这里是差集：Docling 全量解析 text block 减去最终会进入正文的 block。优先人工检查 risk=high / medium。
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这些框显示被排除块，同时叠加真实图表资产框。青色虚线表示该 text block 被图表资产 caption 吸收；红色 STOP 是截断触发点，红色框是截断后被排除的块。
这是实际图表资产输出，不是审计层重新推断。
| # | type | label | page | caption source | suppressed | duplicate reason | rescue reason | group | confidence | bbox | caption |
|---|---|---|---|---|---|---|---|---|---|---|---|
| 1 | figure | Fig. 1 | 3 | direct_caption_ref | 0.82 | [92.41, 274.75, 406.59, 274.15] | Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d synthesized from two different precursors (C for conventional precursor and H for hierarchically structured precursor). Reproduced from Ref. [27] with permission from American Chemical Society. (d) Structural scheme showing the honeycomb pattern consisting of Li@Mn6 superstructure units in LMR layered oxide. Reproduced from Ref. [29]) with permission from Royal Society of Chemistry. | ||||
| 2 | figure | Fig. 2 | 4 | direct_caption_ref | 0.82 | [90.0, 67.07, 410.02, 268.08] | Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chemical Society. (c) p DOS of O 2 p orbitals and Mn 3 d orbitals in Li2MnO3 and the corresponding oxygen environment model. Reproduced from Ref. [47] with permission from Springer Nature. (d) Cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 synthesized by two different synthesis methods at 0.1 C in the voltage range of 2.0-4.8 V. (e) The corresponding capacity-voltage profiles of the re-synthesized Li1.2Ni0.13Co0.13Mn0.54O2 in (d). Reproduced from Ref. [53] with permission from Elsevier. (f) Schematic representation for the structural transformation of trigonal LiMO2 component ( R -3m) and monoclinic Li2MnO3 component ( C 2/ m ) in Li1.2Ni0.1Mn0.525Co0.175O2 during cycling. Reproduced from Ref. [54] with permission from American Chemical Society. (g) Selected area electron diffraction (SAED) pattern obtained along [0001] zone axis of Li1.2Co0.1Mn0.55Ni0.15O2 cathode at the charging voltage of 4.5 V. (h) Schematic diagram of TM migration in Li1.2Co0.1Mn0.55Ni0.15O2 cathode when holding at 4.5 V. Reproduced from Ref. [55] with permission from Royal Society of Chemistry. | ||||
| 3 | figure | Fig. 3 | 6 | direct_caption_ref | 0.82 | [88.8, 229.03, 412.99, 325.76] | Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3 (1x )LiMnO2 nanorods. Reproduced from Ref. [63] with permission from Elsevier. (c) Schematic illustration of the synthetic process of orthogonally arranged nanoplates. Reproduced from Ref. [64] with permission from American Chemical Society. (d) Scheme of the fabrication process of 3D hollow porous bowl-shaped Li1.2Ni0.13Co0.13Mn0.54O2 particles. Reproduced from Ref. [66] with permission from Elsevier. (e) Schematic diagram of the suppression of voltage fading through a preferred orientation (110) plane. Reproduced from Ref. [67] with permission from Royal Society of Chemistry. | ||||
| 4 | figure | Fig. 4 | 7 | direct_caption_ref | 0.82 | [90.18, 66.44, 413.3, 260.3] | Fig. 4. (a) Schematic illustration of the formation of porous Li1.2Ni0.18Co0.08Mn0.54O2. Reproduced from Ref. [68] with permission from Royal Society of Chemistry. (b) Schematic illustration of the synthesizing route for 3D Li1.2Ni0.2Mn0.6O2 and the morphological evolution. Reproduced from Ref. [69] with permission from American Chemical Society. (c) SEM image of Li1.2Ni0.2Mn0.6O2 oxide. Reproduced from Ref. [70] with permission from American Chemical Society. | ||||
| 5 | figure | Fig. 5 | 7 | direct_caption_ref | 0.82 | [86.72, 381.93, 416.16, 275.14] | Fig. 5. (a) Schematic illustration of ice-template coprecipitation method to synthesize Li1.2Ni0.2Mn0.6O2 with hierarchical mesopore structure. (b) The rate performance of Li1.2Ni0.2Mn0.6O2 synthesized by freeze drying (M1) and vacuum drying (M2). Reproduced from Ref. [73] with permission from American Chemical Society. (c) Schematic diagram of building nano-porous structures in Li1.144Ni0.136Co0.136Mn0.544O2. Reproduced from Ref. [74] with permission from American Chemical Society. (d) Schematic diagram to show various structure defects in Li1.143Ni0.136Co0.136Mn0.544O2. (e) TEM image to show nano-defects (stacking faults and cationic mixing) in the Li1.143Ni0.136Co0.136Mn0.544O2. (f) Comparison for the average voltage of highly crystalline Li1.143Ni0.136Co0.136Mn0.544O2 cathode (Pristine-LrLO) and defect abundant sample (NDA-LrCO-5) during cycling at 0.1 C. Reproduced from Ref. [75] with permission from Elsevier. (g) Schematic diagram of the element gradient distribution in LMR cathodes. (h) SEM image of Li1.2Mn0.44Co0.04Ni0.32O2 with element gradient distribution and (i) EDS line scanning along the marked line in (h). Reproduced from Ref. [80] with permission from Elsevier. | ||||
| 6 | figure | Fig. 6 | 10 | direct_caption_ref | 0.82 | [90.49, 66.35, 410.94, 326.93] | Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100 mA g 1 . Reproduced from Ref. [84] with permission from Royal Society of Chemistry. (c) Schematic diagram of pristine LMR, LMR with surface-doped with Na (Na-LMR) and LMR with homogenously Na doping (Na/SDS-LMR) before cycling and after 200 cycles. Reproduced from Ref. [85] with permission from Wiley-VCH. (d) Schematic illustration for the structure of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . (e) The rate performance of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . Reproduced from Ref. [88] with permission from Royal Society of Chemistry. (f) Schematic diagram of Na and F co-doping in Li1.2Ni0.2Mn0.6O2 cathode. (g) The cycling performance of Li1.2Ni0.2Mn0.6O2 cathode (LNMO), Na doped LNMO cathode (Na-LNMO), F doped LNMO cathode (F-LNMO) and Na and F co-doped LNMO cathode (Na&FLNMO) at 0.1 C in the voltage range of 2.0-4.8 V. Reproduced from Ref. [95] with permission from Elsevier. | ||||
| 7 | figure | Fig. 7 | 11 | direct_caption_ref | 0.82 | [92.08, 66.42, 410.13, 377.81] | Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from Elsevier. (c) Schematic illustration of different oxygen migration model in bare and SnO2 coated Li1.2Ni0.13Co0.13Mn0.54O2 (filled with oxygen vacancies at the surface). Reproduced from Ref. [103] with permission from Elsevier. (d) Schematic diagram for the surficial structure of AlPO4 coated LMR oxide. (e) The Coulombic efficiency of the LMR oxides coated with different ALD cycles of AlPO4 during long-term cycling. Reproduced from Ref. [104] with permission from Elsevier. | ||||
| 8 | figure | Fig. 8 | 12 | direct_caption_ref | 0.82 | [89.69, 67.09, 412.07, 329.24] | Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. [107] with permission from Elsevier. (c) The cycling performance of the Li1.2Ni0.13Co0.13Mn0.54O2 cathode coated with different contents of Al2O3 and polyacene at 0.2 C (APL is short for double-shelled of Al2O3 and polyacene, and the number represents different amount of polyacene). Reproduced from Ref. [115] with permission from Royal Society of Chemistry. (d) Schematic diagram of the detailed synthetic process of the LMR cathode coated with a sandwich-like carbon@spinel@layered@spinel@carbon shell. Reproduced from Ref. [116] with permission from Elsevier. (e) Cycle performance of uncoated Li1.2Ni0.13Co0.13Mn0.54O2 (LR) and Mg2TiO4 coated Li1.2Ni0.13Co0.13Mn0.54O2 (LR@MTO) at 2 C. Reproduced from Ref. [117] with permission from John Wiley and Sons. | ||||
| 9 | figure | Fig. 9 | 13 | direct_caption_ref | 0.82 | [90.83, 67.57, 411.14, 195.32] | Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li1.2Mn0.54Ni0.13Co0.13O2 oxide in the bulk and the spinel structure at the surface after GO modification. Reproduced from Ref. [118] with permission from Royal Society of Chemistry. (c) The synthetic scheme of chemical adsorption to modified MoO2S2 at the surface of LMR cathode and the corresponding structure at each step. (d) HRTEM and the corresponding FFT and refined lattice images of the MoO2S2 modified LMR cathode. Reproduced from Ref. [119] with permission from American Chemical Society. | ||||
| 10 | figure | Fig. 10 | 13 | direct_caption_ref | 0.82 | [85.96, 338.34, 420.55, 188.83] | Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode and un-modified cathode at C/3. (c) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode after 100 cycles along [100] zone axis and the corresponding atomic models. Reproduced from Ref. [122] with permission from American Chemical Society. (d) XRD patterns of Li1.2Ni0.16Mn0.56Co0.08O2 samples doped by different Al contents. (e) The average voltage of the Li1.2Ni0.16Mn0.56Co0.08O2 cathode doped by different Al contents during cycling at 0.1 C. Reproduced from Ref. [124] with permission from John Wiley and Sons. | ||||
| 11 | figure | Fig. 11 | 14 | direct_caption_ref | 0.82 | [158.79, 460.21, 277.4, 278.72] | Fig. 11. Schematic illustration for the recent progress in improving the electrochemical performance of LMR cathodes. | ||||
| 12 | table | Table 1 | 3 | direct_caption_ref | 0.82 | [36.11, 631.06, 522.05, 122.96] | Table 1 Researches about understanding the structure of LMR oxides. | ||||
| 13 | table | Table 2 | 6 | direct_caption_ref | 0.82 | [36.35, 85.91, 521.78, 113.37] | Table 2 The electrochemical performance of LMR cathodes with different morphology design reported in recent years. | ||||
| 14 | table | Table 3 | 9 | direct_caption_ref | 0.82 | [35.97, 86.2, 522.2, 105.47] | Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. | ||||
| 15 | table | Table 3 | 9 | nearby_text_caption | 0.82 | [36.08, 231.08, 522.13, 130.31] | Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. | ||||
| 16 | table | Table 5 | 10 | direct_caption_ref | 0.82 | [36.18, 502.54, 522.02, 182.75] | Table 5 The electrochemical performance of LMR cathodes with different surface coatings reported in recent years. | ||||
| 17 | table | Table 6 | 11 | direct_caption_ref | 0.82 | [36.3, 534.89, 521.91, 96.29] | Table 6 The electrochemical performance of LMR cathodes with different surface doping and other surface treatments reported in recent years. |
| risk | page | order | label | role | reason | parser reason | production usage | trunc | body region | region | bg | bbox | raw text | cleaned text |
|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|
| high | 1 | 12 | text | unknown_text | outside_body_flow | outside_body_flow | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 310.07, 79.89, 32.02] | Article history: Received 14 October 2020 Revised 23 January 2021 Accepted 25 January 2021 | Article history: Received 14 October 2020 Revised 23 January 2021 Accepted 25 January 2021 | |||
| high | 1 | 21 | text | body_candidate_excluded | inside_front_matter | inside_front_matter | p1:body_region:0 | p1:page_body:column_2_of_2:white | [255, 255, 255] white | [389.08, 458.95, 168.57, 48.74] | Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion batteries. | Zhibo Li received his B.S. degree from South China Normal University in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion batteries. | ||
| high | 2 | 24 | text | body_candidate_excluded | inside_front_matter | inside_front_matter | p2:body_region:0 | p2:page_body:column_1_of_2:white | [255, 255, 255] white | [120.08, 66.24, 168.58, 48.79] | Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion and sodium ion batteries. | Cong Chen received his B.S. degree from South China University of Technology in 2018. He is currently a M.S. student under the supervision of Prof. Feng Pan at school of Advanced Material, Peking University. His research interests mainly focus on layered cathode material for lithium ion and sodium ion batteries. | ||
| high | 2 | 28 | text | body_candidate_excluded | inside_front_matter | inside_front_matter | p2:body_region:0 | p2:page_body:column_1_of_2:white | [255, 255, 255] white | [120.08, 582.43, 168.59, 48.79] | Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FIB, SEM and TEM. Her research interests mainly focus on the FIB and TEM characterization of battery materials. | Ni Yang is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. She has over 10 years' experience in material characterization using wide range of analytical tools including FIB, SEM and TEM. Her research interests mainly focus on the FIB and TEM characterization of battery materials. | ||
| high | 2 | 30 | text | body_candidate_excluded | inside_front_matter | inside_front_matter | p2:body_region:1 | p2:page_body:column_2_of_2:white | [255, 255, 255] white | [389.08, 66.24, 168.57, 57.35] | Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools including XRD, XPS, SEM and TEM. His research interests mainly focus on the ex/in-situ TEM and ex/in-situ XRD characterization of battery materials. | Wenguang Zhao is an engineer at School of Advanced Materials, Peking University Shenzhen Graduate School, China. He has over 10 years' experience in material characterization using wide range of analytical tools including XRD, XPS, SEM and TEM. His research interests mainly focus on the ex/in-situ TEM and ex/in-situ XRD characterization of battery materials. | ||
| high | 2 | 31 | text | body_candidate_excluded | inside_front_matter | inside_front_matter | p2:body_region:1 | p2:page_body:column_2_of_2:white | [255, 255, 255] white | [389.08, 195.27, 168.57, 48.79] | Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institute of Technology in 2006. He worked at Velocys during 2006-2011 and UES during 2011-2014. | Haibiao Chen is currently a senior researcher at School of Advanced Materials, Peking University Shenzhen Graduate School. He received his Bachelor's degree from Tsinghua University in 2000 and PhD from Stevens Institute of Technology in 2006. He worked at Velocys during 2006-2011 and UES during 2011-2014. | ||
| high | 16 | 170 | text | body_candidate_excluded | inside_back_matter | inside_back_matter | p16:front_matter:right_crossing:white | [255, 255, 255] white | [306.6, 89.67, 251.05, 49.26] | This work was financially supported by the National Key R&D Program of China (2016YFB0700600), the Soft Science Research Project of Guangdong Province (No. 2017B030301013), and the Shenzhen Science and Technology Research Grant (ZDSYS201707281026184). | This work was financially supported by the National Key R&D Program of China (2016YFB0700600), the Soft Science Research Project of Guangdong Province (No. 2017B030301013), and the Shenzhen Science and Technology Research Grant (ZDSYS201707281026184). | |||
| medium | 1 | 3 | text | unknown_text | outside_body_flow | outside_body_flow | p1:body_region:0 | p1:page_body:column_1_of_2:gray | [229, 229, 229] gray | [173.88, 135.67, 247.4, 1.59] | j o u r n a l homepage: www.elsevier.com/locate/jechem | j o u r n a l homepage: | ||
| medium | 1 | 6 | text | body_candidate_excluded | before_body_started | before_body_started | p1:body_region:0 | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 218.99, 494.97, 26.45] | Yiwei Li a,1 , Zhibo Li a,1 , Cong Chen a , Kai Yang a , Bo Cao a , Shenyang Xu a , Ni Yang a , Wenguang Zhao a , Haibiao Chen a , Mingjian Zhang a,b, ⇑ , Feng Pan a, ⇑ | Yiwei Li a,1 , Zhibo Li a,1 , Cong Chen a , Kai Yang a , Bo Cao a , Shenyang Xu a , Ni Yang a , Wenguang Zhao a , Haibiao Chen a , Mingjian Zhang a,b, ⇑ , Feng Pan a, ⇑ | ||
| medium | 1 | 8 | list_item | unknown_text | outside_body_flow_list_item | outside_body_flow_list_item | p1:page_body:column_1_of_2:white | [254, 254, 254] white | [37.64, 259.48, 2.79, 3.96] | b | b | |||
| medium | 1 | 13 | text | abstract_candidate | inside_abstract | inside_abstract | p1:body_region:0 | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [202.17, 310.46, 355.49, 93.18] | Li and Mn rich (LMR) layered oxides, written as x Li2MnO3 (1 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure and superior performance of LMR oxides make them one of the most promising candidates for the next-generation cathode materials. However, the commercialization of these materials is hindered by several drawbacks, such as low initial Coulombic efficiency, the degradation of voltage and capacity during cycling, and poor rate performance. This review summarizes research progress in solving these concerns of LMR cathodes over the past decade by following three classes of strategies: morphology design, bulk design, and surface modification. We elaborate on the processing procedures, electrochemical performance, mechanisms, and limitations of each approach, and finally put forward the concerns left and the possible solutions for the commercialization of LMR cathodes. | Li and Mn rich (LMR) layered oxides, written as x Li2MnO3 (1 x )LiMO2 (M = Mn, Ni, Co, Fe, etc.), have been widely reported in recent years due to their high capacity and high energy density. The stable structure and superior performance of LMR oxides make them one of the most promising candidates for the next-generation cathode materials. However, the commercialization of these materials is hindered by several drawbacks, such as low initial Coulombic efficiency, the degradation of voltage and capacity during cycling, and poor rate performance. This review summarizes research progress in solving these concerns of LMR cathodes over the past decade by following three classes of strategies: morphology design, bulk design, and surface modification. We elaborate on the processing procedures, electrochemical performance, mechanisms, and limitations of each approach, and finally put forward the concerns left and the possible solutions for the commercialization of LMR cathodes. | ||
| medium | 2 | 34 | text | unknown_text | inside_front_matter | inside_front_matter | p2:page_body:column_2_of_2:white | [255, 255, 255] white | [306.6, 556.17, 142.45, 5.93] | (power battery) innovation project since 2013. | (power battery) innovation project since 2013. | |||
| medium | 6 | 69 | text | unknown_text | outside_body_flow | outside_body_flow | p6:body_region:0 | p6:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 203.66, 153.66, 5.93] | Notes. [a] ICE denotes initial Coulombic efficiency. | Notes. [a] ICE denotes initial Coulombic efficiency. | ||
| medium | 16 | 173 | list_item | unknown_text | inside_back_matter | inside_back_matter | p16:front_matter:right:white | [255, 255, 255] white | [313.0, 207.06, 174.31, 5.93] | M.S. Whittingham, Proc. IEEE 100 (2012) 1518-1534. | M.S. Whittingham, Proc. IEEE 100 (2012) 1518-1534. | |||
| medium | 16 | 221 | text | body_candidate_excluded | after_back_matter_stop | after_back_matter_stop | after_stop | p16:body_region:0 | p16:bottom_margin:left_crossing:white | [255, 255, 255] white | [37.59, 726.95, 251.11, 28.34] | The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper. | The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper. | |
| low | 1 | 0 | page_header | page_header | docling_page_header | docling_page_header | p1:body_region:0 | p1:top_margin:column_1_of_2:white | [255, 255, 255] white | [224.33, 47.98, 146.57, 5.93] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 1 | 1 | text | front_matter_heading | first_page_metadata | first_page_metadata | p1:body_region:0 | p1:page_body:column_1_of_2:gray | [229, 229, 229] gray | [220.76, 79.88, 151.02, 1.59] | Contents lists available at ScienceDirect | Contents lists available at ScienceDirect | ||
| low | 1 | 2 | section_header | title_candidate | non_body_heading | non_body_heading | p1:body_region:0 | p1:page_body:column_1_of_2:gray | [229, 229, 229] gray | [201.2, 98.03, 190.03, 12.98] | Journal of Energy Chemistry | Journal of Energy Chemistry | ||
| low | 1 | 4 | section_header | title_candidate | non_body_heading | non_body_heading | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.7, 160.04, 32.05, 8.9] | Review | Review | |||
| low | 1 | 5 | section_header | title_candidate | non_body_heading | non_body_heading | p1:body_region:0 | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 179.19, 423.72, 29.75] | Recent progress in Li and Mn rich layered oxide cathodes for Li-ion batteries | Recent progress in Li and Mn rich layered oxide cathodes for Li-ion batteries | ||
| low | 1 | 7 | list_item | affiliation | outside_body_flow_list_item | outside_body_flow_list_item | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.64, 250.92, 334.71, 7.3] | a School of Advanced Materials, Peking University, Shenzhen Graduate School, Shenzhen 518055, Guangdong, China | a School of Advanced Materials, Peking University, Shenzhen Graduate School, Shenzhen 518055, Guangdong, China | |||
| low | 1 | 9 | text | affiliation | front_matter_author_line | front_matter_author_line | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [41.5, 260.41, 334.48, 6.37] | Center for Advanced Radiation Source (ChemMatCARS), the University of Chicago, Argonne, IL 60439, United States | Center for Advanced Radiation Source (ChemMatCARS), the University of Chicago, Argonne, IL 60439, United States | |||
| low | 1 | 10 | section_header | front_matter_heading | front_matter_heading | front_matter_heading | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.7, 287.39, 94.35, 11.02] | a r t i c l e i n f o | a r t i c l e i n f o | |||
| low | 1 | 11 | section_header | abstract_heading | abstract_heading | abstract_heading | p1:body_region:0 | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [202.22, 287.67, 65.22, 11.02] | a b s t r a c t | a b s t r a c t | ||
| low | 1 | 14 | text | metadata | first_page_metadata | first_page_metadata | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 344.71, 104.89, 5.93] | Available online 10 February 2021 | Available online 10 February 2021 | |||
| low | 1 | 15 | text | front_matter_heading | front_matter_heading | front_matter_heading | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 364.44, 116.82, 40.52] | Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective | Keywords: Li-ion batteries Li and Mn rich layered oxide cathodes Electrochemical concerns Progress and perspective | |||
| low | 1 | 16 | text | metadata | first_page_metadata | first_page_metadata | p1:body_region:0 | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [202.17, 404.52, 355.42, 18.23] | Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved. | Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. | ||
| low | 1 | 17 | text | reference | inside_front_matter | inside_front_matter | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [120.08, 460.31, 168.57, 57.35] | Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking University. His main research work is Li-Rich cathode materials with high voltage and high energy density for Li ion batteries. | Yiwei Li received his B.S. degree in College of Materials Science and Engineering from Huazhong University of Science and Technology in 2017. He is currently a Ph.D. candidate at School of Advanced Materials, Peking University. His main research work is Li-Rich cathode materials with high voltage and high energy density for Li ion batteries. | |||
| low | 1 | 18 | footnote | footnote | first_page_metadata | first_page_metadata | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [42.07, 692.51, 264.1, 18.63] | ⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan). | ⇑ Corresponding authors. E-mail addresses: zhangmj@pkusz.edu.cn (M. Zhang), panfeng@pkusz.edu.cn (F. Pan). | |||
| low | 1 | 19 | footnote | footnote | outside_body_flow_footnote | outside_body_flow_footnote | p1:page_body:column_1_of_2:white | [255, 255, 255] white | [43.09, 712.68, 148.31, 7.21] | 1 These authors contributed equally to this work. | 1 These authors contributed equally to this work. | |||
| low | 1 | 20 | page_footer | page_footer | first_page_metadata | first_page_metadata | p1:bottom_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 731.92, 136.91, 5.93] | https://doi.org/10.1016/j.jechem.2021.01.034 | ||||
| low | 1 | 22 | page_footer | page_footer | first_page_metadata | first_page_metadata | p1:body_region:0 | p1:bottom_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 738.73, 520.05, 8.3] | 2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved. | 2095-4956/ Ó 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. | ||
| low | 2 | 23 | text | page_margin_header | page_margin_header | page_margin_header | p2:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | |||
| low | 2 | 25 | text | reference | inside_front_matter | inside_front_matter | p2:body_region:0 | p2:page_body:column_1_of_2:white | [255, 255, 255] white | [120.08, 195.27, 168.59, 65.91] | Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. His main research interests include advanced silicon carbon materials for lithium ion batteries (LIBs) and advanced technology for interface research in LIBs, such as in-situ AFM and EQCM. | Kai Yang received his B.S. degree in the School of Aerospace from Tsinghua University in 2016, China. He is pursuing his M.S. degree at School of Advanced Materials, Peking University Shenzhen Graduate School, China. His main research interests include advanced silicon carbon materials for lithium ion batteries (LIBs) and advanced technology for interface research in LIBs, such as in-situ AFM and EQCM. | ||
| low | 2 | 26 | text | reference | inside_front_matter | inside_front_matter | p2:body_region:0 | p2:page_body:column_1_of_2:white | [255, 255, 255] white | [120.08, 324.36, 168.59, 65.91] | Bo Cao is currently a Ph.D. candidate in Prof Feng Pan's group at Peking University Shenzhen Graduate School, China. He received his B.S. degree in material science from Huazhong University of Science and Technology in 2018. Currently his research interests focus on high energy density cathode materials for lithium batteries, especially on Li-rich and Ni-rich layered oxide materials. | Bo Cao is currently a Ph.D. candidate in Prof Feng Pan's group at Peking University Shenzhen Graduate School, China. He received his B.S. degree in material science from Huazhong University of Science and Technology in 2018. Currently his research interests focus on high energy density cathode materials for lithium batteries, especially on Li-rich and Ni-rich layered oxide materials. | ||
| low | 2 | 27 | text | reference | inside_front_matter | inside_front_matter | p2:body_region:0 | p2:page_body:column_1_of_2:white | [255, 255, 255] white | [120.08, 453.39, 168.58, 48.79] | Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on development of functional materials for energy storage. | Shenyang Xu received his B.S. degree from Tiangong University in 2015. Xu is currently a Ph.D. student under the supervision of Prof. Feng Pan at School of Advanced Material, Peking University. His research interests mainly focus on development of functional materials for energy storage. | ||
| low | 2 | 29 | text | page_margin_header | page_margin_header | page_margin_header | p2:body_region:1 | p2:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.77, 47.8, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 2 | 32 | text | reference | inside_front_matter | inside_front_matter | p2:body_region:1 | p2:page_body:column_2_of_2:white | [255, 255, 255] white | [389.08, 324.36, 168.58, 100.16] | Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, he was a postdoc at School of Advanced Materials, Peking University, and became an assistant research professor since 2018. Meanwhile, he was a research scholar in Brookhaven National Lab from 2016 to 2019, then in the University of Chicago since 2019. He has been engaged in the fields of electrode materials for Liion batteries, crystal growth and structure analysis of nonlinear optical crystals. | Mingjian Zhang got his Ph.D. degree from Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences in 2013, then worked there as an assistant research fellow for one year. From 2014 to 2018, he was a postdoc at School of Advanced Materials, Peking University, and became an assistant research professor since 2018. Meanwhile, he was a research scholar in Brookhaven National Lab from 2016 to 2019, then in the University of Chicago since 2019. He has been engaged in the fields of electrode materials for Liion batteries, crystal growth and structure analysis of nonlinear optical crystals. | ||
| low | 2 | 33 | text | reference | inside_front_matter | inside_front_matter | p2:body_region:1 | p2:page_body:column_2_of_2:white | [255, 255, 255] white | [389.08, 453.39, 168.57, 100.16] | Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathclyde, Glasgow, UK, with ''Patrick D. Ritchie Prize' for the best Ph.D. in 1994. With more than a decade experience in large international incorporations, Prof. Pan has been engaged in fundamental research and product development of novel optoelectronic and energy storage materials and devices. As Chief Scientist, Prof. Pan led eight entities in Shenzhen to win 150 million RMB grant for the national new energy vehicles | Feng Pan , founding Dean of School of Advanced Materials, Peking University Shenzhen Graduate School, got B.S. from Dept. Chemistry, Peking University in 1985 and Ph.D. from Dept. of P&A Chemistry, University of Strathclyde, Glasgow, UK, with ''Patrick D. Ritchie Prize' for the best Ph.D. in 1994. With more than a decade experience in large international incorporations, Prof. Pan has been engaged in fundamental research and product development of novel optoelectronic and energy storage materials and devices. As Chief Scientist, Prof. Pan led eight entities in Shenzhen to win 150 million RMB grant for the national new energy vehicles | ||
| low | 2 | 35 | page_footer | page_footer | docling_page_footer | docling_page_footer | p2:bottom_margin:column_2_of_2:white | [254, 254, 254] white | [291.91, 764.24, 11.45, 5.93] | 369 | 369 | |||
| low | 3 | 36 | page_header | page_header | docling_page_header | docling_page_header | p3:body_region:0 | p3:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 3 | 37 | section_header | body_heading | body_heading | body_heading | p3:body_region:0 | p3:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.7, 68.75, 60.13, 7.42] | 1. Introduction | 1. Introduction | ||
| low | 3 | 39 | page_header | page_header | docling_page_header | docling_page_header | p3:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.71, 47.86, 139.91, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | |||
| low | 3 | 41 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p3:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.59, 559.63, 520.04, 32.02] | Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d synthesized from two different precursors (C for conventional precursor and H for hierarchically structured precursor). Reproduced from Ref. [27] with permission from American Chemical Society. (d) Structural scheme showing the honeycomb pattern consisting of Li@Mn6 superstructure units in LMR layered oxide. Reproduced from Ref. [29]) with permission from Royal Society of Chemistry. | Fig. 1. (a) Crystal structure of trigonal LiMO2 ( R -3m) and (b) monoclinic Li2MnO3 ( C 2/ m ). Reproduced from Ref. [27] with permission from American Chemical Society. (c) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2+ d synthesized from two different precursors (C for conventional precursor and H for hierarchically structured precursor). Reproduced from Ref. [27] with permission from American Chemical Society. (d) Structural scheme showing the honeycomb pattern consisting of Li@Mn6 superstructure units in LMR layered oxide. Reproduced from Ref. [29]) with permission from Royal Society of Chemistry. | |||
| low | 3 | 42 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p3:body_region:0 | p3:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.59, 613.15, 182.82, 14.49] | Table 1 Researches about understanding the structure of LMR oxides. | Table 1 Researches about understanding the structure of LMR oxides. | ||
| low | 3 | 43 | page_footer | page_footer | docling_page_footer | docling_page_footer | p3:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.38, 5.93] | 370 | 370 | |||
| low | 4 | 44 | page_header | page_header | docling_page_header | docling_page_header | p4:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | |||
| low | 4 | 45 | page_header | page_header | docling_page_header | docling_page_header | p4:body_region:0 | p4:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.77, 47.81, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 4 | 46 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p4:front_matter:column_1_of_2:white | [255, 255, 255] white | [37.59, 345.73, 520.08, 65.91] | Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chemical Society. (c) p DOS of O 2 p orbitals and Mn 3 d orbitals in Li2MnO3 and the corresponding oxygen environment model. Reproduced from Ref. [47] with permission from Springer Nature. (d) Cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 synthesized by two different synthesis methods at 0.1 C in the voltage range of 2.0-4.8 V. (e) The corresponding capacity-voltage profiles of the re-synthesized Li1.2Ni0.13Co0.13Mn0.54O2 in (d). Reproduced from Ref. [53] with permission from Elsevier. (f) Schematic representation for the structural transformation of trigonal LiMO2 component ( R -3m) and monoclinic Li2MnO3 component ( C 2/ m ) in Li1.2Ni0.1Mn0.525Co0.175O2 during cycling. Reproduced from Ref. [54] with permission from American Chemical Society. (g) Selected area electron diffraction (SAED) pattern obtained along [0001] zone axis of Li1.2Co0.1Mn0.55Ni0.15O2 cathode at the charging voltage of 4.5 V. (h) Schematic diagram of TM migration in Li1.2Co0.1Mn0.55Ni0.15O2 cathode when holding at 4.5 V. Reproduced from Ref. [55] with permission from Royal Society of Chemistry. | Fig. 2. (a) Initial charging-discharging profiles of Li2MnO3, LiNi0.5Mn0.5O2 and Li1.2Ni0.2Mn0.6O2. (b) The 1st and 2nd CV curves of Li1.2Ni0.2Mn0.6O2 in (a). Reproduced from Ref. [35] with permission from American Chemical Society. (c) p DOS of O 2 p orbitals and Mn 3 d orbitals in Li2MnO3 and the corresponding oxygen environment model. Reproduced from Ref. [47] with permission from Springer Nature. (d) Cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 synthesized by two different synthesis methods at 0.1 C in the voltage range of 2.0-4.8 V. (e) The corresponding capacity-voltage profiles of the re-synthesized Li1.2Ni0.13Co0.13Mn0.54O2 in (d). Reproduced from Ref. [53] with permission from Elsevier. (f) Schematic representation for the structural transformation of trigonal LiMO2 component ( R -3m) and monoclinic Li2MnO3 component ( C 2/ m ) in Li1.2Ni0.1Mn0.525Co0.175O2 during cycling. Reproduced from Ref. [54] with permission from American Chemical Society. (g) Selected area electron diffraction (SAED) pattern obtained along [0001] zone axis of Li1.2Co0.1Mn0.55Ni0.15O2 cathode at the charging voltage of 4.5 V. (h) Schematic diagram of TM migration in Li1.2Co0.1Mn0.55Ni0.15O2 cathode when holding at 4.5 V. Reproduced from Ref. [55] with permission from Royal Society of Chemistry. | |||
| low | 4 | 49 | section_header | body_heading | body_heading | body_heading | p4:body_region:0 | p4:body_zone:column_2_of_2:white | [255, 255, 255] white | [306.65, 445.24, 248.85, 7.42] | 2. Structure and electrochemical performance of LMR cathode | 2. Structure and electrochemical performance of LMR cathode | ||
| low | 4 | 50 | section_header | body_heading | body_heading | body_heading | p4:body_region:0 | p4:body_zone:column_2_of_2:white | [255, 255, 255] white | [306.65, 465.73, 128.59, 7.96] | 2.1. Crystal structure of LMR oxides | 2.1. Crystal structure of LMR oxides | ||
| low | 4 | 53 | page_footer | page_footer | docling_page_footer | docling_page_footer | p4:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 371 | 371 | |||
| low | 5 | 54 | page_header | page_header | docling_page_header | docling_page_header | p5:body_region:0 | p5:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 5 | 59 | section_header | body_heading | body_heading | body_heading | p5:body_region:0 | p5:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.7, 402.24, 182.07, 7.96] | 2.2. Electrochemical performance of LMR cathodes | 2.2. Electrochemical performance of LMR cathodes | ||
| low | 5 | 62 | page_header | page_header | docling_page_header | docling_page_header | p5:body_region:1 | p5:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.71, 47.86, 139.91, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 5 | 66 | page_footer | page_footer | docling_page_footer | docling_page_footer | p5:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 372 | 372 | |||
| low | 6 | 67 | page_header | page_header | docling_page_header | docling_page_header | p6:body_region:0 | p6:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 6 | 68 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p6:body_region:0 | p6:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 67.94, 328.37, 14.49] | Table 2 The electrochemical performance of LMR cathodes with different morphology design reported in recent years. | Table 2 The electrochemical performance of LMR cathodes with different morphology design reported in recent years. | ||
| low | 6 | 70 | page_header | page_header | docling_page_header | docling_page_header | p6:body_region:1 | p6:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.77, 47.8, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 6 | 71 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p6:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 567.06, 520.06, 40.18] | Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3 (1x )LiMnO2 nanorods. Reproduced from Ref. [63] with permission from Elsevier. (c) Schematic illustration of the synthetic process of orthogonally arranged nanoplates. Reproduced from Ref. [64] with permission from American Chemical Society. (d) Scheme of the fabrication process of 3D hollow porous bowl-shaped Li1.2Ni0.13Co0.13Mn0.54O2 particles. Reproduced from Ref. [66] with permission from Elsevier. (e) Schematic diagram of the suppression of voltage fading through a preferred orientation (110) plane. Reproduced from Ref. [67] with permission from Royal Society of Chemistry. | Fig. 3. (a) Schematic illustration of the synthetic process of Li1.2Ni0.13Co0.13Mn0.54O2 nanowires. Reproduced from Ref. [62] with permission from Elsevier. (b) Scanning electron microscope (SEM) image of x Li2MnO3 (1x )LiMnO2 nanorods. Reproduced from Ref. [63] with permission from Elsevier. (c) Schematic illustration of the synthetic process of orthogonally arranged nanoplates. Reproduced from Ref. [64] with permission from American Chemical Society. (d) Scheme of the fabrication process of 3D hollow porous bowl-shaped Li1.2Ni0.13Co0.13Mn0.54O2 particles. Reproduced from Ref. [66] with permission from Elsevier. (e) Schematic diagram of the suppression of voltage fading through a preferred orientation (110) plane. Reproduced from Ref. [67] with permission from Royal Society of Chemistry. | |||
| low | 6 | 74 | page_footer | page_footer | docling_page_footer | docling_page_footer | p6:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 373 | 373 | |||
| low | 7 | 75 | page_header | page_header | docling_page_header | docling_page_header | p7:top_margin:left:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | |||
| low | 7 | 76 | page_header | page_header | docling_page_header | docling_page_header | p7:top_margin:right:white | [255, 255, 255] white | [417.71, 47.86, 139.91, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | |||
| low | 7 | 77 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p7:page_body:full:white | [255, 255, 255] white | [37.59, 336.66, 520.03, 23.72] | Fig. 4. (a) Schematic illustration of the formation of porous Li1.2Ni0.18Co0.08Mn0.54O2. Reproduced from Ref. [68] with permission from Royal Society of Chemistry. (b) Schematic illustration of the synthesizing route for 3D Li1.2Ni0.2Mn0.6O2 and the morphological evolution. Reproduced from Ref. [69] with permission from American Chemical Society. (c) SEM image of Li1.2Ni0.2Mn0.6O2 oxide. Reproduced from Ref. [70] with permission from American Chemical Society. | Fig. 4. (a) Schematic illustration of the formation of porous Li1.2Ni0.18Co0.08Mn0.54O2. Reproduced from Ref. [68] with permission from Royal Society of Chemistry. (b) Schematic illustration of the synthesizing route for 3D Li1.2Ni0.2Mn0.6O2 and the morphological evolution. Reproduced from Ref. [69] with permission from American Chemical Society. (c) SEM image of Li1.2Ni0.2Mn0.6O2 oxide. Reproduced from Ref. [70] with permission from American Chemical Society. | |||
| low | 7 | 78 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p7:page_body:full:white | [255, 255, 255] white | [37.59, 667.98, 520.07, 57.96] | Fig. 5. (a) Schematic illustration of ice-template coprecipitation method to synthesize Li1.2Ni0.2Mn0.6O2 with hierarchical mesopore structure. (b) The rate performance of Li1.2Ni0.2Mn0.6O2 synthesized by freeze drying (M1) and vacuum drying (M2). Reproduced from Ref. [73] with permission from American Chemical Society. (c) Schematic diagram of building nano-porous structures in Li1.144Ni0.136Co0.136Mn0.544O2. Reproduced from Ref. [74] with permission from American Chemical Society. (d) Schematic diagram to show various structure defects in Li1.143Ni0.136Co0.136Mn0.544O2. (e) TEM image to show nano-defects (stacking faults and cationic mixing) in the Li1.143Ni0.136Co0.136Mn0.544O2. (f) Comparison for the average voltage of highly crystalline Li1.143Ni0.136Co0.136Mn0.544O2 cathode (Pristine-LrLO) and defect abundant sample (NDA-LrCO-5) during cycling at 0.1 C. Reproduced from Ref. [75] with permission from Elsevier. (g) Schematic diagram of the element gradient distribution in LMR cathodes. (h) SEM image of Li1.2Mn0.44Co0.04Ni0.32O2 with element gradient distribution and (i) EDS line scanning along the marked line in (h). Reproduced from Ref. [80] with permission from Elsevier. | Fig. 5. (a) Schematic illustration of ice-template coprecipitation method to synthesize Li1.2Ni0.2Mn0.6O2 with hierarchical mesopore structure. (b) The rate performance of Li1.2Ni0.2Mn0.6O2 synthesized by freeze drying (M1) and vacuum drying (M2). Reproduced from Ref. [73] with permission from American Chemical Society. (c) Schematic diagram of building nano-porous structures in Li1.144Ni0.136Co0.136Mn0.544O2. Reproduced from Ref. [74] with permission from American Chemical Society. (d) Schematic diagram to show various structure defects in Li1.143Ni0.136Co0.136Mn0.544O2. (e) TEM image to show nano-defects (stacking faults and cationic mixing) in the Li1.143Ni0.136Co0.136Mn0.544O2. (f) Comparison for the average voltage of highly crystalline Li1.143Ni0.136Co0.136Mn0.544O2 cathode (Pristine-LrLO) and defect abundant sample (NDA-LrCO-5) during cycling at 0.1 C. Reproduced from Ref. [75] with permission from Elsevier. (g) Schematic diagram of the element gradient distribution in LMR cathodes. (h) SEM image of Li1.2Mn0.44Co0.04Ni0.32O2 with element gradient distribution and (i) EDS line scanning along the marked line in (h). Reproduced from Ref. [80] with permission from Elsevier. | |||
| low | 7 | 79 | page_footer | page_footer | docling_page_footer | docling_page_footer | p7:bottom_margin:left_crossing:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 374 | 374 | |||
| low | 8 | 80 | page_header | page_header | docling_page_header | docling_page_header | p8:body_region:0 | p8:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 8 | 83 | section_header | body_heading | body_heading | body_heading | p8:body_region:0 | p8:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.59, 272.79, 212.3, 17.91] | 3. Recent progress on promoting the electrochemical performance of LMR cathodes | 3. Recent progress on promoting the electrochemical performance of LMR cathodes | ||
| low | 8 | 85 | section_header | body_heading | body_heading | body_heading | p8:body_region:0 | p8:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.7, 391.81, 84.2, 7.96] | 3.1. Morphology design | 3.1. Morphology design | ||
| low | 8 | 88 | page_header | page_header | docling_page_header | docling_page_header | p8:body_region:1 | p8:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.77, 47.81, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 8 | 93 | page_footer | page_footer | docling_page_footer | docling_page_footer | p8:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 375 | 375 | |||
| low | 9 | 94 | section_header | body_heading | body_heading | body_heading | p9:body_region:0 | p9:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 9 | 95 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p9:body_region:0 | p9:front_matter:column_1_of_2:white | [255, 255, 255] white | [37.59, 67.94, 322.38, 14.49] | Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. | Table 3 The electrochemical performance of LMR cathodes with different structure designs reported in recent years. | ||
| low | 9 | 99 | section_header | body_heading | body_heading | body_heading | p9:body_region:0 | p9:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.7, 485.35, 56.76, 7.96] | 3.2. Bulk design | 3.2. Bulk design | ||
| low | 9 | 101 | section_header | body_heading | body_heading | body_heading | p9:body_region:0 | p9:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.7, 548.68, 80.52, 7.96] | 3.2.1. Structure design | 3.2.1. Structure design | ||
| low | 9 | 104 | page_header | page_header | docling_page_header | docling_page_header | p9:body_region:1 | p9:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.71, 47.86, 139.91, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 9 | 107 | page_footer | page_footer | docling_page_footer | docling_page_footer | p9:body_region:0 | p9:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 376 | 376 | ||
| low | 10 | 108 | page_header | page_header | docling_page_header | docling_page_header | p10:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | |||
| low | 10 | 109 | page_header | page_header | docling_page_header | docling_page_header | p10:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.77, 47.8, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | |||
| low | 10 | 110 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p10:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 405.2, 520.07, 57.35] | Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100 mA g 1 . Reproduced from Ref. [84] with permission from Royal Society of Chemistry. (c) Schematic diagram of pristine LMR, LMR with surface-doped with Na (Na-LMR) and LMR with homogenously Na doping (Na/SDS-LMR) before cycling and after 200 cycles. Reproduced from Ref. [85] with permission from Wiley-VCH. (d) Schematic illustration for the structure of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . (e) The rate performance of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . Reproduced from Ref. [88] with permission from Royal Society of Chemistry. (f) Schematic diagram of Na and F co-doping in Li1.2Ni0.2Mn0.6O2 cathode. (g) The cycling performance of Li1.2Ni0.2Mn0.6O2 cathode (LNMO), Na doped LNMO cathode (Na-LNMO), F doped LNMO cathode (F-LNMO) and Na and F co-doped LNMO cathode (Na&FLNMO) at 0.1 C in the voltage range of 2.0-4.8 V. Reproduced from Ref. [95] with permission from Elsevier. | Fig. 6. (a) XRD patterns of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2. (b) The cycling performance of Li1.2Ni0.13Co0.13Mn0.54O2 and Li1.17Na0.03[Ni0.13Co0.13Mn0.54]O2 at the current density of 100 mA g 1 . Reproduced from Ref. [84] with permission from Royal Society of Chemistry. (c) Schematic diagram of pristine LMR, LMR with surface-doped with Na (Na-LMR) and LMR with homogenously Na doping (Na/SDS-LMR) before cycling and after 200 cycles. Reproduced from Ref. [85] with permission from Wiley-VCH. (d) Schematic illustration for the structure of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . (e) The rate performance of Mg-doped Li1.4Mg0.1[Mn0.75Ni0.25]O2+ r . Reproduced from Ref. [88] with permission from Royal Society of Chemistry. (f) Schematic diagram of Na and F co-doping in Li1.2Ni0.2Mn0.6O2 cathode. (g) The cycling performance of Li1.2Ni0.2Mn0.6O2 cathode (LNMO), Na doped LNMO cathode (Na-LNMO), F doped LNMO cathode (F-LNMO) and Na and F co-doped LNMO cathode (Na&FLNMO) at 0.1 C in the voltage range of 2.0-4.8 V. Reproduced from Ref. [95] with permission from Elsevier. | |||
| low | 10 | 111 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p10:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 484.4, 318.95, 14.55] | Table 5 The electrochemical performance of LMR cathodes with different surface coatings reported in recent years. | Table 5 The electrochemical performance of LMR cathodes with different surface coatings reported in recent years. | |||
| low | 10 | 114 | page_footer | page_footer | docling_page_footer | docling_page_footer | p10:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 377 | 377 | |||
| low | 11 | 115 | page_header | page_header | docling_page_header | docling_page_header | p11:body_region:0 | p11:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 11 | 116 | page_header | page_header | docling_page_header | docling_page_header | p11:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.71, 47.86, 139.91, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | |||
| low | 11 | 117 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p11:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 454.36, 520.06, 40.18] | Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from Elsevier. (c) Schematic illustration of different oxygen migration model in bare and SnO2 coated Li1.2Ni0.13Co0.13Mn0.54O2 (filled with oxygen vacancies at the surface). Reproduced from Ref. [103] with permission from Elsevier. (d) Schematic diagram for the surficial structure of AlPO4 coated LMR oxide. (e) The Coulombic efficiency of the LMR oxides coated with different ALD cycles of AlPO4 during long-term cycling. Reproduced from Ref. [104] with permission from Elsevier. | Fig. 7. (a) Schematic diagram of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2. (b) The capacity-voltage profiles of Al2O3 coated Li1.2Ni0.20Co0.08Mn0.52O2 in different cycles. Reproduced from Ref. [102] with permission from Elsevier. (c) Schematic illustration of different oxygen migration model in bare and SnO2 coated Li1.2Ni0.13Co0.13Mn0.54O2 (filled with oxygen vacancies at the surface). Reproduced from Ref. [103] with permission from Elsevier. (d) Schematic diagram for the surficial structure of AlPO4 coated LMR oxide. (e) The Coulombic efficiency of the LMR oxides coated with different ALD cycles of AlPO4 during long-term cycling. Reproduced from Ref. [104] with permission from Elsevier. | |||
| low | 11 | 118 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p11:body_region:0 | p11:page_body:column_1_of_2:white | [255, 255, 255] white | [37.59, 516.32, 403.6, 14.49] | Table 6 The electrochemical performance of LMR cathodes with different surface doping and other surface treatments reported in recent years. | Table 6 The electrochemical performance of LMR cathodes with different surface doping and other surface treatments reported in recent years. | ||
| low | 11 | 122 | page_footer | page_footer | docling_page_footer | docling_page_footer | p11:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 378 | 378 | |||
| low | 12 | 123 | page_header | page_header | docling_page_header | docling_page_header | p12:body_region:0 | p12:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 12 | 124 | page_header | page_header | docling_page_header | docling_page_header | p12:body_region:1 | p12:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.77, 47.81, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 12 | 125 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p12:front_matter:column_1_of_2:white | [255, 255, 255] white | [37.59, 408.83, 520.06, 49.4] | Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. [107] with permission from Elsevier. (c) The cycling performance of the Li1.2Ni0.13Co0.13Mn0.54O2 cathode coated with different contents of Al2O3 and polyacene at 0.2 C (APL is short for double-shelled of Al2O3 and polyacene, and the number represents different amount of polyacene). Reproduced from Ref. [115] with permission from Royal Society of Chemistry. (d) Schematic diagram of the detailed synthetic process of the LMR cathode coated with a sandwich-like carbon@spinel@layered@spinel@carbon shell. Reproduced from Ref. [116] with permission from Elsevier. (e) Cycle performance of uncoated Li1.2Ni0.13Co0.13Mn0.54O2 (LR) and Mg2TiO4 coated Li1.2Ni0.13Co0.13Mn0.54O2 (LR@MTO) at 2 C. Reproduced from Ref. [117] with permission from John Wiley and Sons. | Fig. 8. (a) Illustration of the Li3PO4 coating process at the surface of Li1.2Ni0.2Mn0.6O2 through annealing at different temperatures. (b) TEM image of Li3PO4 coating layer. Reproduced from Ref. [107] with permission from Elsevier. (c) The cycling performance of the Li1.2Ni0.13Co0.13Mn0.54O2 cathode coated with different contents of Al2O3 and polyacene at 0.2 C (APL is short for double-shelled of Al2O3 and polyacene, and the number represents different amount of polyacene). Reproduced from Ref. [115] with permission from Royal Society of Chemistry. (d) Schematic diagram of the detailed synthetic process of the LMR cathode coated with a sandwich-like carbon@spinel@layered@spinel@carbon shell. Reproduced from Ref. [116] with permission from Elsevier. (e) Cycle performance of uncoated Li1.2Ni0.13Co0.13Mn0.54O2 (LR) and Mg2TiO4 coated Li1.2Ni0.13Co0.13Mn0.54O2 (LR@MTO) at 2 C. Reproduced from Ref. [117] with permission from John Wiley and Sons. | |||
| low | 12 | 127 | section_header | body_heading | body_heading | body_heading | p12:body_region:0 | p12:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.7, 527.76, 64.79, 7.96] | 3.2.2. Bulk doping | 3.2.2. Bulk doping | ||
| low | 12 | 132 | page_footer | page_footer | docling_page_footer | docling_page_footer | p12:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 379 | 379 | |||
| low | 13 | 133 | page_header | page_header | docling_page_header | docling_page_header | p13:body_region:0 | p13:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 13 | 134 | page_header | page_header | docling_page_header | docling_page_header | p13:body_region:1 | p13:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.71, 47.86, 139.91, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 13 | 135 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p13:front_matter:column_1_of_2:white | [255, 255, 255] white | [37.59, 273.34, 520.06, 40.18] | Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li1.2Mn0.54Ni0.13Co0.13O2 oxide in the bulk and the spinel structure at the surface after GO modification. Reproduced from Ref. [118] with permission from Royal Society of Chemistry. (c) The synthetic scheme of chemical adsorption to modified MoO2S2 at the surface of LMR cathode and the corresponding structure at each step. (d) HRTEM and the corresponding FFT and refined lattice images of the MoO2S2 modified LMR cathode. Reproduced from Ref. [119] with permission from American Chemical Society. | Fig. 9. (a) Schematic illustration of the detailed process of GO modified at the surface of Li1.2Ni0.13Co0.13Mn0.54O2 cathode and the following heat treatment. (b) HRTEM image and the corresponding FFT of the layered Li1.2Mn0.54Ni0.13Co0.13O2 oxide in the bulk and the spinel structure at the surface after GO modification. Reproduced from Ref. [118] with permission from Royal Society of Chemistry. (c) The synthetic scheme of chemical adsorption to modified MoO2S2 at the surface of LMR cathode and the corresponding structure at each step. (d) HRTEM and the corresponding FFT and refined lattice images of the MoO2S2 modified LMR cathode. Reproduced from Ref. [119] with permission from American Chemical Society. | |||
| low | 13 | 136 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p13:front_matter:column_1_of_2:white | [255, 255, 255] white | [37.59, 537.3, 520.07, 40.23] | Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode and un-modified cathode at C/3. (c) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode after 100 cycles along [100] zone axis and the corresponding atomic models. Reproduced from Ref. [122] with permission from American Chemical Society. (d) XRD patterns of Li1.2Ni0.16Mn0.56Co0.08O2 samples doped by different Al contents. (e) The average voltage of the Li1.2Ni0.16Mn0.56Co0.08O2 cathode doped by different Al contents during cycling at 0.1 C. Reproduced from Ref. [124] with permission from John Wiley and Sons. | Fig. 10. (a) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode along [100] zone axis and the corresponding atomic models. (b) The cycling performance of Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode and un-modified cathode at C/3. (c) HAADF-STEM image of the Zr-modified Li1.2Ni0.13Co0.13Mn0.54O2 cathode after 100 cycles along [100] zone axis and the corresponding atomic models. Reproduced from Ref. [122] with permission from American Chemical Society. (d) XRD patterns of Li1.2Ni0.16Mn0.56Co0.08O2 samples doped by different Al contents. (e) The average voltage of the Li1.2Ni0.16Mn0.56Co0.08O2 cathode doped by different Al contents during cycling at 0.1 C. Reproduced from Ref. [124] with permission from John Wiley and Sons. | |||
| low | 13 | 139 | section_header | body_heading | body_heading | body_heading | p13:body_region:1 | p13:body_zone:column_2_of_2:white | [255, 255, 255] white | [306.65, 642.84, 89.45, 7.96] | 3.3. Surface modification | 3.3. Surface modification | ||
| low | 13 | 141 | section_header | body_heading | body_heading | body_heading | p13:body_region:1 | p13:body_zone:column_2_of_2:white | [255, 255, 255] white | [306.65, 705.6, 77.14, 7.96] | 3.3.1. Surface coating | 3.3.1. Surface coating | ||
| low | 13 | 143 | page_footer | page_footer | docling_page_footer | docling_page_footer | p13:bottom_margin:column_2_of_2:white | [253, 253, 253] white | [291.91, 764.24, 11.38, 5.93] | 380 | 380 | |||
| low | 14 | 144 | page_header | page_header | docling_page_header | docling_page_header | p14:body_region:0 | p14:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 14 | 148 | caption | caption | outside_body_flow_caption | outside_body_flow_caption | p14:bottom_margin:column_1_of_2:white | [255, 255, 255] white | [116.73, 749.05, 361.77, 5.93] | Fig. 11. Schematic illustration for the recent progress in improving the electrochemical performance of LMR cathodes. | Fig. 11. Schematic illustration for the recent progress in improving the electrochemical performance of LMR cathodes. | |||
| low | 14 | 149 | page_header | page_header | docling_page_header | docling_page_header | p14:body_region:1 | p14:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.77, 47.8, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 14 | 152 | page_footer | page_footer | docling_page_footer | docling_page_footer | p14:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 381 | 381 | |||
| low | 15 | 153 | page_header | page_header | docling_page_header | docling_page_header | p15:body_region:0 | p15:top_margin:column_1_of_2:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 15 | 157 | section_header | body_heading | body_heading | body_heading | p15:body_region:0 | p15:body_zone:column_1_of_2:white | [255, 255, 255] white | [37.7, 708.95, 75.28, 7.96] | 3.3.2. Surface doping | 3.3.2. Surface doping | ||
| low | 15 | 159 | page_header | page_header | docling_page_header | docling_page_header | p15:body_region:1 | p15:top_margin:column_2_of_2:white | [255, 255, 255] white | [417.71, 47.86, 139.91, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | ||
| low | 15 | 162 | section_header | body_heading | body_heading | body_heading | p15:body_region:1 | p15:body_zone:column_2_of_2:white | [255, 255, 255] white | [306.65, 510.24, 112.01, 7.96] | 3.3.3. Other surface treatments | 3.3.3. Other surface treatments | ||
| low | 15 | 165 | page_footer | page_footer | docling_page_footer | docling_page_footer | p15:bottom_margin:column_2_of_2:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 382 | 382 | |||
| low | 16 | 166 | page_header | page_header | docling_page_header | docling_page_header | p16:body_region:0 | p16:top_margin:left:white | [255, 255, 255] white | [37.59, 47.86, 69.84, 6.37] | Y. Li, Z. Li, C. Chen et al. | Y. Li, Z. Li, C. Chen et al. | ||
| low | 16 | 167 | page_header | page_header | docling_page_header | docling_page_header | p16:top_margin:right:white | [255, 255, 255] white | [417.77, 47.8, 139.86, 6.37] | Journal of Energy Chemistry 61 (2021) 368-385 | Journal of Energy Chemistry 61 (2021) 368-385 | |||
| low | 16 | 169 | section_header | back_matter_heading | early_back_matter_heading | early_back_matter_heading | p16:front_matter:right_crossing:white | [255, 255, 255] white | [306.6, 68.75, 73.61, 7.42] | Acknowledgments | Acknowledgments | |||
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| low | 18 | 317 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:left_crossing:white | [255, 255, 255] white | [37.64, 83.87, 250.98, 13.93] | H. Zheng, Z. Hu, P. Liu, W. Xu, Q. Xie, W. He, Q. Luo, L. Wang, D. Gu, B. Qu, Z.-Z. Zhu, D.-L. Peng, Energy Storage Mater. 25 (2020) 76-85. | H. Zheng, Z. Hu, P. Liu, W. Xu, Q. Xie, W. He, Q. Luo, L. Wang, D. Gu, B. Qu, Z.-Z. Zhu, D.-L. Peng, Energy Storage Mater. 25 (2020) 76-85. | ||
| low | 18 | 318 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:right_crossing:white | [255, 255, 255] white | [306.65, 67.94, 202.54, 5.93] | P. Hou, G. Li, X. Gao, J. Mater. Chem. A 4 (2016) 7689-7699. | P. Hou, G. Li, X. Gao, J. Mater. Chem. A 4 (2016) 7689-7699. | ||
| low | 18 | 319 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:right_crossing:white | [255, 255, 255] white | [306.65, 75.93, 250.98, 21.86] | E.M. Erickson, H. Sclar, F. Schipper, J. Liu, R. Tian, C. Ghanty, L. Burstein, N. Leifer, J. Grinblat, M. Talianker, J.-Y. Shin, J.K. Lampert, B. Markovsky, A.I. Frenkel, D. Aurbach, Adv. Energy Mater. 7 (2017) 1700708. | E.M. Erickson, H. Sclar, F. Schipper, J. Liu, R. Tian, C. Ghanty, L. Burstein, N. Leifer, J. Grinblat, M. Talianker, J.-Y. Shin, J.K. Lampert, B. Markovsky, A.I. Frenkel, D. Aurbach, Adv. Energy Mater. 7 (2017) 1700708. | ||
| low | 18 | 320 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:left_crossing:white | [255, 255, 255] white | [37.64, 99.8, 250.98, 13.93] | N. Zhang, J. Stark, H. Li, A. Liu, Y. Li, I. Hamam, J.R. Dahn, J. Electrochem. Soc. 167 (2020) 080518. | N. Zhang, J. Stark, H. Li, A. Liu, Y. Li, I. Hamam, J.R. Dahn, J. Electrochem. Soc. 167 (2020) 080518. | ||
| low | 18 | 321 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:right_crossing:white | [255, 255, 255] white | [306.65, 99.8, 251.01, 13.93] | H.Z. Zhang, Q.Q. Qiao, G.R. Li, S.H. Ye, X.P. Gao, J. Mater. Chem. 22 (2012) 13104-13109. | H.Z. Zhang, Q.Q. Qiao, G.R. Li, S.H. Ye, X.P. Gao, J. Mater. Chem. 22 (2012) 13104-13109. | ||
| low | 18 | 322 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:left_crossing:white | [255, 255, 255] white | [37.64, 115.79, 251.02, 13.87] | C.M. Subramaniyam, H. Celio, K. Shiva, H.C. Gao, J.B. Goodneough, H.K. Liu, S. X. Dou, Sustain. Energy Fuels 1 (2017) 1292-1298. | C.M. Subramaniyam, H. Celio, K. Shiva, H.C. Gao, J.B. Goodneough, H.K. Liu, S. X. Dou, Sustain. Energy Fuels 1 (2017) 1292-1298. | ||
| low | 18 | 323 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:right_crossing:white | [255, 255, 255] white | [306.65, 115.79, 250.99, 13.87] | X. Zheng, X. Wang, X. Cai, L. Xing, M. Xu, Y. Liao, X. Li, W. Li, ACS Appl. Mater. Interfaces 8 (2016) 30116-30125. | X. Zheng, X. Wang, X. Cai, L. Xing, M. Xu, Y. Liao, X. Li, W. Li, ACS Appl. Mater. Interfaces 8 (2016) 30116-30125. | ||
| low | 18 | 324 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:left_crossing:white | [255, 255, 255] white | [37.65, 131.72, 251.0, 13.87] | D. Luo, X. Ding, J. Fan, Z. Zhang, P. Liu, X. Yang, J. Guo, S. Sun, Z. Lin, Angew. Chem. Int. Ed. 59 (2020) 23061-23066. | D. Luo, X. Ding, J. Fan, Z. Zhang, P. Liu, X. Yang, J. Guo, S. Sun, Z. Lin, Angew. Chem. Int. Ed. 59 (2020) 23061-23066. | ||
| low | 18 | 325 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:right_crossing:white | [255, 255, 255] white | [306.65, 131.72, 250.97, 13.87] | S. Tan, Z. Zhang, Y. Li, Y. Li, J. Zheng, Z. Zhou, Y. Yang, J. Electrochem. Soc. 160 (2012) A285-A292. | S. Tan, Z. Zhang, Y. Li, Y. Li, J. Zheng, Z. Zhou, Y. Yang, J. Electrochem. Soc. 160 (2012) A285-A292. | ||
| low | 18 | 326 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:left_crossing:white | [255, 255, 255] white | [37.64, 179.51, 251.01, 5.93] | H.Z. Zhang, Q.Q. Qiao, G.R. Li, X.P. Gao, J. Mater. Chem. A 2 (2014) 7454-7460. | H.Z. Zhang, Q.Q. Qiao, G.R. Li, X.P. Gao, J. Mater. Chem. A 2 (2014) 7454-7460. | ||
| low | 18 | 327 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:left:white | [255, 255, 255] white | [37.64, 147.65, 214.9, 5.93] | J. Zheng, X. Wu, Y. Yang, Electrochim. Acta 105 (2013) 200-208. | J. Zheng, X. Wu, Y. Yang, Electrochim. Acta 105 (2013) 200-208. | ||
| low | 18 | 328 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:left_crossing:white | [255, 255, 255] white | [37.64, 155.64, 251.0, 21.86] | U. Breddemann, E.M. Erickson, V. Davis, F. Schipper, M. Ellwanger, M. Daub, A. Hoffmann, C. Erk, B. Markovsky, D. Aurbach, I. Krossing, Chemelectrochem 6 (2019) 3337-3349. | U. Breddemann, E.M. Erickson, V. Davis, F. Schipper, M. Ellwanger, M. Daub, A. Hoffmann, C. Erk, B. Markovsky, D. Aurbach, I. Krossing, Chemelectrochem 6 (2019) 3337-3349. | ||
| low | 18 | 329 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:right_crossing:white | [255, 255, 255] white | [306.65, 147.65, 250.98, 13.93] | H. Li, J. Li, N. Zaker, N. Zhang, G.A. Botton, J.R. Dahn, J. Electrochem. Soc. 166 (2019) A1956-A1963. | H. Li, J. Li, N. Zaker, N. Zhang, G.A. Botton, J.R. Dahn, J. Electrochem. Soc. 166 (2019) A1956-A1963. | ||
| low | 18 | 330 | list_item | reference | after_back_matter_stop | after_back_matter_stop | after_stop | p18:page_body:right_crossing:white | [255, 255, 255] white | [306.65, 163.58, 250.99, 21.86] | S. Nakamura, A. Maljuk, Y. Maruyama, M. Nagao, S. Watauchi, T. Hayashi, Y. Anzai, Y. Furukawa, C.D. Ling, G. Deng, M. Aydeev, B. Buechner, I. Tanaka, Cryst. Growth Des. 19 (2019) 415-420. | S. Nakamura, A. Maljuk, Y. Maruyama, M. Nagao, S. Watauchi, T. Hayashi, Y. Anzai, Y. Furukawa, C.D. Ling, G. Deng, M. Aydeev, B. Buechner, I. Tanaka, Cryst. Growth Des. 19 (2019) 415-420. | ||
| low | 18 | 331 | page_footer | page_footer | after_back_matter_stop | after_back_matter_stop | after_stop | p18:bottom_margin:right_crossing:white | [255, 255, 255] white | [291.91, 764.24, 11.45, 5.93] | 385 | 385 |