page source_page_order layout_page_order layout_order ref label role_guess included_in_body excluded_risk_level body_decision_reason parser_body_decision_reason production_usage visual_asset_type visual_asset_label visual_asset_caption_preview truncation_marker inside_body_region body_region_id zone column column_index column_count region_id background_rgb background_class is_gray_background has_frame_evidence bbox text_preview cleaned_text_preview text cleaned_text 1 1 1 0 #/texts/0 page_header page_header False low docling_page_header docling_page_header True p1:body_region:0 top_margin column_1_of_2 1 2 p1:top_margin:column_1_of_2:white [255, 255, 255] white False False [224.33, 47.98, 146.57, 5.93] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 1 19 2 1 #/texts/18 text front_matter_heading False low first_page_metadata first_page_metadata True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:gray [229, 229, 229] gray True False [220.76, 79.88, 151.02, 1.59] Contents lists available at ScienceDirect Contents lists available at ScienceDirect Contents lists available at ScienceDirect Contents lists available at ScienceDirect 1 20 3 2 #/texts/19 section_header title_candidate False low non_body_heading non_body_heading True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:gray [229, 229, 229] gray True False [201.2, 98.03, 190.03, 12.98] Journal of Energy Chemistry Journal of Energy Chemistry Journal of Energy Chemistry Journal of Energy Chemistry 1 21 4 3 #/texts/20 text unknown_text False medium outside_body_flow outside_body_flow True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:gray [229, 229, 229] gray True True [173.88, 135.67, 247.4, 1.59] j o u r n a l homepage: www.elsevier.com/locate/jechem j o u r n a l homepage: j o u r n a l homepage: www.elsevier.com/locate/jechem j o u r n a l homepage: 1 2 5 4 #/texts/1 section_header title_candidate False low non_body_heading non_body_heading False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.7, 160.04, 32.05, 8.9] Review Review Review Review 1 3 6 5 #/texts/2 section_header title_candidate False low non_body_heading non_body_heading True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 179.19, 423.72, 29.75] Recent progress in Li and Mn rich layered oxide cathodes for Li-ion batteries Recent progress in Li and Mn rich layered oxide cathodes for Li-ion batteries Recent progress in Li and Mn rich layered oxide cathodes for Li-ion batteries Recent progress in Li and Mn rich layered oxide cathodes for Li-ion batteries 1 4 7 6 #/texts/3 text body_candidate_excluded False medium before_body_started before_body_started True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 218.99, 494.97, 26.45] Yiwei Li a,1 , Zhibo Li a,1 , Cong Chen a , Kai Yang a , Bo Cao a , Shenyang Xu a , Ni Yang a , Wenguang Zhao a , Haibiao Chen a , Mingjian Zhang a,b, ⇑ , Feng Pan a, ⇑ Yiwei Li a,1 , Zhibo Li a,1 , Cong Chen a , Kai Yang a , Bo Cao a , Shenyang Xu a , Ni Yang a , Wenguang Zhao a , Haibiao Chen a , Mingjian Zhang a,b, ⇑ , Feng Pan a, ⇑ Yiwei Li a,1 , Zhibo Li a,1 , Cong Chen a , Kai Yang a , Bo Cao a , Shenyang Xu a , Ni Yang a , Wenguang Zhao a , Haibiao Chen a , Mingjian Zhang a,b, ⇑ , Feng Pan a, ⇑ Yiwei Li a,1 , Zhibo Li a,1 , Cong Chen a , Kai Yang a , Bo Cao a , Shenyang Xu a , Ni Yang a , Wenguang Zhao a , Haibiao Chen a , Mingjian Zhang a,b, ⇑ , Feng Pan a, ⇑ 1 5 8 7 #/texts/4 list_item affiliation False low outside_body_flow_list_item outside_body_flow_list_item False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.64, 250.92, 334.71, 7.3] a School of Advanced Materials, Peking University, Shenzhen Graduate School, Shenzhen 518055, Guangdong, China a School of Advanced Materials, Peking University, Shenzhen Graduate School, Shenzhen 518055, Guangdong, China a School of Advanced Materials, Peking University, Shenzhen Graduate School, Shenzhen 518055, Guangdong, China a School of Advanced Materials, Peking University, Shenzhen Graduate School, Shenzhen 518055, Guangdong, China 1 6 9 8 #/texts/5 list_item unknown_text False medium outside_body_flow_list_item outside_body_flow_list_item False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [254, 254, 254] white False True [37.64, 259.48, 2.79, 3.96] b b b b 1 7 10 9 #/texts/6 text affiliation False low front_matter_author_line front_matter_author_line False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [41.5, 260.41, 334.48, 6.37] Center for Advanced Radiation Source (ChemMatCARS), the University of Chicago, Argonne, IL 60439, United States Center for Advanced Radiation Source (ChemMatCARS), the University of Chicago, Argonne, IL 60439, United States Center for Advanced Radiation Source (ChemMatCARS), the University of Chicago, Argonne, IL 60439, United States Center for Advanced Radiation Source (ChemMatCARS), the University of Chicago, Argonne, IL 60439, United States 1 8 11 10 #/texts/7 section_header front_matter_heading False low front_matter_heading front_matter_heading False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.7, 287.39, 94.35, 11.02] a r t i c l e i n f o a r t i c l e i n f o a r t i c l e i n f o a r t i c l e i n f o 1 12 12 11 #/texts/11 section_header abstract_heading False low abstract_heading abstract_heading True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [202.22, 287.67, 65.22, 11.02] a b s t r a c t a b s t r a c t a b s t r a c t a b s t r a c t 1 9 13 12 #/texts/8 text unknown_text False high outside_body_flow outside_body_flow False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 310.07, 79.89, 32.02] Article history: Received 14 October 2020 Revised 23 January 2021 Accepted 25 January 2021 Article history: Received 14 October 2020 Revised 23 January 2021 Accepted 25 January 2021 Article history: Received 14 October 2020 Revised 23 January 2021 Accepted 25 January 2021 Article history: Received 14 October 2020 Revised 23 January 2021 Accepted 25 January 2021 1 13 14 13 #/texts/12 text abstract_candidate False medium inside_abstract inside_abstract True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [202.17, 310.46, 355.49, 93.18] Li and Mn rich (LMR) layered oxides, written as x Li2MnO3  (1 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure an… Li and Mn rich (LMR) layered oxides, written as x Li2MnO3  (1 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure an… Li and Mn rich (LMR) layered oxides, written as x Li2MnO3  (1 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure and superior performance of LMR oxides make them one of the most promising candidates for the next-generation cathode materials. However, the commercialization of these materials is hindered by several drawbacks, such as low initial Coulombic efficiency, the degradation of voltage and capacity during cycling, and poor rate performance. This review summarizes research progress in solving these concerns of LMR cathodes over the past decade by following three classes of strategies: morphology design, bulk design, and surface modification. We elaborate on the processing procedures, electrochemical performance, mechanisms, and limitations of each approach, and finally put forward the concerns left and the possible solutions for the commercialization of LMR cathodes. Li and Mn rich (LMR) layered oxides, written as x Li2MnO3  (1 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure and superior performance of LMR oxides make them one of the most promising candidates for the next-generation cathode materials. However, the commercialization of these materials is hindered by several drawbacks, such as low initial Coulombic efficiency, the degradation of voltage and capacity during cycling, and poor rate performance. This review summarizes research progress in solving these concerns of LMR cathodes over the past decade by following three classes of strategies: morphology design, bulk design, and surface modification. We elaborate on the processing procedures, electrochemical performance, mechanisms, and limitations of each approach, and finally put forward the concerns left and the possible solutions for the commercialization of LMR cathodes. 1 10 15 14 #/texts/9 text metadata False low first_page_metadata first_page_metadata False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 344.71, 104.89, 5.93] Available online 10 February 2021 Available online 10 February 2021 Available online 10 February 2021 Available online 10 February 2021 1 11 16 15 #/texts/10 text front_matter_heading False low front_matter_heading front_matter_heading False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 364.44, 116.82, 40.52] Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective 1 14 17 16 #/texts/13 text metadata False low first_page_metadata first_page_metadata True p1:body_region:0 page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [202.17, 404.52, 355.42, 18.23] Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved. Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved. Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. 1 15 18 17 #/texts/14 text reference False low inside_front_matter inside_front_matter False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [120.08, 460.31, 168.57, 57.35] Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking Uni… Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking Uni… Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking University. His main research work is Li-Rich cathode materials with high voltage and high energy density for Li ion batteries. Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking University. His main research work is Li-Rich cathode materials with high voltage and high energy density for Li ion batteries. 1 16 19 18 #/texts/15 footnote footnote False low first_page_metadata first_page_metadata False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [42.07, 692.51, 264.1, 18.63] ⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan). ⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan). ⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan). ⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan). 1 17 20 19 #/texts/16 footnote footnote False low outside_body_flow_footnote outside_body_flow_footnote False None page_body column_1_of_2 1 2 p1:page_body:column_1_of_2:white [255, 255, 255] white False False [43.09, 712.68, 148.31, 7.21] 1 These authors contributed equally to this work. 1 These authors contributed equally to this work. 1 These authors contributed equally to this work. 1 These authors contributed equally to this work. 1 22 21 20 #/texts/21 page_footer page_footer False low first_page_metadata first_page_metadata False None bottom_margin column_1_of_2 1 2 p1:bottom_margin:column_1_of_2:white [255, 255, 255] white False True [37.59, 731.92, 136.91, 5.93] https://doi.org/10.1016/j.jechem.2021.01.034 https://doi.org/10.1016/j.jechem.2021.01.034 1 18 22 21 #/texts/17 text body_candidate_excluded False high inside_front_matter inside_front_matter True p1:body_region:0 page_body column_2_of_2 2 2 p1:page_body:column_2_of_2:white [255, 255, 255] white False False [389.08, 458.95, 168.57, 48.74] Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research intere… Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research intere… Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion batteries. Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion batteries. 1 23 23 22 #/texts/22 page_footer page_footer False low first_page_metadata first_page_metadata True p1:body_region:0 bottom_margin column_1_of_2 1 2 p1:bottom_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 738.73, 520.05, 8.3] 2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved. 2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. 2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved. 2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. 2 1 1 23 #/texts/23 text page_margin_header False low page_margin_header page_margin_header False None top_margin column_1_of_2 1 2 p2:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 2 2 2 24 #/texts/24 text body_candidate_excluded False high inside_front_matter inside_front_matter True p2:body_region:0 page_body column_1_of_2 1 2 p2:page_body:column_1_of_2:white [255, 255, 255] white False False [120.08, 66.24, 168.58, 48.79] Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His researc… Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His researc… Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion and sodium ion batteries. Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion and sodium ion batteries. 2 3 3 25 #/texts/25 text reference False low inside_front_matter inside_front_matter True p2:body_region:0 page_body column_1_of_2 1 2 p2:page_body:column_1_of_2:white [255, 255, 255] white False False [120.08, 195.27, 168.59, 65.91] Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. Hi… Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. Hi… Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. His main research interests include advanced silicon carbon materials for lithium ion batteries (LIBs) and advanced technology for interface research in LIBs, such as in-situ AFM and EQCM. Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. His main research interests include advanced silicon carbon materials for lithium ion batteries (LIBs) and advanced technology for interface research in LIBs, such as in-situ AFM and EQCM. 2 4 4 26 #/texts/26 text reference False low inside_front_matter inside_front_matter True p2:body_region:0 page_body column_1_of_2 1 2 p2:page_body:column_1_of_2:white [255, 255, 255] white False False [120.08, 324.36, 168.59, 65.91] Bo Cao is currently a Ph.D. candidate in Prof Feng Pan's group at Peking University Shenzhen Graduate School, China. He received his B.S. degree in material science from Huazhong University of Science and Technology in … Bo Cao is currently a Ph.D. candidate in Prof Feng Pan's group at Peking University Shenzhen Graduate School, China. He received his B.S. degree in material science from Huazhong University of Science and Technology in … Bo Cao is currently a Ph.D. candidate in Prof Feng Pan's group at Peking University Shenzhen Graduate School, China. He received his B.S. degree in material science from Huazhong University of Science and Technology in 2018. Currently his research interests focus on high energy density cathode materials for lithium batteries, especially on Li-rich and Ni-rich layered oxide materials. Bo Cao is currently a Ph.D. candidate in Prof Feng Pan's group at Peking University Shenzhen Graduate School, China. He received his B.S. degree in material science from Huazhong University of Science and Technology in 2018. Currently his research interests focus on high energy density cathode materials for lithium batteries, especially on Li-rich and Ni-rich layered oxide materials. 2 5 5 27 #/texts/27 text reference False low inside_front_matter inside_front_matter True p2:body_region:0 page_body column_1_of_2 1 2 p2:page_body:column_1_of_2:white [255, 255, 255] white False False [120.08, 453.39, 168.58, 48.79] Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests ma… Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests ma… Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on development of functional materials for energy storage. Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on development of functional materials for energy storage. 2 6 6 28 #/texts/28 text body_candidate_excluded False high inside_front_matter inside_front_matter True p2:body_region:0 page_body column_1_of_2 1 2 p2:page_body:column_1_of_2:white [255, 255, 255] white False False [120.08, 582.43, 168.59, 48.79] Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FI… Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FI… Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FIB, SEM and TEM. Her research interests mainly focus on the FIB and TEM characterization of battery materials. Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FIB, SEM and TEM. Her research interests mainly focus on the FIB and TEM characterization of battery materials. 2 7 7 29 #/texts/29 text page_margin_header False low page_margin_header page_margin_header True p2:body_region:1 top_margin column_2_of_2 2 2 p2:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.77, 47.8, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 2 8 8 30 #/texts/30 text body_candidate_excluded False high inside_front_matter inside_front_matter True p2:body_region:1 page_body column_2_of_2 2 2 p2:page_body:column_2_of_2:white [255, 255, 255] white False False [389.08, 66.24, 168.57, 57.35] Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools includi… Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools includi… Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools including XRD, XPS, SEM and TEM. His research interests mainly focus on the ex/in-situ TEM and ex/in-situ XRD characterization of battery materials. Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools including XRD, XPS, SEM and TEM. His research interests mainly focus on the ex/in-situ TEM and ex/in-situ XRD characterization of battery materials. 2 9 9 31 #/texts/31 text body_candidate_excluded False high inside_front_matter inside_front_matter True p2:body_region:1 page_body column_2_of_2 2 2 p2:page_body:column_2_of_2:white [255, 255, 255] white False False [389.08, 195.27, 168.57, 48.79] Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institut… Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institut… Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institute of Technology in 2006. He worked at Velocys during 2006-2011 and UES during 2011-2014. Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institute of Technology in 2006. He worked at Velocys during 2006-2011 and UES during 2011-2014. 2 10 10 32 #/texts/32 text reference False low inside_front_matter inside_front_matter True p2:body_region:1 page_body column_2_of_2 2 2 p2:page_body:column_2_of_2:white [255, 255, 255] white False False [389.08, 324.36, 168.58, 100.16] Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, h… Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, h… Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, he was a postdoc at School of Advanced Materials, Peking University, and became an assistant research professor since 2018. Meanwhile, he was a research scholar in Brookhaven National Lab from 2016 to 2019, then in the University of Chicago since 2019. He has been engaged in the fields of electrode materials for Liion batteries, crystal growth and structure analysis of nonlinear optical crystals. Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, he was a postdoc at School of Advanced Materials, Peking University, and became an assistant research professor since 2018. Meanwhile, he was a research scholar in Brookhaven National Lab from 2016 to 2019, then in the University of Chicago since 2019. He has been engaged in the fields of electrode materials for Liion batteries, crystal growth and structure analysis of nonlinear optical crystals. 2 11 11 33 #/texts/33 text reference False low inside_front_matter inside_front_matter True p2:body_region:1 page_body column_2_of_2 2 2 p2:page_body:column_2_of_2:white [255, 255, 255] white False False [389.08, 453.39, 168.57, 100.16] Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathc… Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathc… Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathclyde, Glasgow, UK, with ''Patrick D. Ritchie Prize' for the best Ph.D. in 1994. With more than a decade experience in large international incorporations, Prof. Pan has been engaged in fundamental research and product development of novel optoelectronic and energy storage materials and devices. As Chief Scientist, Prof. Pan led eight entities in Shenzhen to win 150 million RMB grant for the national new energy vehicles Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathclyde, Glasgow, UK, with ''Patrick D. Ritchie Prize' for the best Ph.D. in 1994. With more than a decade experience in large international incorporations, Prof. Pan has been engaged in fundamental research and product development of novel optoelectronic and energy storage materials and devices. As Chief Scientist, Prof. Pan led eight entities in Shenzhen to win 150 million RMB grant for the national new energy vehicles 2 12 12 34 #/texts/34 text unknown_text False medium inside_front_matter inside_front_matter False None page_body column_2_of_2 2 2 p2:page_body:column_2_of_2:white [255, 255, 255] white False False [306.6, 556.17, 142.45, 5.93] (power battery) innovation project since 2013. (power battery) innovation project since 2013. (power battery) innovation project since 2013. (power battery) innovation project since 2013. 2 13 13 35 #/texts/35 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p2:bottom_margin:column_2_of_2:white [254, 254, 254] white False False [291.91, 764.24, 11.45, 5.93] 369 369 369 369 3 1 1 36 #/texts/36 page_header page_header False low docling_page_header docling_page_header True p3:body_region:0 top_margin column_1_of_2 1 2 p3:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 3 3 2 37 #/texts/38 section_header body_heading False low body_heading body_heading True p3:body_region:0 body_zone column_1_of_2 1 2 p3:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.7, 68.75, 60.13, 7.42] 1. Introduction 1. Introduction 1. Introduction 1. Introduction 3 2 4 39 #/texts/37 page_header page_header False low docling_page_header docling_page_header False None top_margin column_2_of_2 2 2 p3:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.71, 47.86, 139.91, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 3 6 6 41 #/texts/41 caption caption False low outside_body_flow_caption outside_body_flow_caption False None body_zone column_1_of_2 1 2 p3:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.59, 559.63, 520.04, 32.02] Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d … Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d … Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d synthesized from two different precursors (C for conventional precursor and H for hierarchically structured precursor). Reproduced from Ref. [27] with permission from American Chemical Society. (d) Structural scheme showing the honeycomb pattern consisting of Li@Mn6 superstructure units in LMR layered oxide. Reproduced from Ref. [29]) with permission from Royal Society of Chemistry. Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d synthesized from two different precursors (C for conventional precursor and H for hierarchically structured precursor). Reproduced from Ref. [27] with permission from American Chemical Society. (d) Structural scheme showing the honeycomb pattern consisting of Li@Mn6 superstructure units in LMR layered oxide. Reproduced from Ref. [29]) with permission from Royal Society of Chemistry. 3 7 7 42 #/texts/42 caption caption False low outside_body_flow_caption outside_body_flow_caption True p3:body_region:0 body_zone column_1_of_2 1 2 p3:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.59, 613.15, 182.82, 14.49] Table 1 Researches about understanding the structure of LMR oxides. Table 1 Researches about understanding the structure of LMR oxides. Table 1 Researches about understanding the structure of LMR oxides. Table 1 Researches about understanding the structure of LMR oxides. 3 8 8 43 #/texts/43 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p3:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.38, 5.93] 370 370 370 370 4 2 1 44 #/texts/44 page_header page_header False low docling_page_header docling_page_header False None top_margin column_1_of_2 1 2 p4:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 4 3 2 45 #/texts/45 page_header page_header False low docling_page_header docling_page_header True p4:body_region:0 top_margin column_2_of_2 2 2 p4:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.77, 47.81, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 4 4 3 46 #/texts/46 caption caption False low outside_body_flow_caption outside_body_flow_caption False None front_matter column_1_of_2 1 2 p4:front_matter:column_1_of_2:white [255, 255, 255] white False False [37.59, 345.73, 520.08, 65.91] Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chem… Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chem… Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chemical Society. (c) p DOS of O 2 p orbitals and Mn 3 d orbitals in Li2MnO3 and the corresponding oxygen environment model. Reproduced from Ref. [47] with permission from Springer Nature. (d) Cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 synthesized by two different synthesis methods at 0.1 C in the voltage range of 2.0-4.8 V. (e) The corresponding capacity-voltage profiles of the re-synthesized Li1.2Ni0.13Co0.13Mn0.54O2 in (d). Reproduced from Ref. [53] with permission from Elsevier. (f) Schematic representation for the structural transformation of trigonal LiMO2 component ( R -3m) and monoclinic Li2MnO3 component ( C 2/ m ) in Li1.2Ni0.1Mn0.525Co0.175O2 during cycling. Reproduced from Ref. [54] with permission from American Chemical Society. (g) Selected area electron diffraction (SAED) pattern obtained along [0001] zone axis of Li1.2Co0.1Mn0.55Ni0.15O2 cathode at the charging voltage of 4.5 V. (h) Schematic diagram of TM migration in Li1.2Co0.1Mn0.55Ni0.15O2 cathode when holding at 4.5 V. Reproduced from Ref. [55] with permission from Royal Society of Chemistry. Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chemical Society. (c) p DOS of O 2 p orbitals and Mn 3 d orbitals in Li2MnO3 and the corresponding oxygen environment model. Reproduced from Ref. [47] with permission from Springer Nature. (d) Cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 synthesized by two different synthesis methods at 0.1 C in the voltage range of 2.0-4.8 V. (e) The corresponding capacity-voltage profiles of the re-synthesized Li1.2Ni0.13Co0.13Mn0.54O2 in (d). Reproduced from Ref. [53] with permission from Elsevier. (f) Schematic representation for the structural transformation of trigonal LiMO2 component ( R -3m) and monoclinic Li2MnO3 component ( C 2/ m ) in Li1.2Ni0.1Mn0.525Co0.175O2 during cycling. Reproduced from Ref. [54] with permission from American Chemical Society. (g) Selected area electron diffraction (SAED) pattern obtained along [0001] zone axis of Li1.2Co0.1Mn0.55Ni0.15O2 cathode at the charging voltage of 4.5 V. (h) Schematic diagram of TM migration in Li1.2Co0.1Mn0.55Ni0.15O2 cathode when holding at 4.5 V. Reproduced from Ref. [55] with permission from Royal Society of Chemistry. 4 6 6 49 #/texts/48 section_header body_heading False low body_heading body_heading True p4:body_region:0 body_zone column_2_of_2 2 2 p4:body_zone:column_2_of_2:white [255, 255, 255] white False False [306.65, 445.24, 248.85, 7.42] 2. Structure and electrochemical performance of LMR cathode 2. Structure and electrochemical performance of LMR cathode 2. Structure and electrochemical performance of LMR cathode 2. Structure and electrochemical performance of LMR cathode 4 7 7 50 #/texts/49 section_header body_heading False low body_heading body_heading True p4:body_region:0 body_zone column_2_of_2 2 2 p4:body_zone:column_2_of_2:white [255, 255, 255] white False False [306.65, 465.73, 128.59, 7.96] 2.1. Crystal structure of LMR oxides 2.1. Crystal structure of LMR oxides 2.1. Crystal structure of LMR oxides 2.1. Crystal structure of LMR oxides 4 10 10 53 #/texts/52 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p4:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 371 371 371 371 5 2 1 54 #/texts/53 page_header page_header False low docling_page_header docling_page_header True p5:body_region:0 top_margin column_1_of_2 1 2 p5:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 5 7 6 59 #/texts/58 section_header body_heading False low body_heading body_heading True p5:body_region:0 body_zone column_1_of_2 1 2 p5:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.7, 402.24, 182.07, 7.96] 2.2. Electrochemical performance of LMR cathodes 2.2. Electrochemical performance of LMR cathodes 2.2. Electrochemical performance of LMR cathodes 2.2. Electrochemical performance of LMR cathodes 5 3 9 62 #/texts/54 page_header page_header False low docling_page_header docling_page_header True p5:body_region:1 top_margin column_2_of_2 2 2 p5:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.71, 47.86, 139.91, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 5 13 13 66 #/texts/64 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p5:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 372 372 372 372 6 1 1 67 #/texts/65 page_header page_header False low docling_page_header docling_page_header True p6:body_region:0 top_margin column_1_of_2 1 2 p6:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 6 3 2 68 #/texts/67 caption caption False low outside_body_flow_caption outside_body_flow_caption True p6:body_region:0 page_body column_1_of_2 1 2 p6:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 67.94, 328.37, 14.49] Table 2 The electrochemical performance of LMR cathodes with different morphology design reported in recent years. Table 2 The electrochemical performance of LMR cathodes with different morphology design reported in recent years. Table 2 The electrochemical performance of LMR cathodes with different morphology design reported in recent years. Table 2 The electrochemical performance of LMR cathodes with different morphology design reported in recent years. 6 4 3 69 #/texts/68 text unknown_text False medium outside_body_flow outside_body_flow True p6:body_region:0 page_body column_1_of_2 1 2 p6:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 203.66, 153.66, 5.93] Notes. [a] ICE denotes initial Coulombic efficiency. Notes. [a] ICE denotes initial Coulombic efficiency. Notes. [a] ICE denotes initial Coulombic efficiency. Notes. [a] ICE denotes initial Coulombic efficiency. 6 2 4 70 #/texts/66 page_header page_header False low docling_page_header docling_page_header True p6:body_region:1 top_margin column_2_of_2 2 2 p6:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.77, 47.8, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 6 5 5 71 #/texts/69 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body column_1_of_2 1 2 p6:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 567.06, 520.06, 40.18] Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3  (1… Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3  (1… Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3  (1x )LiMnO2 nanorods. Reproduced from Ref. [63] with permission from Elsevier. (c) Schematic illustration of the synthetic process of orthogonally arranged nanoplates. Reproduced from Ref. [64] with permission from American Chemical Society. (d) Scheme of the fabrication process of 3D hollow porous bowl-shaped Li1.2Ni0.13Co0.13Mn0.54O2 particles. Reproduced from Ref. [66] with permission from Elsevier. (e) Schematic diagram of the suppression of voltage fading through a preferred orientation (110) plane. Reproduced from Ref. [67] with permission from Royal Society of Chemistry. Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3  (1x )LiMnO2 nanorods. Reproduced from Ref. [63] with permission from Elsevier. (c) Schematic illustration of the synthetic process of orthogonally arranged nanoplates. Reproduced from Ref. [64] with permission from American Chemical Society. (d) Scheme of the fabrication process of 3D hollow porous bowl-shaped Li1.2Ni0.13Co0.13Mn0.54O2 particles. Reproduced from Ref. [66] with permission from Elsevier. (e) Schematic diagram of the suppression of voltage fading through a preferred orientation (110) plane. Reproduced from Ref. [67] with permission from Royal Society of Chemistry. 6 8 8 74 #/texts/71 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p6:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 373 373 373 373 7 1 1 75 #/texts/72 page_header page_header False low docling_page_header docling_page_header False None top_margin left None None p7:top_margin:left:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 7 2 2 76 #/texts/73 page_header page_header False low docling_page_header docling_page_header False None top_margin right None None p7:top_margin:right:white [255, 255, 255] white False False [417.71, 47.86, 139.91, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 7 3 3 77 #/texts/74 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body full None None p7:page_body:full:white [255, 255, 255] white False False [37.59, 336.66, 520.03, 23.72] Fig. 4. (a) Schematic illustration of the formation of porous Li1.2Ni0.18Co0.08Mn0.54O2. Reproduced from Ref. [68] with permission from Royal Society of Chemistry. (b) Schematic illustration of the synthesizing route fo… Fig. 4. (a) Schematic illustration of the formation of porous Li1.2Ni0.18Co0.08Mn0.54O2. Reproduced from Ref. [68] with permission from Royal Society of Chemistry. (b) Schematic illustration of the synthesizing route fo… Fig. 4. (a) Schematic illustration of the formation of porous Li1.2Ni0.18Co0.08Mn0.54O2. Reproduced from Ref. [68] with permission from Royal Society of Chemistry. (b) Schematic illustration of the synthesizing route for 3D Li1.2Ni0.2Mn0.6O2 and the morphological evolution. Reproduced from Ref. [69] with permission from American Chemical Society. (c) SEM image of Li1.2Ni0.2Mn0.6O2 oxide. Reproduced from Ref. [70] with permission from American Chemical Society. Fig. 4. (a) Schematic illustration of the formation of porous Li1.2Ni0.18Co0.08Mn0.54O2. Reproduced from Ref. [68] with permission from Royal Society of Chemistry. (b) Schematic illustration of the synthesizing route for 3D Li1.2Ni0.2Mn0.6O2 and the morphological evolution. Reproduced from Ref. [69] with permission from American Chemical Society. (c) SEM image of Li1.2Ni0.2Mn0.6O2 oxide. Reproduced from Ref. [70] with permission from American Chemical Society. 7 4 4 78 #/texts/75 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body full None None p7:page_body:full:white [255, 255, 255] white False False [37.59, 667.98, 520.07, 57.96] Fig. 5. (a) Schematic illustration of ice-template coprecipitation method to synthesize Li1.2Ni0.2Mn0.6O2 with hierarchical mesopore structure. (b) The rate performance of Li1.2Ni0.2Mn0.6O2 synthesized by freeze drying … Fig. 5. (a) Schematic illustration of ice-template coprecipitation method to synthesize Li1.2Ni0.2Mn0.6O2 with hierarchical mesopore structure. (b) The rate performance of Li1.2Ni0.2Mn0.6O2 synthesized by freeze drying … Fig. 5. (a) Schematic illustration of ice-template coprecipitation method to synthesize Li1.2Ni0.2Mn0.6O2 with hierarchical mesopore structure. (b) The rate performance of Li1.2Ni0.2Mn0.6O2 synthesized by freeze drying (M1) and vacuum drying (M2). Reproduced from Ref. [73] with permission from American Chemical Society. (c) Schematic diagram of building nano-porous structures in Li1.144Ni0.136Co0.136Mn0.544O2. Reproduced from Ref. [74] with permission from American Chemical Society. (d) Schematic diagram to show various structure defects in Li1.143Ni0.136Co0.136Mn0.544O2. (e) TEM image to show nano-defects (stacking faults and cationic mixing) in the Li1.143Ni0.136Co0.136Mn0.544O2. (f) Comparison for the average voltage of highly crystalline Li1.143Ni0.136Co0.136Mn0.544O2 cathode (Pristine-LrLO) and defect abundant sample (NDA-LrCO-5) during cycling at 0.1 C. Reproduced from Ref. [75] with permission from Elsevier. (g) Schematic diagram of the element gradient distribution in LMR cathodes. (h) SEM image of Li1.2Mn0.44Co0.04Ni0.32O2 with element gradient distribution and (i) EDS line scanning along the marked line in (h). Reproduced from Ref. [80] with permission from Elsevier. Fig. 5. (a) Schematic illustration of ice-template coprecipitation method to synthesize Li1.2Ni0.2Mn0.6O2 with hierarchical mesopore structure. (b) The rate performance of Li1.2Ni0.2Mn0.6O2 synthesized by freeze drying (M1) and vacuum drying (M2). Reproduced from Ref. [73] with permission from American Chemical Society. (c) Schematic diagram of building nano-porous structures in Li1.144Ni0.136Co0.136Mn0.544O2. Reproduced from Ref. [74] with permission from American Chemical Society. (d) Schematic diagram to show various structure defects in Li1.143Ni0.136Co0.136Mn0.544O2. (e) TEM image to show nano-defects (stacking faults and cationic mixing) in the Li1.143Ni0.136Co0.136Mn0.544O2. (f) Comparison for the average voltage of highly crystalline Li1.143Ni0.136Co0.136Mn0.544O2 cathode (Pristine-LrLO) and defect abundant sample (NDA-LrCO-5) during cycling at 0.1 C. Reproduced from Ref. [75] with permission from Elsevier. (g) Schematic diagram of the element gradient distribution in LMR cathodes. (h) SEM image of Li1.2Mn0.44Co0.04Ni0.32O2 with element gradient distribution and (i) EDS line scanning along the marked line in (h). Reproduced from Ref. [80] with permission from Elsevier. 7 5 5 79 #/texts/76 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin left_crossing None None p7:bottom_margin:left_crossing:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 374 374 374 374 8 2 1 80 #/texts/77 page_header page_header False low docling_page_header docling_page_header True p8:body_region:0 top_margin column_1_of_2 1 2 p8:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 8 5 4 83 #/texts/80 section_header body_heading False low body_heading body_heading True p8:body_region:0 body_zone column_1_of_2 1 2 p8:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.59, 272.79, 212.3, 17.91] 3. Recent progress on promoting the electrochemical performance of LMR cathodes 3. Recent progress on promoting the electrochemical performance of LMR cathodes 3. Recent progress on promoting the electrochemical performance of LMR cathodes 3. Recent progress on promoting the electrochemical performance of LMR cathodes 8 7 6 85 #/texts/82 section_header body_heading False low body_heading body_heading True p8:body_region:0 body_zone column_1_of_2 1 2 p8:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.7, 391.81, 84.2, 7.96] 3.1. Morphology design 3.1. Morphology design 3.1. Morphology design 3.1. Morphology design 8 3 9 88 #/texts/78 page_header page_header False low docling_page_header docling_page_header True p8:body_region:1 top_margin column_2_of_2 2 2 p8:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.77, 47.81, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 8 14 14 93 #/texts/88 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p8:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 375 375 375 375 9 2 1 94 #/texts/90 section_header body_heading False low body_heading body_heading True p9:body_region:0 top_margin column_1_of_2 1 2 p9:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 9 3 2 95 #/texts/91 caption caption False low outside_body_flow_caption outside_body_flow_caption True p9:body_region:0 front_matter column_1_of_2 1 2 p9:front_matter:column_1_of_2:white [255, 255, 255] white False False [37.59, 67.94, 322.38, 14.49] Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. 9 7 6 99 #/texts/95 section_header body_heading False low body_heading body_heading True p9:body_region:0 body_zone column_1_of_2 1 2 p9:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.7, 485.35, 56.76, 7.96] 3.2. Bulk design 3.2. Bulk design 3.2. Bulk design 3.2. Bulk design 9 9 8 101 #/texts/97 section_header body_heading False low body_heading body_heading True p9:body_region:0 body_zone column_1_of_2 1 2 p9:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.7, 548.68, 80.52, 7.96] 3.2.1. Structure design 3.2.1. Structure design 3.2.1. Structure design 3.2.1. Structure design 9 1 11 104 #/texts/89 page_header page_header False low docling_page_header docling_page_header True p9:body_region:1 top_margin column_2_of_2 2 2 p9:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.71, 47.86, 139.91, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 9 14 14 107 #/texts/101 page_footer page_footer False low docling_page_footer docling_page_footer True p9:body_region:0 bottom_margin column_2_of_2 2 2 p9:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 376 376 376 376 10 1 1 108 #/texts/102 page_header page_header False low docling_page_header docling_page_header False None top_margin column_1_of_2 1 2 p10:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 10 2 2 109 #/texts/103 page_header page_header False low docling_page_header docling_page_header False None top_margin column_2_of_2 2 2 p10:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.77, 47.8, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 10 3 3 110 #/texts/104 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body column_1_of_2 1 2 p10:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 405.2, 520.07, 57.35] Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100… Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100… Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100 mA g 1 . Reproduced from Ref. [84] with permission from Royal Society of Chemistry. (c) Schematic diagram of pristine LMR, LMR with surface-doped with Na (Na-LMR) and LMR with homogenously Na doping (Na/SDS-LMR) before cycling and after 200 cycles. Reproduced from Ref. [85] with permission from Wiley-VCH. (d) Schematic illustration for the structure of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . (e) The rate performance of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . Reproduced from Ref. [88] with permission from Royal Society of Chemistry. (f) Schematic diagram of Na and F co-doping in Li1.2Ni0.2Mn0.6O2 cathode. (g) The cycling performance of Li1.2Ni0.2Mn0.6O2 cathode (LNMO), Na doped LNMO cathode (Na-LNMO), F doped LNMO cathode (F-LNMO) and Na and F co-doped LNMO cathode (Na&FLNMO) at 0.1 C in the voltage range of 2.0-4.8 V. Reproduced from Ref. [95] with permission from Elsevier. Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100 mA g 1 . Reproduced from Ref. [84] with permission from Royal Society of Chemistry. (c) Schematic diagram of pristine LMR, LMR with surface-doped with Na (Na-LMR) and LMR with homogenously Na doping (Na/SDS-LMR) before cycling and after 200 cycles. Reproduced from Ref. [85] with permission from Wiley-VCH. (d) Schematic illustration for the structure of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . (e) The rate performance of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . Reproduced from Ref. [88] with permission from Royal Society of Chemistry. (f) Schematic diagram of Na and F co-doping in Li1.2Ni0.2Mn0.6O2 cathode. (g) The cycling performance of Li1.2Ni0.2Mn0.6O2 cathode (LNMO), Na doped LNMO cathode (Na-LNMO), F doped LNMO cathode (F-LNMO) and Na and F co-doped LNMO cathode (Na&FLNMO) at 0.1 C in the voltage range of 2.0-4.8 V. Reproduced from Ref. [95] with permission from Elsevier. 10 4 4 111 #/texts/105 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body column_1_of_2 1 2 p10:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 484.4, 318.95, 14.55] Table 5 The electrochemical performance of LMR cathodes with different surface coatings reported in recent years. Table 5 The electrochemical performance of LMR cathodes with different surface coatings reported in recent years. Table 5 The electrochemical performance of LMR cathodes with different surface coatings reported in recent years. Table 5 The electrochemical performance of LMR cathodes with different surface coatings reported in recent years. 10 7 7 114 #/texts/108 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p10:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 377 377 377 377 11 2 1 115 #/texts/109 page_header page_header False low docling_page_header docling_page_header True p11:body_region:0 top_margin column_1_of_2 1 2 p11:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 11 3 2 116 #/texts/110 page_header page_header False low docling_page_header docling_page_header False None top_margin column_2_of_2 2 2 p11:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.71, 47.86, 139.91, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 11 4 3 117 #/texts/111 caption caption False low outside_body_flow_caption outside_body_flow_caption False None page_body column_1_of_2 1 2 p11:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 454.36, 520.06, 40.18] Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from E… Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from E… Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from Elsevier. (c) Schematic illustration of different oxygen migration model in bare and SnO2 coated Li1.2Ni0.13Co0.13Mn0.54O2 (filled with oxygen vacancies at the surface). Reproduced from Ref. [103] with permission from Elsevier. (d) Schematic diagram for the surficial structure of AlPO4 coated LMR oxide. (e) The Coulombic efficiency of the LMR oxides coated with different ALD cycles of AlPO4 during long-term cycling. Reproduced from Ref. [104] with permission from Elsevier. Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from Elsevier. (c) Schematic illustration of different oxygen migration model in bare and SnO2 coated Li1.2Ni0.13Co0.13Mn0.54O2 (filled with oxygen vacancies at the surface). Reproduced from Ref. [103] with permission from Elsevier. (d) Schematic diagram for the surficial structure of AlPO4 coated LMR oxide. (e) The Coulombic efficiency of the LMR oxides coated with different ALD cycles of AlPO4 during long-term cycling. Reproduced from Ref. [104] with permission from Elsevier. 11 5 4 118 #/texts/112 caption caption False low outside_body_flow_caption outside_body_flow_caption True p11:body_region:0 page_body column_1_of_2 1 2 p11:page_body:column_1_of_2:white [255, 255, 255] white False False [37.59, 516.32, 403.6, 14.49] Table 6 The electrochemical performance of LMR cathodes with different surface doping and other surface treatments reported in recent years. Table 6 The electrochemical performance of LMR cathodes with different surface doping and other surface treatments reported in recent years. Table 6 The electrochemical performance of LMR cathodes with different surface doping and other surface treatments reported in recent years. Table 6 The electrochemical performance of LMR cathodes with different surface doping and other surface treatments reported in recent years. 11 8 8 122 #/texts/115 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p11:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 378 378 378 378 12 2 1 123 #/texts/116 page_header page_header False low docling_page_header docling_page_header True p12:body_region:0 top_margin column_1_of_2 1 2 p12:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 12 3 2 124 #/texts/117 page_header page_header False low docling_page_header docling_page_header True p12:body_region:1 top_margin column_2_of_2 2 2 p12:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.77, 47.81, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 12 4 3 125 #/texts/118 caption caption False low outside_body_flow_caption outside_body_flow_caption False None front_matter column_1_of_2 1 2 p12:front_matter:column_1_of_2:white [255, 255, 255] white False False [37.59, 408.83, 520.06, 49.4] Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. [107] with permission f… Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. [107] with permission f… Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. [107] with permission from Elsevier. (c) The cycling performance of the Li1.2Ni0.13Co0.13Mn0.54O2 cathode coated with different contents of Al2O3 and polyacene at 0.2 C (APL is short for double-shelled of Al2O3 and polyacene, and the number represents different amount of polyacene). Reproduced from Ref. [115] with permission from Royal Society of Chemistry. (d) Schematic diagram of the detailed synthetic process of the LMR cathode coated with a sandwich-like carbon@spinel@layered@spinel@carbon shell. Reproduced from Ref. [116] with permission from Elsevier. (e) Cycle performance of uncoated Li1.2Ni0.13Co0.13Mn0.54O2 (LR) and Mg2TiO4 coated Li1.2Ni0.13Co0.13Mn0.54O2 (LR@MTO) at 2 C. Reproduced from Ref. [117] with permission from John Wiley and Sons. Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. [107] with permission from Elsevier. (c) The cycling performance of the Li1.2Ni0.13Co0.13Mn0.54O2 cathode coated with different contents of Al2O3 and polyacene at 0.2 C (APL is short for double-shelled of Al2O3 and polyacene, and the number represents different amount of polyacene). Reproduced from Ref. [115] with permission from Royal Society of Chemistry. (d) Schematic diagram of the detailed synthetic process of the LMR cathode coated with a sandwich-like carbon@spinel@layered@spinel@carbon shell. Reproduced from Ref. [116] with permission from Elsevier. (e) Cycle performance of uncoated Li1.2Ni0.13Co0.13Mn0.54O2 (LR) and Mg2TiO4 coated Li1.2Ni0.13Co0.13Mn0.54O2 (LR@MTO) at 2 C. Reproduced from Ref. [117] with permission from John Wiley and Sons. 12 5 5 127 #/texts/119 section_header body_heading False low body_heading body_heading True p12:body_region:0 body_zone column_1_of_2 1 2 p12:body_zone:column_1_of_2:white [255, 255, 255] white False False [37.7, 527.76, 64.79, 7.96] 3.2.2. Bulk doping 3.2.2. Bulk doping 3.2.2. Bulk doping 3.2.2. Bulk doping 12 10 10 132 #/texts/123 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p12:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 379 379 379 379 13 2 1 133 #/texts/124 page_header page_header False low docling_page_header docling_page_header True p13:body_region:0 top_margin column_1_of_2 1 2 p13:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 13 3 2 134 #/texts/125 page_header page_header False low docling_page_header docling_page_header True p13:body_region:1 top_margin column_2_of_2 2 2 p13:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.71, 47.86, 139.91, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 13 4 3 135 #/texts/126 caption caption False low outside_body_flow_caption outside_body_flow_caption False None front_matter column_1_of_2 1 2 p13:front_matter:column_1_of_2:white [255, 255, 255] white False False [37.59, 273.34, 520.06, 40.18] Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li… Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li… Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li1.2Mn0.54Ni0.13Co0.13O2 oxide in the bulk and the spinel structure at the surface after GO modification. Reproduced from Ref. [118] with permission from Royal Society of Chemistry. (c) The synthetic scheme of chemical adsorption to modified MoO2S2 at the surface of LMR cathode and the corresponding structure at each step. (d) HRTEM and the corresponding FFT and refined lattice images of the MoO2S2 modified LMR cathode. Reproduced from Ref. [119] with permission from American Chemical Society. Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li1.2Mn0.54Ni0.13Co0.13O2 oxide in the bulk and the spinel structure at the surface after GO modification. Reproduced from Ref. [118] with permission from Royal Society of Chemistry. (c) The synthetic scheme of chemical adsorption to modified MoO2S2 at the surface of LMR cathode and the corresponding structure at each step. (d) HRTEM and the corresponding FFT and refined lattice images of the MoO2S2 modified LMR cathode. Reproduced from Ref. [119] with permission from American Chemical Society. 13 5 4 136 #/texts/127 caption caption False low outside_body_flow_caption outside_body_flow_caption False None front_matter column_1_of_2 1 2 p13:front_matter:column_1_of_2:white [255, 255, 255] white False False [37.59, 537.3, 520.07, 40.23] Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode … Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode … Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode and un-modified cathode at C/3. (c) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode after 100 cycles along [100] zone axis and the corresponding atomic models. Reproduced from Ref. [122] with permission from American Chemical Society. (d) XRD patterns of Li1.2Ni0.16Mn0.56Co0.08O2 samples doped by different Al contents. (e) The average voltage of the Li1.2Ni0.16Mn0.56Co0.08O2 cathode doped by different Al contents during cycling at 0.1 C. Reproduced from Ref. [124] with permission from John Wiley and Sons. Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode and un-modified cathode at C/3. (c) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode after 100 cycles along [100] zone axis and the corresponding atomic models. Reproduced from Ref. [122] with permission from American Chemical Society. (d) XRD patterns of Li1.2Ni0.16Mn0.56Co0.08O2 samples doped by different Al contents. (e) The average voltage of the Li1.2Ni0.16Mn0.56Co0.08O2 cathode doped by different Al contents during cycling at 0.1 C. Reproduced from Ref. [124] with permission from John Wiley and Sons. 13 7 7 139 #/texts/129 section_header body_heading False low body_heading body_heading True p13:body_region:1 body_zone column_2_of_2 2 2 p13:body_zone:column_2_of_2:white [255, 255, 255] white False False [306.65, 642.84, 89.45, 7.96] 3.3. Surface modification 3.3. Surface modification 3.3. Surface modification 3.3. Surface modification 13 9 9 141 #/texts/131 section_header body_heading False low body_heading body_heading True p13:body_region:1 body_zone column_2_of_2 2 2 p13:body_zone:column_2_of_2:white [255, 255, 255] white False False [306.65, 705.6, 77.14, 7.96] 3.3.1. Surface coating 3.3.1. Surface coating 3.3.1. Surface coating 3.3.1. Surface coating 13 11 11 143 #/texts/133 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p13:bottom_margin:column_2_of_2:white [253, 253, 253] white False True [291.91, 764.24, 11.38, 5.93] 380 380 380 380 14 2 1 144 #/texts/134 page_header page_header False low docling_page_header docling_page_header True p14:body_region:0 top_margin column_1_of_2 1 2 p14:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 14 8 5 148 #/texts/139 caption caption False low outside_body_flow_caption outside_body_flow_caption False None bottom_margin column_1_of_2 1 2 p14:bottom_margin:column_1_of_2:white [255, 255, 255] white False False [116.73, 749.05, 361.77, 5.93] Fig. 11. Schematic illustration for the recent progress in improving the electrochemical performance of LMR cathodes. Fig. 11. Schematic illustration for the recent progress in improving the electrochemical performance of LMR cathodes. Fig. 11. Schematic illustration for the recent progress in improving the electrochemical performance of LMR cathodes. Fig. 11. Schematic illustration for the recent progress in improving the electrochemical performance of LMR cathodes. 14 3 6 149 #/texts/135 page_header page_header False low docling_page_header docling_page_header True p14:body_region:1 top_margin column_2_of_2 2 2 p14:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.77, 47.8, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 14 9 9 152 #/texts/140 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p14:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 381 381 381 381 15 2 1 153 #/texts/141 page_header page_header False low docling_page_header docling_page_header True p15:body_region:0 top_margin column_1_of_2 1 2 p15:top_margin:column_1_of_2:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. 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Surface doping 15 3 7 159 #/texts/142 page_header page_header False low docling_page_header docling_page_header True p15:body_region:1 top_margin column_2_of_2 2 2 p15:top_margin:column_2_of_2:white [255, 255, 255] white False False [417.71, 47.86, 139.91, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 15 10 10 162 #/texts/148 section_header body_heading False low body_heading body_heading True p15:body_region:1 body_zone column_2_of_2 2 2 p15:body_zone:column_2_of_2:white [255, 255, 255] white False False [306.65, 510.24, 112.01, 7.96] 3.3.3. Other surface treatments 3.3.3. Other surface treatments 3.3.3. Other surface treatments 3.3.3. Other surface treatments 15 13 13 165 #/texts/151 page_footer page_footer False low docling_page_footer docling_page_footer False None bottom_margin column_2_of_2 2 2 p15:bottom_margin:column_2_of_2:white [255, 255, 255] white False False [291.91, 764.24, 11.45, 5.93] 382 382 382 382 16 2 1 166 #/texts/152 page_header page_header False low docling_page_header docling_page_header True p16:body_region:0 top_margin left None None p16:top_margin:left:white [255, 255, 255] white False False [37.59, 47.86, 69.84, 6.37] Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. Y. Li, Z. Li, C. Chen et al. 16 3 2 167 #/texts/153 page_header page_header False low docling_page_header docling_page_header False None top_margin right None None p16:top_margin:right:white [255, 255, 255] white False False [417.77, 47.8, 139.86, 6.37] Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 Journal of Energy Chemistry 61 (2021) 368-385 16 15 4 169 #/texts/165 section_header back_matter_heading False low early_back_matter_heading early_back_matter_heading False None front_matter right_crossing None None p16:front_matter:right_crossing:white [255, 255, 255] white False False [306.6, 68.75, 73.61, 7.42] Acknowledgments Acknowledgments Acknowledgments Acknowledgments 16 16 5 170 #/texts/166 text body_candidate_excluded False high inside_back_matter inside_back_matter False None front_matter right_crossing None None p16:front_matter:right_crossing:white [255, 255, 255] white False False [306.6, 89.67, 251.05, 49.26] This work was financially supported by the National Key R&D Program of China (2016YFB0700600), the Soft Science Research Project of Guangdong Province (No. 2017B030301013), and the Shenzhen Science and Technology Resear… This work was financially supported by the National Key R&D Program of China (2016YFB0700600), the Soft Science Research Project of Guangdong Province (No. 2017B030301013), and the Shenzhen Science and Technology Resear… This work was financially supported by the National Key R&D Program of China (2016YFB0700600), the Soft Science Research Project of Guangdong Province (No. 2017B030301013), and the Shenzhen Science and Technology Research Grant (ZDSYS201707281026184). 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