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"layout_order": 16, "layout_page_order": 17, "bbox": [ 202.0, 382.68, 357.8, 73.53 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "1,3-Divinyltetramethyldisiloxane (DTMS) is a multifunctional additive that is used to improves the cycling stability and capacity retention of Li-rich Mn-based layered oxide cathodes (LRMs). Cycling performance evaluations demonstrate that LRM/Li cells without the additive exhibit lower capacity retention. DTMS can significantly improve the capacity retention of LRM/Li cells from 42.8% to 75% at 0.5C. Theoretical calculations indicate that DTMS is preferentially oxidized on the LRM surface. Physical characterization results reveal that DTMS generates a layer on the LRM surface that is both less resistive and thinner than the LRM by reacting with HF/F from the electrolyte. This DTMS-derived layer inhibits adverse reactions between the cathode and electrolyte, thus, effectively maintaining the cathode structure.", "text_preview": "1,3-Divinyltetramethyldisiloxane (DTMS) is a multifunctional additive that is used to improves the cycling stability and capacity retention of Li-rich Mn-based layered oxide cathodes (LRMs). Cycling performance evaluati…", "word_count": 113, "cleaned_text": "1,3-Divinyltetramethyldisiloxane (DTMS) is a multifunctional additive that is used to improves the cycling stability and capacity retention of Li-rich Mn-based layered oxide cathodes (LRMs). Cycling performance evaluations demonstrate that LRM/Li cells without the additive exhibit lower capacity retention. DTMS can significantly improve the capacity retention of LRM/Li cells from 42.8% to 75% at 0.5C. Theoretical calculations indicate that DTMS is preferentially oxidized on the LRM surface. Physical characterization results reveal that DTMS generates a layer on the LRM surface that is both less resistive and thinner than the LRM by reacting with HF/F from the electrolyte. This DTMS-derived layer inhibits adverse reactions between the cathode and electrolyte, thus, effectively maintaining the cathode structure.", "cleaned_text_preview": "1,3-Divinyltetramethyldisiloxane (DTMS) is a multifunctional additive that is used to improves the cycling stability and capacity retention of Li-rich Mn-based layered oxide cathodes (LRMs). 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Introduction", "text_preview": "1. Introduction", "word_count": 2, "cleaned_text": "1. Introduction", "cleaned_text_preview": "1. Introduction", "included_in_body": false, "body_decision_reason": "body_heading", "parser_body_decision_reason": "body_heading", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p1:body_region:0", "role_guess": "body_heading", "zone": "body_zone", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": true, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.137, "bottom": 0.0, "left": 0.03, "right": 0.0 }, "excluded_risk_level": "low", "region_id": "p1:body_zone:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/18", "page": 1, "label": "footnote", "order": 18000, "source_page_order": 19, "layout_order": 19, "layout_page_order": 20, "bbox": [ 42.63, 672.84, 153.92, 16.16 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "* Corresponding author. E-mail address: mxwu@fjirsm.ac.cn (M. Wu).", "text_preview": "* Corresponding author. E-mail address: mxwu@fjirsm.ac.cn (M. Wu).", "word_count": 8, "cleaned_text": "* Corresponding author. E-mail address: mxwu@fjirsm.ac.cn (M. Wu).", "cleaned_text_preview": "* Corresponding author. E-mail address: mxwu@fjirsm.ac.cn (M. 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It can be found that the cells in the 2 vol% DTMS-containing electrolyte have a large charge capacity of 321.2 mAh g 1 and that they delivered a lower coulombic efficiency (92.5%) than the cells in the BE electrolyte (97.2%). This may be due to DTMS oxidation occurring prior to that of electrolyte solvents. Fig. 2 presents the comparison of the cycling performance of LRM/Li cells in the", "text_preview": "Supplementary Material. 2 shows the charge -discharge curve performance of LRM/Li cells with and without 2 vol% DTMS electrolytes during the first pre-cycle process. It can be found that the cells in the 2 vol% DTMS-con…", "word_count": 92, "cleaned_text": "Supplementary Material. 2 shows the charge -discharge curve performance of LRM/Li cells with and without 2 vol% DTMS electrolytes during the first pre-cycle process. It can be found that the cells in the 2 vol% DTMS-containing electrolyte have a large charge capacity of 321.2 mAh g 1 and that they delivered a lower coulombic efficiency (92.5%) than the cells in the BE electrolyte (97.2%). This may be due to DTMS oxidation occurring prior to that of electrolyte solvents. Fig. 2 presents the comparison of the cycling performance of LRM/Li cells in the", "cleaned_text_preview": "Supplementary Material. 2 shows the charge -discharge curve performance of LRM/Li cells with and without 2 vol% DTMS electrolytes during the first pre-cycle process. It can be found that the cells in the 2 vol% DTMS-con…", "included_in_body": false, "body_decision_reason": "early_back_matter_heading", "parser_body_decision_reason": "early_back_matter_heading", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p2:body_region:1", "role_guess": "back_matter_heading", "zone": "bottom_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": true, "body_heading": false, "heading_kind": "back_matter", "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.095, "bottom": 0.017, "left": 0.09, "right": 0.0 }, "excluded_risk_level": "low", "region_id": "p2:bottom_margin:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/49", "page": 2, "label": "page_footer", "order": 49000, "source_page_order": 24, "layout_order": 49, "layout_page_order": 24, "bbox": [ 296.21, 754.45, 3.59, 10.42 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "2", "text_preview": "2", "word_count": 1, "cleaned_text": "2", "cleaned_text_preview": "2", "included_in_body": false, "body_decision_reason": "docling_page_footer", "parser_body_decision_reason": "docling_page_footer", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "page_footer", "zone": "bottom_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": true, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.0, "bottom": 0.0, "left": 0.078, "right": 0.133 }, "excluded_risk_level": "low", "region_id": "p2:bottom_margin:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/50", "page": 3, "label": "page_header", "order": 50000, "source_page_order": 2, "layout_order": 50, "layout_page_order": 1, "bbox": [ 433.38, 33.65, 124.91, 10.42 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Journal of Power Sources 580 (2023) 233437", "text_preview": "Journal of Power Sources 580 (2023) 233437", "word_count": 7, "cleaned_text": "Journal of Power Sources 580 (2023) 233437", "cleaned_text_preview": "Journal of Power Sources 580 (2023) 233437", "included_in_body": false, "body_decision_reason": "docling_page_header", "parser_body_decision_reason": "docling_page_header", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:1", "role_guess": "page_header", "zone": "top_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": true, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.0, "bottom": 0.002, "left": 0.073, "right": 0.125 }, "excluded_risk_level": "low", "region_id": "p3:top_margin:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/48#prov1", "page": 3, "label": "text", "order": 48001, "source_page_order": 1, "layout_order": 51, "layout_page_order": 2, "bbox": [ 37.59, 36.99, 463.07, 5.85 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "T. Huang et al.", "text_preview": "T. Huang et al.", "word_count": 4, "cleaned_text": "T. Huang et al.", "cleaned_text_preview": "T. Huang et al.", "included_in_body": false, "body_decision_reason": "page_margin_header", "parser_body_decision_reason": "page_margin_header", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:0", "role_guess": "page_margin_header", "zone": "top_margin", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": true, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.017, "bottom": 0.021, "left": 0.074, "right": 0.185 }, "excluded_risk_level": "low", "region_id": "p3:top_margin:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/51", "page": 3, "label": "caption", "order": 51000, "source_page_order": 3, "layout_order": 52, "layout_page_order": 3, "bbox": [ 179.09, 187.18, 241.32, 8.3 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Fig. 1. Optimized structures and Eb values of solvents-Li + and DTMS-Li + .", "text_preview": "Fig. 1. Optimized structures and Eb values of solvents-Li + and DTMS-Li + .", "word_count": 14, "cleaned_text": "Fig. 1. Optimized structures and Eb values of solvents-Li + and DTMS-Li + .", "cleaned_text_preview": "Fig. 1. Optimized structures and Eb values of solvents-Li + and DTMS-Li + .", "included_in_body": false, "body_decision_reason": "outside_body_flow_caption", "parser_body_decision_reason": "outside_body_flow_caption", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "caption", "zone": "page_body", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.0, "bottom": 0.108, "left": 0.115, "right": 0.0 }, "excluded_risk_level": "low", "region_id": "p3:page_body:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/52", "page": 3, "label": "caption", "order": 52000, "source_page_order": 4, "layout_order": 53, "layout_page_order": 4, "bbox": [ 38.95, 472.99, 521.55, 6.58 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Fig. 2. (a) Cycling performance and (b) rate capability of LRM/Li cell. (c) (d) 1st, 20th, 50th, and 100th charge -discharge curves of LRM/Li cell during cycling.", "text_preview": "Fig. 2. (a) Cycling performance and (b) rate capability of LRM/Li cell. (c) (d) 1st, 20th, 50th, and 100th charge -discharge curves of LRM/Li cell during cycling.", "word_count": 27, "cleaned_text": "Fig. 2. (a) Cycling performance and (b) rate capability of LRM/Li cell. (c) (d) 1st, 20th, 50th, and 100th charge -discharge curves of LRM/Li cell during cycling.", "cleaned_text_preview": "Fig. 2. (a) Cycling performance and (b) rate capability of LRM/Li cell. (c) (d) 1st, 20th, 50th, and 100th charge -discharge curves of LRM/Li cell during cycling.", "included_in_body": false, "body_decision_reason": "outside_body_flow_caption", "parser_body_decision_reason": "outside_body_flow_caption", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "caption", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.056, "bottom": 0.119, "left": 0.233, "right": 0.0 }, "excluded_risk_level": "low", "region_id": "p3:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/53", "page": 3, "label": "text", "order": 53000, "source_page_order": 5, "layout_order": 54, "layout_page_order": 5, "bbox": [ 37.59, 494.91, 253.44, 174.67 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "different electrolytes. The LRM/Li cells with 2 vol% DTMS showed great cycling stability. The discharge capacity of LRM/Li cells in the BE electrolyte decreased from 262.3 to 57.7 mAh g 1 after 100 cycles (57.2% capacity loss). However, in the 2 vol% DTMS-containing electrolyte, the discharge capacity decreased from 256.2 to 192.7 mAh g 1 (25% capacity loss). To estimate whether the Li/Li-rich cells with the DTMS-containing electrolyte are capable of fast charge transport, the rate capability of LRM/Li cells was evaluated. The Li/Li-rich cells with 2 vol% DTMS delivered a higher discharge capacity of 100 mAh g 1 at 5C. In contrast, the LRM/Li cells with the BE electrolyte exhibited substantial capacity loss. The 1st, 20th, 50th, and 100th charge -discharge curves of the LRM/Li cell during cycling are presented in Fig. 2c and d. An obvious decrease in the discharge capacity and voltage platform can be seen for the cell without additives during cycling, which may indicate increased interfacial instability. The charge and discharge capacities of LRM/Li cells in DTMS-containing electrolyte remained at a desirable level.", "text_preview": "different electrolytes. The LRM/Li cells with 2 vol% DTMS showed great cycling stability. The discharge capacity of LRM/Li cells in the BE electrolyte decreased from 262.3 to 57.7 mAh g 1 after 100 cycles (57.2% capacit…", "word_count": 178, "cleaned_text": "different electrolytes. The LRM/Li cells with 2 vol% DTMS showed great cycling stability. The discharge capacity of LRM/Li cells in the BE electrolyte decreased from 262.3 to 57.7 mAh g 1 after 100 cycles (57.2% capacity loss). However, in the 2 vol% DTMS-containing electrolyte, the discharge capacity decreased from 256.2 to 192.7 mAh g 1 (25% capacity loss). To estimate whether the Li/Li-rich cells with the DTMS-containing electrolyte are capable of fast charge transport, the rate capability of LRM/Li cells was evaluated. The Li/Li-rich cells with 2 vol% DTMS delivered a higher discharge capacity of 100 mAh g 1 at 5C. In contrast, the LRM/Li cells with the BE electrolyte exhibited substantial capacity loss. The 1st, 20th, 50th, and 100th charge -discharge curves of the LRM/Li cell during cycling are presented in Fig. 2c and d. An obvious decrease in the discharge capacity and voltage platform can be seen for the cell without additives during cycling, which may indicate increased interfacial instability. The charge and discharge capacities of LRM/Li cells in DTMS-containing electrolyte remained at a desirable level.", "cleaned_text_preview": "different electrolytes. The LRM/Li cells with 2 vol% DTMS showed great cycling stability. The discharge capacity of LRM/Li cells in the BE electrolyte decreased from 262.3 to 57.7 mAh g 1 after 100 cycles (57.2% capacit…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:0", "role_guess": "body_candidate_excluded", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.151, "bottom": 0.0, "left": 0.103, "right": 0.0 }, "excluded_risk_level": "high", "region_id": "p3:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/54#prov0", "page": 3, "label": "text", "order": 54000, "source_page_order": 6, "layout_order": 55, "layout_page_order": 6, "bbox": [ 37.59, 672.7, 253.44, 70.07 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "EIS was carried out on LRM/Li cells after pre-cycling and cycling with the BE and 2 vol% DTMS-containing electrolytes, as shown in Fig. 3. The results can be divided into two parts: a depressed semicircle followed by a slanting line. The depressed semicircle contains two parts: the surface-film resistance (Rf) and the charge-transfer resistance (Rct) between the electrode and electrolyte. 24 The values in Fig. 3c reveal that the cell with the BE electrolyte shows a greater numerical variation", "text_preview": "EIS was carried out on LRM/Li cells after pre-cycling and cycling with the BE and 2 vol% DTMS-containing electrolytes, as shown in Fig. 3. The results can be divided into two parts: a depressed semicircle followed by a …", "word_count": 79, "cleaned_text": "EIS was carried out on LRM/Li cells after pre-cycling and cycling with the BE and 2 vol% DTMS-containing electrolytes, as shown in Fig. 3. The results can be divided into two parts: a depressed semicircle followed by a slanting line. The depressed semicircle contains two parts: the surface-film resistance (Rf) and the charge-transfer resistance (Rct) between the electrode and electrolyte. 24 The values in Fig. 3c reveal that the cell with the BE electrolyte shows a greater numerical variation", "cleaned_text_preview": "EIS was carried out on LRM/Li cells after pre-cycling and cycling with the BE and 2 vol% DTMS-containing electrolytes, as shown in Fig. 3. The results can be divided into two parts: a depressed semicircle followed by a …", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:0", "role_guess": "body_candidate_excluded", "zone": "bottom_margin", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.109, "bottom": 0.004, "left": 0.083, "right": 0.0 }, "excluded_risk_level": "high", "region_id": "p3:bottom_margin:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/54#prov1", "page": 3, "label": "text", "order": 54001, "source_page_order": 7, "layout_order": 56, "layout_page_order": 7, "bbox": [ 306.59, 494.91, 253.4, 38.66 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "in Rf and Rct compared with the cells with the DTMS-containing electrolyte. The electrolyte decomposition substantially deteriorates the properties of the interface between the LRM and BE electrolyte and thereby reduces the cycling performance.", "text_preview": "in Rf and Rct compared with the cells with the DTMS-containing electrolyte. The electrolyte decomposition substantially deteriorates the properties of the interface between the LRM and BE electrolyte and thereby reduces…", "word_count": 34, "cleaned_text": "in Rf and Rct compared with the cells with the DTMS-containing electrolyte. The electrolyte decomposition substantially deteriorates the properties of the interface between the LRM and BE electrolyte and thereby reduces the cycling performance.", "cleaned_text_preview": "in Rf and Rct compared with the cells with the DTMS-containing electrolyte. The electrolyte decomposition substantially deteriorates the properties of the interface between the LRM and BE electrolyte and thereby reduces…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:1", "role_guess": "body_candidate_excluded", "zone": "page_body", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.135, "bottom": 0.014, "left": 0.078, "right": 0.0 }, "excluded_risk_level": "high", "region_id": "p3:page_body:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/55", "page": 3, "label": "text", "order": 55000, "source_page_order": 8, "layout_order": 57, "layout_page_order": 8, "bbox": [ 306.59, 536.75, 253.43, 122.34 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "The surface morphologies of the cathodes in the BE and DTMScontaining electrolytes were analyzed after cycling by SEM and TEM (Fig. 4). As shown in Fig. 4a, the cathode surface in the BE electrolyte was covered with a thick and uneven layer. The thickness is approximately 10 -15 nm. In contrast, the thickness of the cathode surface in the DTMS-containing electrolytes is only 2 -4 nm (Fig. 4b). After cycling, serious structure damage was found for the LRM particles in the BE electrolytes (Fig. 4c). These changes in surface morphology are most likely due to the HF continuous corrosion. The microstructure of the LRM particles in the DTMS-containing electrolytes was well maintained, as shown in Fig. 4d. It could be assumed the CEI layer was created by DTMS inhibiting HF corrosion on the cathode surface.", "text_preview": "The surface morphologies of the cathodes in the BE and DTMScontaining electrolytes were analyzed after cycling by SEM and TEM (Fig. 4). As shown in Fig. 4a, the cathode surface in the BE electrolyte was covered with a t…", "word_count": 135, "cleaned_text": "The surface morphologies of the cathodes in the BE and DTMScontaining electrolytes were analyzed after cycling by SEM and TEM (Fig. 4). As shown in Fig. 4a, the cathode surface in the BE electrolyte was covered with a thick and uneven layer. The thickness is approximately 10 -15 nm. In contrast, the thickness of the cathode surface in the DTMS-containing electrolytes is only 2 -4 nm (Fig. 4b). After cycling, serious structure damage was found for the LRM particles in the BE electrolytes (Fig. 4c). These changes in surface morphology are most likely due to the HF continuous corrosion. The microstructure of the LRM particles in the DTMS-containing electrolytes was well maintained, as shown in Fig. 4d. It could be assumed the CEI layer was created by DTMS inhibiting HF corrosion on the cathode surface.", "cleaned_text_preview": "The surface morphologies of the cathodes in the BE and DTMScontaining electrolytes were analyzed after cycling by SEM and TEM (Fig. 4). As shown in Fig. 4a, the cathode surface in the BE electrolyte was covered with a t…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:1", "role_guess": "body_candidate_excluded", "zone": "page_body", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.118, "bottom": 0.002, "left": 0.026, "right": 0.0 }, "excluded_risk_level": "high", "region_id": "p3:page_body:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/56", "page": 3, "label": "text", "order": 56000, "source_page_order": 9, "layout_order": 58, "layout_page_order": 9, "bbox": [ 306.59, 662.27, 253.42, 80.5 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Fig. 5a depicts the obtained XPS of LRM cells with BE and DMSEcontaining electrolytes after cycling. The C 1s peaks at 290.3 and 285.4 eV correspond to PVDF [19,25], and the peak at 284.6 eV is assigned to acetylene black [17]. Furthermore, the peak intensities of the PVDF and acetylene black of the LRM electrode in the BE electrolyte after cycling were higher than those in DTMS-containing electrolytes, which indicates that a thinner CEI film was formed with DTMS. The peaks corresponding to electrolyte decomposition products [19,25]", "text_preview": "Fig. 5a depicts the obtained XPS of LRM cells with BE and DMSEcontaining electrolytes after cycling. The C 1s peaks at 290.3 and 285.4 eV correspond to PVDF [19,25], and the peak at 284.6 eV is assigned to acetylene bla…", "word_count": 87, "cleaned_text": "Fig. 5a depicts the obtained XPS of LRM cells with BE and DMSEcontaining electrolytes after cycling. The C 1s peaks at 290.3 and 285.4 eV correspond to PVDF [19,25], and the peak at 284.6 eV is assigned to acetylene black [17]. Furthermore, the peak intensities of the PVDF and acetylene black of the LRM electrode in the BE electrolyte after cycling were higher than those in DTMS-containing electrolytes, which indicates that a thinner CEI film was formed with DTMS. The peaks corresponding to electrolyte decomposition products [19,25]", "cleaned_text_preview": "Fig. 5a depicts the obtained XPS of LRM cells with BE and DMSEcontaining electrolytes after cycling. The C 1s peaks at 290.3 and 285.4 eV correspond to PVDF [19,25], and the peak at 284.6 eV is assigned to acetylene bla…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p3:body_region:1", "role_guess": "body_candidate_excluded", "zone": "bottom_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.158, "bottom": 0.017, "left": 0.09, "right": 0.0 }, "excluded_risk_level": "high", "region_id": "p3:bottom_margin:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/57", "page": 3, "label": "page_footer", "order": 57000, "source_page_order": 10, "layout_order": 59, "layout_page_order": 10, "bbox": [ 296.21, 754.45, 3.59, 10.42 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "3", "text_preview": "3", "word_count": 1, "cleaned_text": "3", "cleaned_text_preview": "3", "included_in_body": false, "body_decision_reason": "docling_page_footer", "parser_body_decision_reason": "docling_page_footer", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "page_footer", "zone": "bottom_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": true, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.0, "bottom": 0.0, "left": 0.067, "right": 0.133 }, "excluded_risk_level": "low", "region_id": "p3:bottom_margin:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/58", "page": 4, "label": "page_header", "order": 58000, "source_page_order": 1, "layout_order": 60, "layout_page_order": 1, "bbox": [ 433.38, 33.65, 124.91, 10.42 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Journal of Power Sources 580 (2023) 233437", "text_preview": "Journal of Power Sources 580 (2023) 233437", "word_count": 7, "cleaned_text": "Journal of Power Sources 580 (2023) 233437", "cleaned_text_preview": "Journal of Power Sources 580 (2023) 233437", "included_in_body": false, "body_decision_reason": "docling_page_header", "parser_body_decision_reason": "docling_page_header", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p4:body_region:1", "role_guess": "page_header", "zone": "top_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": true, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.0, "bottom": 0.002, "left": 0.073, "right": 0.125 }, "excluded_risk_level": "low", "region_id": "p4:top_margin:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/59", "page": 4, "label": "text", "order": 59000, "source_page_order": 2, "layout_order": 61, "layout_page_order": 2, "bbox": [ 37.59, 36.99, 463.07, 5.85 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "T. Huang et al.", "text_preview": "T. Huang et al.", "word_count": 4, "cleaned_text": "T. Huang et al.", "cleaned_text_preview": "T. Huang et al.", "included_in_body": false, "body_decision_reason": "page_margin_header", "parser_body_decision_reason": "page_margin_header", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p4:body_region:0", "role_guess": "page_margin_header", "zone": "top_margin", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": true, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.017, "bottom": 0.021, "left": 0.074, "right": 0.185 }, "excluded_risk_level": "low", "region_id": "p4:top_margin:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/60", "page": 4, "label": "caption", "order": 60000, "source_page_order": 3, "layout_order": 62, "layout_page_order": 3, "bbox": [ 86.63, 307.39, 426.25, 6.58 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Fig. 3. EIS results of LRM/Li cell in BE and 2 vol% DTMS electrolyte after (a) pre-cycling and (b) cycling. (c) Values of Rf and Rct.", "text_preview": "Fig. 3. EIS results of LRM/Li cell in BE and 2 vol% DTMS electrolyte after (a) pre-cycling and (b) cycling. (c) Values of Rf and Rct.", "word_count": 26, "cleaned_text": "Fig. 3. EIS results of LRM/Li cell in BE and 2 vol% DTMS electrolyte after (a) pre-cycling and (b) cycling. (c) Values of Rf and Rct.", "cleaned_text_preview": "Fig. 3. EIS results of LRM/Li cell in BE and 2 vol% DTMS electrolyte after (a) pre-cycling and (b) cycling. (c) Values of Rf and Rct.", "included_in_body": false, "body_decision_reason": "outside_body_flow_caption", "parser_body_decision_reason": "outside_body_flow_caption", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "caption", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.142, "bottom": 0.023, "left": 0.15, "right": 0.0 }, "excluded_risk_level": "low", "region_id": "p4:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/61", "page": 4, "label": "caption", "order": 61000, "source_page_order": 4, "layout_order": 63, "layout_page_order": 4, "bbox": [ 112.82, 587.51, 373.83, 6.58 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "Fig. 4. TEM and SEM images of LRM cathodes after cycling (a), (c) with BE and (b), (d) 2 vol% DTMS electrolyte.", "text_preview": "Fig. 4. TEM and SEM images of LRM cathodes after cycling (a), (c) with BE and (b), (d) 2 vol% DTMS electrolyte.", "word_count": 22, "cleaned_text": "Fig. 4. TEM and SEM images of LRM cathodes after cycling (a), (c) with BE and (b), (d) 2 vol% DTMS electrolyte.", "cleaned_text_preview": "Fig. 4. TEM and SEM images of LRM cathodes after cycling (a), (c) with BE and (b), (d) 2 vol% DTMS electrolyte.", "included_in_body": false, "body_decision_reason": "outside_body_flow_caption", "parser_body_decision_reason": "outside_body_flow_caption", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": false, "body_region_id": null, "role_guess": "caption", "zone": "page_body", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": true, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": false, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.171, "bottom": 0.016, "left": 0.233, "right": 0.0 }, "excluded_risk_level": "low", "region_id": "p4:page_body:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/62#prov0", "page": 4, "label": "text", "order": 62000, "source_page_order": 5, "layout_order": 64, "layout_page_order": 5, "bbox": [ 37.59, 609.43, 253.44, 132.83 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "(ROCO2Li, ROLi, and Li2CO3) at 286 and 288.8 eV were observed. The peak intensities for the electrolyte with DTMS were lower than those for the BE electrolyte. The same result can be observed in O 1s spectra. The peak intensities corresponding to C --O (531.9 eV) [17,19], C -O (533.4 eV)[ 25], and Li2CO3 (531.2 eV) [19] for the electrolyte with DTMS were lower. The F 1s peaks at 684.5 and 685.8 eV were assigned to LiF and Me -F [19], respectively. The peak at 56 eV [31] corresponds to LiF in the Li 1s spectra. For the BE electrolyte, the peak intensities of LiF and Me -F are higher in the F 1s spectra. The peaks at 686.9 eV [19] for LixPFy and LixPOyFz in the BE electrolyte are higher than those in the DTMS-containing electrolyte in the F 1s spectra, which may be due to the LiPF6 decomposition. This is in accordance with the P 1s spectra for the peaks of LixPFy (136.5 eV) and LixPOyFz (133.8 eV) [23]. In", "text_preview": "(ROCO2Li, ROLi, and Li2CO3) at 286 and 288.8 eV were observed. The peak intensities for the electrolyte with DTMS were lower than those for the BE electrolyte. The same result can be observed in O 1s spectra. The peak i…", "word_count": 172, "cleaned_text": "(ROCO2Li, ROLi, and Li2CO3) at 286 and 288.8 eV were observed. The peak intensities for the electrolyte with DTMS were lower than those for the BE electrolyte. The same result can be observed in O 1s spectra. The peak intensities corresponding to C --O (531.9 eV) [17,19], C -O (533.4 eV)[ 25], and Li2CO3 (531.2 eV) [19] for the electrolyte with DTMS were lower. The F 1s peaks at 684.5 and 685.8 eV were assigned to LiF and Me -F [19], respectively. The peak at 56 eV [31] corresponds to LiF in the Li 1s spectra. For the BE electrolyte, the peak intensities of LiF and Me -F are higher in the F 1s spectra. The peaks at 686.9 eV [19] for LixPFy and LixPOyFz in the BE electrolyte are higher than those in the DTMS-containing electrolyte in the F 1s spectra, which may be due to the LiPF6 decomposition. This is in accordance with the P 1s spectra for the peaks of LixPFy (136.5 eV) and LixPOyFz (133.8 eV) [23]. In", "cleaned_text_preview": "(ROCO2Li, ROLi, and Li2CO3) at 286 and 288.8 eV were observed. The peak intensities for the electrolyte with DTMS were lower than those for the BE electrolyte. The same result can be observed in O 1s spectra. The peak i…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p4:body_region:0", "role_guess": "body_candidate_excluded", "zone": "bottom_margin", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": false, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.142, "bottom": 0.021, "left": 0.167, "right": 0.0 }, "excluded_risk_level": "high", "region_id": "p4:bottom_margin:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/62#prov1", "page": 4, "label": "text", "order": 62001, "source_page_order": 6, "layout_order": 65, "layout_page_order": 6, "bbox": [ 306.59, 609.43, 253.42, 49.15 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "conclusion, the peak intensities for the electrolyte decomposition products on the cathode in the DTMS-containing electrolyte were weaker, confirming that the electrolyte decomposition could be inhibited by DTMS. The existence of Si (Si 2p spectrum) indicates that the film on the cathode is formed from the oxidation of DTMS.", "text_preview": "conclusion, the peak intensities for the electrolyte decomposition products on the cathode in the DTMS-containing electrolyte were weaker, confirming that the electrolyte decomposition could be inhibited by DTMS. The ex…", "word_count": 49, "cleaned_text": "conclusion, the peak intensities for the electrolyte decomposition products on the cathode in the DTMS-containing electrolyte were weaker, confirming that the electrolyte decomposition could be inhibited by DTMS. The existence of Si (Si 2p spectrum) indicates that the film on the cathode is formed from the oxidation of DTMS.", "cleaned_text_preview": "conclusion, the peak intensities for the electrolyte decomposition products on the cathode in the DTMS-containing electrolyte were weaker, confirming that the electrolyte decomposition could be inhibited by DTMS. The ex…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p4:body_region:1", "role_guess": "body_heading", "zone": "page_body", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": true, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.113, "bottom": 0.0, "left": 0.115, "right": 0.0 }, "excluded_risk_level": "low", "region_id": "p4:page_body:column_2_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/63#prov0", "page": 4, "label": "text", "order": 63000, "source_page_order": 7, "layout_order": 66, "layout_page_order": 7, "bbox": [ 306.59, 661.76, 253.43, 80.5 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "The XRD results for the cathodes before and after cycling with the BE and 2% DTMS-containing electrolytes are shown in Fig. 5b: the XRD peak intensity of the cathode in the BE electrolyte reduces drastically after cycling. The peak (003) broadens and shifts slightly to a higher angle [19], indicating severe structural damage on the LRM electrode in the BE electrolyte. However, after cycling, the LRM electrode with the 2% DTMS-containing electrolyte exhibits almost the same diffraction pattern as that before cycling, indicating that the crystal structure of the", "text_preview": "The XRD results for the cathodes before and after cycling with the BE and 2% DTMS-containing electrolytes are shown in Fig. 5b: the XRD peak intensity of the cathode in the BE electrolyte reduces drastically after cycli…", "word_count": 89, "cleaned_text": "The XRD results for the cathodes before and after cycling with the BE and 2% DTMS-containing electrolytes are shown in Fig. 5b: the XRD peak intensity of the cathode in the BE electrolyte reduces drastically after cycling. The peak (003) broadens and shifts slightly to a higher angle [19], indicating severe structural damage on the LRM electrode in the BE electrolyte. However, after cycling, the LRM electrode with the 2% DTMS-containing electrolyte exhibits almost the same diffraction pattern as that before cycling, indicating that the crystal structure of the", "cleaned_text_preview": "The XRD results for the cathodes before and after cycling with the BE and 2% DTMS-containing electrolytes are shown in Fig. 5b: the XRD peak intensity of the cathode in the BE electrolyte reduces drastically after cycli…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p4:body_region:1", "role_guess": "body_candidate_excluded", "zone": "bottom_margin", "column": "column_2_of_2", "column_index": 2, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": 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(a)XPS spectra of LRM cathodes after cycling with BE and 2 vol% DTMS electrolytes. (b) XRD patterns of LRM cathodes and (c) dissolution of transition metal on Li electrode taken from cell after cycling.", "text_preview": "Fig. 5. (a)XPS spectra of LRM cathodes after cycling with BE and 2 vol% DTMS electrolytes. (b) XRD patterns of LRM cathodes and (c) dissolution of transition metal on Li electrode taken from cell after cycling.", "word_count": 36, "cleaned_text": "Fig. 5. (a)XPS spectra of LRM cathodes after cycling with BE and 2 vol% DTMS electrolytes. (b) XRD patterns of LRM cathodes and (c) dissolution of transition metal on Li electrode taken from cell after cycling.", "cleaned_text_preview": "Fig. 5. (a)XPS spectra of LRM cathodes after cycling with BE and 2 vol% DTMS electrolytes. 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This further confirms that the DTMS is beneficial for maintaining structure stability during cycling. As shown in Fig. 5c, the Mn, Ni, and Co contents were 0.284, 0.074, and 0.021 ppm, respectively, for the electrolyte without an additive, and 0.73, 0.316, and 0.087 ppm, respectively, for the electrolyte with DTMS. Thus, the XRD and ICP-MS results show that the dissolution of transition metals was suppressed by the protective CEI formed via DTMS oxidation.", "text_preview": "cathode was well maintained in DTMS-containing electrolyte. This further confirms that the DTMS is beneficial for maintaining structure stability during cycling. As shown in Fig. 5c, the Mn, Ni, and Co contents were 0.2…", "word_count": 80, "cleaned_text": "cathode was well maintained in DTMS-containing electrolyte. This further confirms that the DTMS is beneficial for maintaining structure stability during cycling. As shown in Fig. 5c, the Mn, Ni, and Co contents were 0.284, 0.074, and 0.021 ppm, respectively, for the electrolyte without an additive, and 0.73, 0.316, and 0.087 ppm, respectively, for the electrolyte with DTMS. Thus, the XRD and ICP-MS results show that the dissolution of transition metals was suppressed by the protective CEI formed via DTMS oxidation.", "cleaned_text_preview": "cathode was well maintained in DTMS-containing electrolyte. This further confirms that the DTMS is beneficial for maintaining structure stability during cycling. As shown in Fig. 5c, the Mn, Ni, and Co contents were 0.2…", "included_in_body": false, "body_decision_reason": "inside_back_matter", "parser_body_decision_reason": "inside_back_matter", "production_usage": "", "visual_asset_type": "", "visual_asset_label": "", "visual_asset_caption_preview": "", "visual_asset_anchor_ref": "", "inside_body_region": true, "body_region_id": "p5:body_region:0", "role_guess": "body_candidate_excluded", "zone": "front_matter", "column": "column_1_of_2", "column_index": 1, "column_count": 2, "flags": { "docling_non_body_label": false, "page_margin_noise": false, "metadata_line": false, "affiliation_block": false, "reference_item": false, "body_sentence": true, "body_candidate": true, "body_heading": false, "heading_kind": null, "has_front_matter_zone": false, "visual_text": false, "publisher_landing_page": false, "caption_continuation_used_by_asset": false }, "background_rgb": [ 255, 255, 255 ], "page_background_rgb": [ 255, 255, 255 ], "background_delta": 0, "background_class": "white", "is_gray_background": false, "has_frame_evidence": false, "edge_dark_ratios": { "top": 0.137, "bottom": 0.0, "left": 0.128, "right": 0.0 }, "excluded_risk_level": "high", "region_id": "p5:front_matter:column_1_of_2:white", "truncation_marker": "" }, { "ref": "#/texts/68", "page": 5, "label": "section_header", "order": 68000, "source_page_order": 5, "layout_order": 72, "layout_page_order": 5, "bbox": [ 37.59, 683.75, 124.69, 7.31 ], "page_size": { "width": 595.28, "height": 793.7 }, "text": "3.3. 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