Excluded Docling blocks

这里是差集:Docling 全量解析 text block 减去最终会进入正文的 block。优先人工检查 risk=high / medium。

layout_review.html excluded_blocks.json excluded_blocks.tsv final_body_blocks.tsv visual_assets.tsv original.pdf

Diff Summary

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Truncation

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Excluded Page Overlays

这些框显示被排除块,同时叠加真实图表资产框。青色虚线表示该 text block 被图表资产 caption 吸收;红色 STOP 是截断触发点,红色框是截断后被排除的块。

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Visual Assets

这是实际图表资产输出,不是审计层重新推断。

#typelabelpagecaption sourcesuppressedduplicate reasonrescue reasongroupconfidencebboxcaption
1figureDocling Figure 12missing_caption0.55[11.0, 134.54, 227.6, 76.07]
2figureDocling Figure 23missing_caption0.55[263.44, 56.87, 224.54, 159.46]
3figureDocling Figure 34missing_caption0.55[10.93, 229.51, 228.07, 102.35]
4figureDocling Figure 44missing_caption0.55[276.07, 324.95, 201.04, 184.75]
5figureDocling Figure 55missing_caption0.55[262.05, 60.76, 228.59, 136.38]
6figureDocling Figure 66missing_caption0.55[11.13, 351.37, 227.76, 249.05]
7figureDocling Figure 78missing_caption0.55[37.88, 101.21, 172.68, 158.9]
8tableDocling Table 89missing_caption0.55[9.42, 539.2, 483.14, 193.82]

Excluded Blocks

riskpageorderlabelrolereasonparser reasonproduction usage truncbody regionregionbgbboxraw textcleaned text
high112textbody_candidate_excludedempty_after_cleaningempty_after_cleaning
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[9.94, 390.9, 481.81, 28.48]( The Key Laboratory of Fuel Cells Technology of Guangdong Province ꎬ School of Chemistry and Chemical Engineering ꎬ South China University of Technology ꎬ Guangzhou 510641ꎬ China )
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[9.94, 437.38, 481.99, 187.13]Abstract Lithium ̄rich manganese ̄based layered cathode materials ( x Li 2 MnO 3􀅰(1- x ) LiMO 2 ꎬ M = Ni ꎬ Co ꎬ Mn ꎬ etc. )ꎬ owing to their high specific capacity (≥ 250 mAh 􀅰 g -1 )ꎬ low cost and environmental friendliness ꎬ are considered as one of the best candidate cathode materials for the new generation of lithium ̄ion batteries. However ꎬ these materials suffer from severe capacity / voltage fading during the cycle process and low rate capability which seriously hinder commercial development. In this paper ꎬ we analyze the structural characteristics and the reasons which lead to the deterioration of the electrochemical performance of the lithium ̄rich manganese ̄ based layered cathode materials ꎬ systematically review the latest progress and achievements on improving the stability of the cathode materials ꎬ and the efforts to improve the electrochemical properties of the cathode materials through bulk doping and surface modification. In this process ꎬ the effects of bulk doping at different sites and different coating materials on the structure and electrochemical behavior of lithium ̄rich manganese ̄based layered cathode materials are further analyzed. Finally ꎬ considering the advantages and disadvantages of the two modification methods of bulk doping and surface coating ꎬ a joint modification mechanism combining bulk doping
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[9.94, 56.22, 481.77, 28.48]and surface coating has been suggested to improve the stability of lithium ̄rich cathode materials in the long cycle process ꎬ and the introduction and prospect of this mechanism are also given.
high223textunknown_textempty_after_cleaningempty_after_cleaning
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[9.94, 87.66, 481.77, 24.64]Key words lithium ̄rich manganese ̄based layered cathode materials ꎻ cycle stability ꎻ bulk doping ꎻ surface modification
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[9.65, 374.88, 230.77, 28.97]3 Bulk doping improves the cycle stability of lith ̄ ium ̄rich manganese ̄based materials
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[268.54, 277.08, 216.24, 74.13]Fig.1 Crystal structures and XRD of the ( a) LiTMO2 ꎬ (b) Li 2 MnO3 ̄likeꎬ ( c ) Li 1+ x Ni a Co b Mn c O2 [26~30] ꎻ ( d ) Aberration ̄corrected scanning transmission electron microscopy (STEM) image of the Li [ Li 0􀆰 2 Ni 0􀆰 2 Mn0􀆰6 ] O 2 crystal [31]
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[268.54, 566.43, 216.15, 69.76]Fig.3 ( a) The participation degree of different layered oxides in lattice oxygen during the electrochemical reaction process [42] . (b) Schematic of local atomic coordination and electron band structure of Li ̄excess cathodesꎬ that enables the anionic redox reaction [50]
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[9.94, 70.15, 230.4, 22.93][ 1 ] Ji Mꎬ Xu Yꎬ Zhao Zꎬ Zhang Hꎬ Liu Dꎬ Zhao Cꎬ Qian Xꎬ Zhao C. J. Power Sourcesꎬ 2014ꎬ 263: 296.
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[9.94, 96.74, 230.46, 22.93][ 2 ] Cao Yꎬ Li Mꎬ Lu Jꎬ Liu Jꎬ Amine K. Nat. Nanotech.ꎬ 2019ꎬ 14: 200.
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[9.94, 123.33, 230.4, 22.93][ 3 ] Yuan L Xꎬ Wang Z Hꎬ Zhang W Xꎬ Hu X Lꎬ Chen J Tꎬ Huang Y Hꎬ Goodenough J B. Energ. Environ. Sci.ꎬ 2011ꎬ 4: 269.
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[9.94, 149.92, 230.07, 22.93][ 4 ] Yu S Hꎬ Feng Xꎬ Zhang Nꎬ Seok Jꎬ Abruna H D. Acc. Chem. Res.ꎬ 2018ꎬ 51: 273.
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[9.94, 176.41, 230.46, 22.92][ 5 ] Kim Tꎬ Song Wꎬ Son D Yꎬ Ono L Kꎬ Qi Y. J. Mater. Chem. Aꎬ 2019ꎬ 7: 2942.
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[9.94, 202.99, 230.46, 22.93][ 6 ] Thackeray M Mꎬ Kang S Hꎬ Johnson C Sꎬ Vaughey J Tꎬ Benedek Rꎬ Hackney S A. J. Mater. Chem.ꎬ 2007ꎬ 17: 3112.
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[9.94, 229.58, 230.46, 22.93][ 7 ] Rozier Pꎬ Tarascon J M. J. Electrochem. Soc.ꎬ 2015ꎬ 162: A2490.
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[9.94, 256.17, 230.07, 22.93][ 8 ] Manthiram Aꎬ Knight J Cꎬ Myung S Tꎬ Oh S Mꎬ Sun Y K. Adv. Energy Mater.ꎬ 2016ꎬ 6.
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[9.94, 282.66, 230.39, 36.22][ 9 ] Shi J Lꎬ Xiao D Dꎬ Ge Mꎬ Yu Xꎬ Chu Yꎬ Huang Xꎬ Zhang X Dꎬ Yin Y Xꎬ Yang X Qꎬ Guo Y Gꎬ Gu Lꎬ Wan L. J. Adv. Mater.ꎬ 2018ꎬ 30.
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[9.94, 322.54, 230.4, 22.93]Ito Aꎬ Li Dꎬ Sato Yꎬ Arao Mꎬ Watanabe Mꎬ Hatano Mꎬ Horie Hꎬ Ohsawa Y. J. Power Sourcesꎬ 2010ꎬ 195: 567.
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[9.94, 349.13, 230.46, 36.22]Gu Mꎬ Belharouak Iꎬ Zheng Jꎬ Wu Hꎬ Xiao Jꎬ Genc Aꎬ Amine Kꎬ Thevuthasan Sꎬ Baer D Rꎬ Zhang J Gꎬ Browning N Dꎬ Liu Jꎬ Wang C. ACS Nanoꎬ 2013ꎬ 7: 760.
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[9.94, 389.01, 230.46, 49.42]Gauthier Mꎬ Carney T Jꎬ Grimaud Aꎬ Giordano Lꎬ Pour Nꎬ Chang H Hꎬ Fenning D Pꎬ Lux S Fꎬ Paschos Oꎬ Bauer Cꎬ Magia Fꎬ Lupart Sꎬ Lamp Pꎬ Shao ̄Horn Y. J. Phys. Chem. Lett.ꎬ 2015ꎬ 6: 4653.
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[9.94, 442.09, 230.46, 49.51]Sathiya Mꎬ Abakumov A Mꎬ Foix Dꎬ Rousse Gꎬ Ramesha Kꎬ Saubanere Mꎬ Doublet M Lꎬ Vezin Hꎬ Laisa C Pꎬ Prakash A Sꎬ Gonbeau Dꎬ VanTendeloo Gꎬ Tarascon J M. Nature Mater.ꎬ 2015ꎬ 14: 230.
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[9.94, 508.46, 230.46, 22.93]Thackeray M Mꎬ de Kock Aꎬ Rossouw M Hꎬ Liles Dꎬ Bittihn Rꎬ Hoge D. J. Electrochem. Soc.ꎬ 1992ꎬ 139: 363.
high10156list_itemunknown_textoutside_body_flow_list_itemoutside_body_flow_list_item
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[9.94, 535.05, 230.46, 22.93]Rossouw M Hꎬ Liles D Cꎬ Thackeray M M. J. Solid State Chem.ꎬ 1993ꎬ 104: 464.
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[9.94, 574.93, 230.46, 22.93]Numata Kꎬ Sakaki Cꎬ Yamanaka S. Solid State Ionicsꎬ 1999ꎬ 117: 257.
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[9.94, 601.52, 230.46, 22.93]Kalyani Pꎬ Chitra Sꎬ Mohan Tꎬ Gopukumar S. J. Power Sourcesꎬ 1999ꎬ 80: 103.
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[9.94, 628.01, 230.4, 22.92]Johnson C Sꎬ Kim J Sꎬ Lefief Cꎬ Li Nꎬ Vaughey J Tꎬ Thackeray M M. Electrochem. Commun.ꎬ 2004ꎬ 6: 1085.
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[9.94, 654.6, 230.46, 36.22]Jeom ̄Soo Kꎬ Johnson C Sꎬ Vaughey J Tꎬ Thackeray M Mꎬ Hackney S Aꎬ Wonsub Yꎬ Grey C P. Chem. Mater.ꎬ 2004ꎬ 16: 1996.
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[9.94, 694.48, 230.36, 22.92]Thackeray M Mꎬ Johnson C Sꎬ Vaughey J Tꎬ Li Nꎬ Hackney S A. J. Mater. Chem.ꎬ 2005ꎬ 15: 2257.
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[9.94, 721.06, 230.07, 22.83]Park C Wꎬ Kim S Hꎬ Mangani I Rꎬ Lee J Hꎬ Boo Sꎬ Kim J. Mater. Res. Bull.ꎬ 2007ꎬ 42: 1374.
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[261.46, 55.89, 230.4, 22.93]Guo X Jꎬ Li Y Xꎬ Zheng Mꎬ Zheng J Mꎬ Li Jꎬ Gong Z Lꎬ Yang Y. J. Power Sourcesꎬ 2008ꎬ 184: 414.
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[261.46, 82.48, 230.46, 22.92]Jacob Cꎬ Jian Jꎬ Zhu Yꎬ Su Qꎬ Wang H. J.Mater. Chem. Aꎬ 2014ꎬ 2: 2283.
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[261.46, 109.06, 230.46, 22.93]Yu Hꎬ Ishikawa Rꎬ So Y Gꎬ Shibata Nꎬ Kudo Tꎬ Zhou Hꎬ Ikuhara Y. Angew. Chem. Int. Ed. Engl.ꎬ 2013ꎬ 52: 5969.
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[261.46, 135.65, 230.07, 22.93]Huang Z Dꎬ Liu X Mꎬ Zhang Bꎬ Oh S Wꎬ Ma P Cꎬ Kim J K. Scripta Mater.ꎬ 2011ꎬ 64: 122.
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[261.46, 162.24, 230.46, 22.93]Boulineau Aꎬ Croguennec Lꎬ Delmas Cꎬ Weill F. Chem. Mater.ꎬ 2009ꎬ 21: 4216.
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[261.46, 202.22, 230.36, 22.93]Jarvis K Aꎬ Deng Zꎬ Allard L Fꎬ Manthiram Aꎬ Ferreira P J. J. Mater. Chem.ꎬ 2012ꎬ 22: 11550.
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[261.46, 228.81, 230.07, 22.93]Jarvis K Aꎬ Deng Zꎬ Allard L Fꎬ Manthiram Aꎬ Ferreira P J. Chem. Mater.ꎬ 2011ꎬ 23: 3614.
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[261.46, 255.39, 230.46, 22.93]Thackeray M Mꎬ Kang S Hꎬ Johnson C Sꎬ Vaughey J Tꎬ Hackney S A. Electrochem. Commun.ꎬ 2006ꎬ 8: 1531.
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[261.46, 281.98, 230.46, 22.92]Thackeray M Mꎬ Kang S Hꎬ Johnson C Sꎬ Vaughey J Tꎬ Benedek Rꎬ Hackney S A. J. Mater. Chem.ꎬ 2007ꎬ 17.
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[261.46, 308.57, 230.36, 22.93]Yu Hꎬ Kim Hꎬ Wang Yꎬ He Pꎬ Asakura Dꎬ Nakamura Yꎬ Zhou H. PCCPꎬ 2012ꎬ 14: 6584.
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[261.46, 335.25, 230.39, 22.93]Mohanty Dꎬ Huq Aꎬ Payzant E Aꎬ Sefat A Sꎬ Li Jꎬ Abraham D Pꎬ Wood D Lꎬ IIIꎬ Daniel C. Chem. Mater.ꎬ 2013ꎬ 25: 4064.
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[261.46, 361.84, 230.46, 22.92]Lu Z Hꎬ Chen Z Hꎬ Dahn J R. Chem. Materialsꎬ 2003ꎬ 15: 3214.
high10179list_itembody_candidate_excludedoutside_body_flow_body_candidateoutside_body_flow_body_candidate
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[261.46, 388.43, 230.46, 36.22]Johnson C Sꎬ Kim J Sꎬ Kropf A Jꎬ Kahaian A Jꎬ Vaughey J Tꎬ Fransson L M Lꎬ Edstrom Kꎬ Thackeray M M. Chem. Mater.ꎬ 2003ꎬ 15: 2313.
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[261.46, 428.31, 230.07, 22.92]Yabuuchi Nꎬ Yoshii Kꎬ Myung S Tꎬ Nakai Iꎬ Komaba S. J. Am. Chem. Soc.ꎬ 2011ꎬ 133: 4404.
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[261.46, 454.9, 230.46, 23.02]Genevois Cꎬ Koga Hꎬ Croguennec Lꎬ Menetrier Mꎬ Delmas Cꎬ Weill F. J. Phys. Chem. Cꎬ 2015ꎬ 119: 75.
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[261.46, 494.88, 230.07, 22.92]Sharifi ̄Asl Sꎬ Lu Jꎬ Amine Kꎬ Shahbazian ̄Yassar R. Adv. Energy Mater.ꎬ 2019ꎬ 9.
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[261.46, 521.46, 230.46, 22.93]Qiu Bꎬ Zhang Mꎬ Xia Yꎬ Liu Zꎬ Meng Y S. Chem. Mater.ꎬ 2017ꎬ 29: 908.
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[261.46, 548.05, 230.46, 36.22]Pearce P Eꎬ Perez A Jꎬ Rousse Gꎬ Saubanere Mꎬ Batuk Dꎬ Foix Dꎬ McCalla Eꎬ Abakumov A Mꎬ Van Tendeloo Gꎬ Doublet M Lꎬ Tarascon J M. Nature Mater.ꎬ 2017ꎬ 16: 580.
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[261.46, 587.93, 230.07, 22.93]Saubanere Mꎬ McCalla Eꎬ Tarascon J Mꎬ Doublet M L. Energ. Environ. Sci.ꎬ 2016ꎬ 9: 984.
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[261.46, 614.62, 230.07, 22.93]Wu Yꎬ Ma Cꎬ Yang Jꎬ Li Zꎬ Allard L Fꎬ Liang Cꎬ Chi M. J. Mater. Chem. Aꎬ 2015ꎬ 3: 5385.
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[261.46, 641.2, 205.52, 9.63]Kim J Hꎬ Sun Y K. J. Power Sourcesꎬ 2003ꎬ 119: 166.
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[261.46, 654.5, 230.07, 22.93]Hong Y Sꎬ Park Y Jꎬ Ryu K Sꎬ Chang S Hꎬ Kim M G. J. Mater. Chem.ꎬ 2004ꎬ 14: 1424.
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[261.46, 681.09, 230.07, 22.93]Nayak P Kꎬ Grinblat Jꎬ Levi Mꎬ Markovsky Bꎬ Aurbach D. J. Electrochem. Soc.ꎬ 2014ꎬ 161: A1534.
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[9.94, 111.98, 165.74, 14.16]鲁志远 刘燕妮 廖世军 ∗ ∗鲁志远 刘燕妮 廖世军 ∗ ∗
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[9.94, 132.88, 349.62, 12.76]( 华南理工大学化学与化工学院 广东省燃料电池重点实验室 广州 510641 )( 华南理工大学化学与化工学院 广东省燃料电池重点实验室 广州 510641 )
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[9.94, 274.26, 345.64, 9.16]关键词 富锂锰基层状正极材料 循环稳定性 体相掺杂 表面修饰关键词 富锂锰基层状正极材料 循环稳定性 体相掺杂 表面修饰
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[9.94, 289.88, 52.2, 9.0]中图分类号中图分类号
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[9.94, 373.53, 165.54, 14.4]Zhiyuan Lu ꎬ Yanni Liu ꎬ Shijun Liao ∗ ∗
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[9.65, 245.34, 65.4, 12.76]1 Introduction
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[9.65, 261.55, 230.59, 45.17]2 Structural characteristic and electrochemical behaviors of lithium ̄rich manganese ̄based materials
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[9.65, 310.16, 230.66, 28.97]2􀆰 1 Lithium ̄rich manganese ̄based materials and its structural characteristic
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[9.65, 342.47, 182.56, 12.76]2􀆰 2 Charge ̄discharge reaction mechanism
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[9.65, 358.68, 201.78, 12.76]2􀆰 3 Structural evolution and decay mechanism
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[9.65, 407.29, 83.64, 12.76]3􀆰 1 Li site doping
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[9.65, 423.5, 88.78, 12.76]3􀆰 2 TM site doping
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[9.65, 439.7, 81.99, 12.76]3􀆰 3 O site doping
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[9.65, 455.81, 230.59, 28.97]4 Surface modification improves the cycle stability of lithium ̄rich manganese ̄based materials.
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[9.65, 488.22, 89.17, 12.76]4􀆰 1 Surface coating
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[9.65, 504.43, 98.23, 12.76]4􀆰 2 Surface treatment
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[9.65, 520.63, 93.87, 12.76]5 A joint mechanism
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[9.65, 536.84, 112.85, 12.76]6 Conclusion and outlook
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[261.17, 470.66, 193.68, 12.76]2􀆰 1 富锂锰基层状正极材料及其结构特征2􀆰 1 富锂锰基层状正极材料及其结构特征
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[261.46, 188.83, 204.06, 9.63]Choi J Wꎬ Aurbach D. Nature Rev. Materialsꎬ 2016ꎬ 1.
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[261.46, 481.58, 201.06, 9.63]Assat Gꎬ Tarascon J M. Nature Energyꎬ 2018ꎬ 3: 373.
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[35.27, 55.89, 72.97, 9.63]Chem.ꎬ 2016ꎬ 8: 692.
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[261.46, 306.63, 174.27, 9.63]Zhu Zꎬ Cai Fꎬ Yu J. Ionicsꎬ 2016ꎬ 22: 1353.
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[261.46, 438.6, 195.82, 9.63]Okamoto Y. J. Electrochem. Soc.ꎬ 2012ꎬ 159: A152.
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[9.94, 11.74, 96.25, 25.99]PROGRESS IN CHEMISTRY
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[436.9, 27.11, 52.21, 9.22]化 学 进 展化 学 进 展
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[403.81, 45.12, 88.05, 9.63]DOI : 10􀆰 7536/ PC200220
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[10.43, 70.11, 409.88, 21.74]锂离子电池富锂锰基层状正极材料的稳定性 ∗锂离子电池富锂锰基层状正极材料的稳定性 ∗
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[9.94, 321.67, 481.63, 31.02]Enhancing the Stability of Lithium ̄Rich Manganese ̄Based Layered Cathode Materials for Li ̄Ion Batteries Application ∗
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[25.86, 646.35, 286.84, 9.63]收稿 : 2020 年 2 月 24 日 ꎬ 收修改稿 : 2020 年 6 月 5 日 ꎬ 网络出版 : 2020 年 9 月 2 日收稿 : 2020 年 2 月 24 日 ꎬ 收修改稿 : 2020 年 6 月 5 日 ꎬ 网络出版 : 2020 年 9 月 2 日
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[17.9, 659.54, 473.92, 22.83]∗ 国家重点研发计划项目 (No. 2017YFB0102900ꎬ 2016YFB0101201)、 国家自然科学基金项目 (No. 21476088ꎬ 21776104)、 广东省科学技术厅 (No. 2015B010106012) 和广州市科技创新委员会 (No. 201504281614372ꎬ 2016GJ006) 资助∗ 国家重点研发计划项目 (No. 2017YFB0102900ꎬ 2016YFB0101201)、 国家自然科学基金项目 (No. 21476088ꎬ 21776104)、 广东省科学技术厅 (No. 2015B010106012) 和广州市科技创新委员会 (No. 201504281614372ꎬ 2016GJ006) 资助
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[25.66, 685.94, 466.2, 36.02]The work was supported by the National Key Research and Development Program of China ( No. 2017YFB0102900ꎬ 2016YFB0101201)ꎬ the National Natural Science Foundation of China (No. 21476088ꎬ 21776104)ꎬ the Guangdong Provincial Department of Science and Technology (No. 2015B010106012)ꎬ and the Guangzhou Science Technology and Innovation Committee (No. 201504281614372ꎬ 2016GJ006).
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[13.92, 725.53, 174.47, 9.63]∗ ∗Corresponding author e ̄mail: chsjliao@ scut.edu.cn
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[214.49, 752.8, 93.54, 9.63]http : / / www.progchem.ac.cn
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[324.14, 752.8, 167.68, 9.63]Progress in Chemistry ꎬ 2020ꎬ 32(10): 1504~1514
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[9.94, 30.41, 211.83, 10.96]鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性
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[434.18, 29.93, 52.2, 9.22]综述与评论综述与评论
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[9.94, 229.24, 39.12, 8.87]Contents
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[9.65, 560.43, 42.11, 10.36]1 引言1 引言
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[261.17, 431.47, 230.65, 28.21]2 富锂锰基层状正极材料的结构特性及电 化学行为2 富锂锰基层状正极材料的结构特性及电 化学行为
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[465.62, 752.8, 26.2, 9.63]􀅰 1505 􀅰
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[19.74, 27.4, 35.06, 9.03]Review
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[9.94, 752.8, 26.2, 9.63]􀅰 1506 􀅰
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[439.71, 27.4, 52.2, 9.22]化 学 进 展化 学 进 展
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[261.17, 460.76, 193.68, 12.76]2􀆰 2 富锂锰基层状正极材料的充放电反应2􀆰 2 富锂锰基层状正极材料的充放电反应
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[324.14, 752.8, 167.68, 9.63]Progress in Chemistry ꎬ 2020ꎬ 32(10): 1504~1514
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[9.94, 30.41, 211.83, 10.96]鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性
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[17.03, 342.57, 216.1, 26.09]图 2 (a) 富锂锰基正极材料典型的第 1、2 圈充放电曲 线 ꎻ(b) 前两次循环的容量  ̄ 电压微分曲线 [48]图 2 (a) 富锂锰基正极材料典型的第 1、2 圈充放电曲 线 ꎻ(b) 前两次循环的容量  ̄ 电压微分曲线 [48]
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[17.03, 371.98, 216.13, 54.62]Fig. 2 Lithium ̄rich manganese ̄based layered cathode materials (a) galvanostatic charge ̄discharge voltage profiles measured at 0􀆰 1 Cꎬ (b) differential capacity (d Q / d V vs E) plots obtained from voltage profiles [48]
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[9.94, 752.8, 129.35, 9.63]化学进展 ꎬ 2020ꎬ 32(10): 1504~1514化学进展 ꎬ 2020ꎬ 32(10): 1504~1514
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[434.18, 29.93, 52.2, 9.22]综述与评论综述与评论
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[268.54, 521.89, 216.1, 38.49]图 3 (a) 在电化学反应过程中不同层状氧化物的晶格 氧参与程度 [42] ꎻ(b) 锂过量正极的局域原子配位和电子 带结构示意图 [50]图 3 (a) 在电化学反应过程中不同层状氧化物的晶格 氧参与程度 [42] ꎻ(b) 锂过量正极的局域原子配位和电子 带结构示意图 [50]
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[261.17, 650.56, 230.65, 25.28]2􀆰 3 富锂锰基层状正极材料的结构演变及衰减 机理2􀆰 3 富锂锰基层状正极材料的结构演变及衰减 机理
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[465.62, 752.8, 26.2, 9.63]􀅰 1507 􀅰
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[19.74, 27.4, 35.06, 9.03]Review
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[9.94, 752.8, 26.2, 9.63]􀅰 1508 􀅰
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[439.71, 27.4, 52.2, 9.22]化 学 进 展化 学 进 展
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[268.54, 207.89, 216.1, 23.35]图 4 富锂层状正极材料在循环过程中结构的变化机 理 [60]图 4 富锂层状正极材料在循环过程中结构的变化机 理 [60]
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[268.54, 237.29, 216.13, 26.09]Fig.4 The mechanism of the lithium ̄rich layered cathode materials change during the cycle [60]
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[261.17, 532.87, 230.65, 27.63]3 掺杂提升富锂锰基层状正极材料的循环 稳定性3 掺杂提升富锂锰基层状正极材料的循环 稳定性
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[261.17, 712.18, 89.08, 12.76]3􀆰 1 锂 (Li) 位掺杂3􀆰 1 锂 (Li) 位掺杂
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[324.14, 752.8, 167.68, 9.63]Progress in Chemistry ꎬ 2020ꎬ 32(10): 1504~1514
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[9.94, 30.41, 211.83, 10.96]鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性
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[17.03, 667.54, 216.21, 68.89]Fig. 5 ( aꎬ b ) The charge ̄discharge curves of the unmodified anode material ( PLR ) and modified anode material (SLR) at 0.1 Cꎬ respectively. (cꎬ e) the charge ̄ discharge curves and cycling stability tested at 0. 2 C and (d) rate performance of PLR and SLR [68]
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[9.94, 752.8, 129.35, 9.63]化学进展 ꎬ 2020ꎬ 32(10): 1504~1514化学进展 ꎬ 2020ꎬ 32(10): 1504~1514
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[434.18, 29.93, 52.2, 9.22]综述与评论综述与评论
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[261.17, 182.76, 125.66, 12.76]3􀆰 2 过渡金属 (TM) 位掺杂3􀆰 2 过渡金属 (TM) 位掺杂
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[261.17, 637.95, 87.43, 12.76]3􀆰 3 氧 (O) 位掺杂3􀆰 3 氧 (O) 位掺杂
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[465.62, 752.8, 26.2, 9.63]􀅰 1509 􀅰
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[19.74, 27.4, 35.06, 9.03]Review
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[9.65, 583.23, 230.65, 27.63]4 表面修饰提升富锂锰基层状正极材料循 环稳定性4 表面修饰提升富锂锰基层状正极材料循 环稳定性
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[9.94, 752.8, 26.2, 9.63]􀅰 1510 􀅰
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[439.71, 27.4, 52.2, 9.22]化 学 进 展化 学 进 展
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[261.17, 181.98, 67.93, 12.76]4􀆰 1 表面包覆4􀆰 1 表面包覆
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[261.17, 402.05, 88.69, 12.76]4􀆰 1􀆰 1 碳材料包覆4􀆰 1􀆰 1 碳材料包覆
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[324.14, 752.8, 167.68, 9.63]Progress in Chemistry ꎬ 2020ꎬ 32(10): 1504~1514
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[9.94, 30.41, 211.83, 10.96]鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性
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[17.03, 268.25, 98.73, 9.67]图 6 碳包覆示意图 [78]图 6 碳包覆示意图 [78]
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[17.03, 283.38, 137.26, 12.41]Fig.6 Illustration of the C ̄coating [78]
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[9.65, 312.39, 104.41, 12.76]4􀆰 1􀆰 2 氧 / 氟化物包覆4􀆰 1􀆰 2 氧 / 氟化物包覆
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[9.65, 665.6, 107.71, 12.79]4􀆰 1􀆰 3 AlPO4 材料包覆4􀆰 1􀆰 3 AlPO4 材料包覆
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[9.94, 752.8, 129.35, 9.63]化学进展 ꎬ 2020ꎬ 32(10): 1504~1514化学进展 ꎬ 2020ꎬ 32(10): 1504~1514
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[434.18, 29.93, 52.2, 9.22]综述与评论综述与评论
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[261.17, 244.86, 67.93, 12.76]4􀆰 2 表面处理4􀆰 2 表面处理
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[465.62, 752.8, 26.2, 9.63]􀅰 1511 􀅰
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[19.74, 27.4, 35.06, 9.03]Review
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[9.65, 63.22, 90.24, 10.36]5 联合改性机制5 联合改性机制
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[439.71, 27.4, 52.2, 9.22]化 学 进 展化 学 进 展
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[261.17, 229.73, 78.21, 10.36]6 结论与展望6 结论与展望
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[9.94, 506.08, 481.91, 23.47]表 1 近年来关于富锂锰基正极材料改性策略的代表性研究工作及其相关材料的主要电化学性能 Table 1 Electrochemical performance of typical modification research works about lithium ̄rich manganese ̄based layered cathode表 1 近年来关于富锂锰基正极材料改性策略的代表性研究工作及其相关材料的主要电化学性能 Table 1 Electrochemical performance of typical modification research works about lithium ̄rich manganese ̄based layered cathode
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[9.94, 531.11, 87.26, 10.96]materials in recent years
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[9.94, 752.8, 26.2, 9.63]􀅰 1512 􀅰
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[324.14, 752.8, 167.68, 9.63]Progress in Chemistry ꎬ 2020ꎬ 32(10): 1504~1514
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[9.94, 30.41, 211.83, 10.96]鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性鲁志远等 : 锂离子电池富锂锰基层状正极材料的稳定性
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[99.31, 56.03, 51.62, 7.73]参 考 文 献参 考 文 献
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[9.94, 752.8, 129.35, 9.63]化学进展 ꎬ 2020ꎬ 32(10): 1504~1514化学进展 ꎬ 2020ꎬ 32(10): 1504~1514
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[434.18, 29.93, 52.2, 9.22]综述与评论综述与评论
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[465.62, 752.8, 26.2, 9.63]􀅰 1513 􀅰
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[19.74, 27.4, 35.06, 9.03]Review
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[9.94, 752.8, 26.2, 9.63]􀅰 1514 􀅰
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[439.71, 27.4, 52.2, 9.22]化 学 进 展化 学 进 展
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[324.14, 752.8, 167.68, 9.63]Progress in Chemistry ꎬ 2020ꎬ 32(10): 1504~1514