2_of_2 2 2 p3:top_margin:column_2_of_2:white [255, 255, 255] white False False [209.03, 47.78, 167.65, 6.37] R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 4 1 1 60 #/texts/59 page_header page_header False low docling_page_header docling_page_header False None top_margin right_crossing None None p4:top_margin:right_crossing:white [255, 255, 255] white False False [218.72, 47.78, 167.65, 6.37] R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 4 2 2 61 #/texts/60 page_header page_header False low docling_page_header docling_page_header False None top_margin right None None p4:top_margin:right:white [255, 255, 255] white False False [555.42, 48.2, 7.16, 5.94] 73 73 73 73 4 3 3 62 #/texts/61 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body full None None p4:page_body:full:white [255, 255, 255] white False False [42.52, 485.86, 520.07, 32.94] Fig. 2. (a) The conductivity of commercial electrolytes containing different weight ratios of succinonitrile at temperatures range from 30  C to 80  C. (b) LSV of the 1 M LiPF6/EC/ DEC commercial electrolyte with or… Fig. 2. (a) The conductivity of commercial electrolytes containing different weight ratios of succinonitrile at temperatures range from 30  C to 80  C. (b) LSV of the 1 M LiPF6/EC/ DEC commercial electrolyte with or… Fig. 2. (a) The conductivity of commercial electrolytes containing different weight ratios of succinonitrile at temperatures range from 30  C to 80  C. (b) LSV of the 1 M LiPF6/EC/ DEC commercial electrolyte with or without 1wt% SN. Working electrode: Pt, counter and reference electrodes: Li, scan rate: 1 mV s 1 . (c) Frontier molecular orbitals of EC, DEC and SN and their energies of occupied (HOMO) and unoccupied (LUMO) (in Ha). (d) Discharge capacity after 50 cycles of Li/Li1.2Ni0.2Mn0.6O2 half-cells containing various weight ratios of SN. Fig. 2. (a) The conductivity of commercial electrolytes containing different weight ratios of succinonitrile at temperatures range from 30  C to 80  C. (b) LSV of the 1 M LiPF6/EC/ DEC commercial electrolyte with or without 1wt% SN. Working electrode: Pt, counter and reference electrodes: Li, scan rate: 1 mV s 1 . (c) Frontier molecular orbitals of EC, DEC and SN and their energies of occupied (HOMO) and unoccupied (LUMO) (in Ha). (d) Discharge capacity after 50 cycles of Li/Li1.2Ni0.2Mn0.6O2 half-cells containing various weight ratios of SN. 4 4 4 63 #/texts/62 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body right_crossing None None p4:page_body:right_crossing:white [255, 255, 255] white False False [95.02, 716.67, 415.04, 6.98] Fig. 3. Ac impedance spectra of the Li/Li1.2Ni0.2Mn0.6O2 half-cells containing various weight ratios of SN: (a) After 1 cycles, (b) After 5 cycles. Fig. 3. Ac impedance spectra of the Li/Li1.2Ni0.2Mn0.6O2 half-cells containing various weight ratios of SN: (a) After 1 cycles, (b) After 5 cycles. Fig. 3. Ac impedance spectra of the Li/Li1.2Ni0.2Mn0.6O2 half-cells containing various weight ratios of SN: (a) After 1 cycles, (b) After 5 cycles. Fig. 3. Ac impedance spectra of the Li/Li1.2Ni0.2Mn0.6O2 half-cells containing various weight ratios of SN: (a) After 1 cycles, (b) After 5 cycles. 5 2 1 64 #/texts/63 page_header page_header False low docling_page_header docling_page_header True p5:body_region:0 top_margin column_1_of_2 1 2 p5:top_margin:column_1_of_2:white [255, 255, 255] white False True [32.82, 48.2, 6.82, 5.94] 74 74 74 74 5 4 2 65 #/texts/65 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body column_1_of_2 1 2 p5:page_body:column_1_of_2:white [255, 255, 255] white False False [150.29, 225.77, 285.11, 6.38] Fig. 4. TGA diagrams and DTG curves of commercial electrolyte (a) and 1wt % SN electrolyte (b). Fig. 4. TGA diagrams and DTG curves of commercial electrolyte (a) and 1wt % SN electrolyte (b). Fig. 4. TGA diagrams and DTG curves of commercial electrolyte (a) and 1wt % SN electrolyte (b). Fig. 4. TGA diagrams and DTG curves of commercial electrolyte (a) and 1wt % SN electrolyte (b). 5 7 5 68 #/texts/67 caption caption False low outside_body_flow_caption outside_body_flow_caption True p5:body_region:0 bottom_margin column_1_of_2 1 2 p5:bottom_margin:column_1_of_2:white [255, 255, 255] white False False [32.82, 719.9, 251.05, 23.4] Fig. 5. Discharge capacities and coulombic ef fi ciencies of the Li/Li1.2Ni0.2Mn0.6O2 half-cells at a 0.1 C current density with or without 1wt % SN at 55  C, the inset displays SEM images of the batteries after 50 cyc… Fig. 5. Discharge capacities and coulombic ef fi ciencies of the Li/Li1.2Ni0.2Mn0.6O2 half-cells at a 0.1 C current density with or without 1wt % SN at 55  C, the inset displays SEM images of the batteries after 50 cyc… Fig. 5. Discharge capacities and coulombic ef fi ciencies of the Li/Li1.2Ni0.2Mn0.6O2 half-cells at a 0.1 C current density with or without 1wt % SN at 55  C, the inset displays SEM images of the batteries after 50 cycles. Fig. 5. Discharge capacities and coulombic ef fi ciencies of the Li/Li1.2Ni0.2Mn0.6O2 half-cells at a 0.1 C current density with or without 1wt % SN at 55  C, the inset displays SEM images of the batteries after 50 cycles. 5 3 6 69 #/texts/64 page_header page_header False low docling_page_header docling_page_header False None top_margin column_2_of_2 2 2 p5:top_margin:column_2_of_2:white [255, 255, 255] white False False [209.03, 47.78, 167.65, 6.37] R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 6 1 1 73 #/texts/70 page_header page_header False low docling_page_header docling_page_header False None top_margin column_2_of_2 2 2 p6:top_margin:column_2_of_2:white [255, 255, 255] white False False [218.72, 47.78, 167.65, 6.37] R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 6 2 2 74 #/texts/71 page_header page_header False low docling_page_header docling_page_header True p6:body_region:1 top_margin column_2_of_2 2 2 p6:top_margin:column_2_of_2:white [255, 255, 255] white False False [555.25, 48.21, 7.29, 5.94] 75 75 75 75 6 3 3 75 #/texts/72 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body column_1_of_2 1 2 p6:page_body:column_1_of_2:white [255, 255, 255] white False False [49.04, 356.3, 506.98, 7.01] Fig. 6. Discharge capacities of Li/Li1.2Ni0.2Mn0.6O2 with 1wt% SN-based electrolyte at different cut-off voltages: (a) 2.0 e 4.8 V, (b) 2.0 e 4.9 V, (c) 2.0 e 5.0 V and (d) 2.0 e 5.2 V. Fig. 6. Discharge capacities of Li/Li1.2Ni0.2Mn0.6O2 with 1wt% SN-based electrolyte at different cut-off voltages: (a) 2.0 e 4.8 V, (b) 2.0 e 4.9 V, (c) 2.0 e 5.0 V and (d) 2.0 e 5.2 V. Fig. 6. Discharge capacities of Li/Li1.2Ni0.2Mn0.6O2 with 1wt% SN-based electrolyte at different cut-off voltages: (a) 2.0 e 4.8 V, (b) 2.0 e 4.9 V, (c) 2.0 e 5.0 V and (d) 2.0 e 5.2 V. Fig. 6. Discharge capacities of Li/Li1.2Ni0.2Mn0.6O2 with 1wt% SN-based electrolyte at different cut-off voltages: (a) 2.0 e 4.8 V, (b) 2.0 e 4.9 V, (c) 2.0 e 5.0 V and (d) 2.0 e 5.2 V. 6 4 4 76 #/texts/73 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body column_1_of_2 1 2 p6:page_body:column_1_of_2:white [255, 255, 255] white False False [137.93, 565.02, 329.18, 6.38] Fig. 7. SEM images of the surface of LNMO cathode after 5 cycles with: (a) commercial electrolyte (b) 1wt% SN. Fig. 7. SEM images of the surface of LNMO cathode after 5 cycles with: (a) commercial electrolyte (b) 1wt% SN. Fig. 7. SEM images of the surface of LNMO cathode after 5 cycles with: (a) commercial electrolyte (b) 1wt% SN. Fig. 7. SEM images of the surface of LNMO cathode after 5 cycles with: (a) commercial electrolyte (b) 1wt% SN. 7 2 1 79 #/texts/75 page_header page_header False low docling_page_header docling_page_header True p7:body_region:0 top_margin left None None p7:top_margin:left:white [255, 255, 255] white False False [32.82, 48.21, 7.05, 5.94] 76 76 76 76 7 3 2 80 #/texts/76 page_header page_header False low docling_page_header docling_page_header False None top_margin left_crossing None None p7:top_margin:left_crossing:white [255, 255, 255] white False False [209.03, 47.78, 167.65, 6.37] R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 R. Chen et al. / Journal of Power Sources 306 (2016) 70 e 77 7 4 3 81 #/texts/77 caption caption False low outside_body_flow_caption outside_body_flow_caption False None front_matter full None None p7:front_matter:full:white [255, 255, 255] white False False [32.82, 372.37, 520.08, 14.84] Fig. 8. XPS spectra of the regions of Li1.2Ni0.2Mn0.6O2 after 50 cycles: (a) N1s with commercial electrolyte, (b) N1s with 1wt% SN-based electrolyte, (c) Mn2p with commercial electrolyte, (d) Mn2p with 1wt% SN-based ele… Fig. 8. XPS spectra of the regions of Li1.2Ni0.2Mn0.6O2 after 50 cycles: (a) N1s with commercial electrolyte, (b) N1s with 1wt% SN-based electrolyte, (c) Mn2p with commercial electrolyte, (d) Mn2p with 1wt% SN-based ele… Fig. 8. XPS spectra of the regions of Li1.2Ni0.2Mn0.6O2 after 50 cycles: (a) N1s with commercial electrolyte, (b) N1s with 1wt% SN-based electrolyte, (c) Mn2p with commercial electrolyte, (d) Mn2p with 1wt% SN-based electrolyte, (e) Ni2p with commercial electrolyte, (f) Ni2p with 1wt% SN-based electrolyte. Fig. 8. XPS spectra of the regions of Li1.2Ni0.2Mn0.6O2 after 50 cycles: (a) N1s with commercial electrolyte, (b) N1s with 1wt% SN-based electrolyte, (c) Mn2p with commercial electrolyte, (d) Mn2p with 1wt% SN-based electrolyte, (e) Ni2p with commercial electrolyte, (f) Ni2p with 1wt% SN-based electrolyte. 7 5 5 83 #/texts/78 section_header body_heading False low body_heading body_heading True p7:body_region:0 body_zone left None None p7:body_zone:left:white [255, 255, 255] white False False [32.83, 441.25, 55.77, 7.97] 4. Conclusion 4. Conclusion 4. Conclusion 4. Conclusion 7 24 8 86 #/texts/96 list_item reference False low outside_body_flow_reference outside_body_flow_reference False None body_zone right_crossing None None p7:body_zone:right_crossing:white [255, 255, 255] white False False [301.83, 657.71, 251.01, 13.88] L. Chen, Y. Su, S. Chen, N. Li, L. Bao, W. Li, Z. Wang, M. Wang, F. Wu, Adv. Mater. 26 (2014) 6756 e 6760. L. Chen, Y. Su, S. Chen, N. Li, L. Bao, W. Li, Z. Wang, M. Wang, F. Wu, Adv. Mater. 26 (2014) 6756 e 6760. L. Chen, Y. Su, S. Chen, N. Li, L. Bao, W. Li, Z. Wang, M. Wang, F. Wu, Adv. Mater. 26 (2014) 6756 e 6760. L. Chen, Y. Su, S. Chen, N. Li, L. Bao, W. Li, Z. Wang, M. Wang, F. Wu, Adv. Mater. 26 (2014) 6756 e 6760. 7 25 9 87 #/texts/97 list_item reference False low outside_body_flow_reference outside_body_flow_reference False None body_zone right_crossing None None p7:body_zone:right_crossing:white [255, 255, 255] white False False [301.83, 673.64, 251.04, 21.87] M. Gu, I. Belharouak, J. Zheng, H. Wu, J. Xiao, A. 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